Related papers: Nonlinear optical response in higher fullerenes
Optical non-linearities, such as thermo-optic effects and free-carrier-dispersion, are often considered as undesired effects in silicon-based resonators and, more specifically, optomechanical (OM) cavities, affecting the relative detuning…
The recent advances in modelling nonlinear interference of systems operating beyond the C-band are discussed. Estimation accuracy as well as computational complexity of current approaches are compared and addressed.
Simultaneous measurements of the intensity and phase of a probe wave reflected from an interface between silica and elemental alpha-gallium reveal its very strong optical nonlinearity, affecting both these parameters of the reflected wave.…
Considering the photoionization of Ar@C60, we predict resonant femtosecond decays of both Ar and C60 vacancies through the continua of atom-fullerene hybrid final states. The resulting resonances emerge from the interference between…
Nonlinear optical (NLO) phenomena such as harmonic generation, Kerr, and Pockels effects are of great technological importance for lasers, frequency converters, modulators, switches, etc. Recently, two-dimensional (2D) materials have drawn…
We present a full formalism for the calculation of the linear and second-order optical response for semiconductors and insulators. The expressions for the optical susceptibilities are derived within perturbation theory. As a starting point…
It is well known that collective electronic excitations in fullerene C$_{60}$ are manifested as Mie plasmons, and in graphene (the limiting case of an infinitely large fullerene) collective excitations are of plasmon-polariton type. How the…
The formation and evolution mechanism of fullerenes in the planetary nebula or in the interstellar medium are still not understood. Here we present the study on the cluster formation and the relative reactivity of fullerene cations (from…
We investigate the effect of phenomenological relaxation parameters on the third order optical nonlinearity of doped graphene by perturbatively solving the semiconductor Bloch equation around the Dirac points. An analytic expression for the…
A density-matrix formalism within the length gauge is developed for the purpose of calculating the nonlinear response of intrinsic bilayer graphene at terahertz frequencies. Employing a tight-binding model, we find that interplay between…
Two-dimensional materials constitute an exciting platform for nonlinear optics with large nonlinearities that are tunable by gating. Hence, gate-tunable harmonic generation and intensity-dependent refraction have been observed in e.g.…
We compute from first principles the infrared dispersion of the nonlinear susceptibility $\chi^{(2)}$ in zincblende semiconductors. At terahertz frequencies the nonlinear susceptibility depends not only on the purely electronic response…
Fullerenes, including \ce{C60} and \ce{C70}, have been detected in various astronomical environments. Understanding how their structures evolve over time is essential for gaining insights into their life cycle and making further…
We propose a new concept to generate efficient one-third harmonic light from an unseeded third harmonic process in optical fibers. Our concept is based on the dynamic constant (Hamiltonian) of the nonlinear third harmonic generation in…
Nonlinear optical effects provide a natural way of light manipulation and interaction, and form the foundation of applied photonics -- from high-speed signal processing and telecommunication, to ultra-high bandwidth interconnects and…
We present a method, based on noncollinear second harmonic generation, to evaluate the non-zero elements of the nonlinear optical susceptibility. At a fixed incidence angle, the generated signal is investigated by varying the polarization…
Nonlinear optics is a rapidly growing field that has found a wide range of applications. A major limitation, however, is the demand of high power, especially for high-order nonlinearities. Here, by reconfiguring a multiple-scattering…
Using a hydrodynamic approach we examine bulk- and surface-induced second and third harmonic generation from semiconductor nanowire gratings having a resonant nonlinearity in the absorption region. We demonstrate resonant, broadband and…
Nonlinear optical phenomena play important roles in the vast emerging fields of micro- and nano-technology. This paper describes the general characteristics of nonlinear optical materials and systems, with a focus on parametric…
Although massless Dirac fermions in graphene constitute a centrosymmetric medium for in-plane excitations, their second-order nonlinear optical response is nonzero if the effects of spatial dispersion are taken into account. Here we present…