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We present parameter-free LDA+DMFT results for the many-particle density of states of cubic SrVO3 and orthorhombic CaVO3. Both systems are found to be strongly correlated metals, but em not on the verge of a metal-insulator transition. In…

Strongly Correlated Electrons · Physics 2007-05-23 I. A. Nekrasov , G. Keller , D. E. Kondakov , A. V. Kozhevnikov , Th. Pruschke , K. Held , D. Vollhardt , V. I. Anisimov

We study the transfer of spectral weight in the optical spectra of a strongly correlated electron system as a function of temperature and interaction strength. Within a dynamical mean field theory of the Hubbard model that becomes exact in…

Condensed Matter · Physics 2009-10-28 M. J. Rozenberg , G. Kotliar , H. Kajueter , G. A. Thomas , D. H. Rapkine , J. M. Honig , P. Metcalf

Ca1-xSrxVO3 is a Mott-Hubbard-type correlated electron system whose bandwidth can be varied by the V-O-V bond angle, but the actual effect of bandwidth control on the electronic structure has been controversial in previous photoemission…

Strongly Correlated Electrons · Physics 2015-05-18 T. Yoshida , M. Hashimoto , T. Takizawa , A. Fujimori , M. Kubota , K. Ono , H. Eisaki

The evolution of electron correlation in Sr$_{x}$Ca$_{1-x}$VO$_3$ has been studied using a combination of bulk-sensitive resonant soft x-ray emission spectroscopy (RXES), surface-sensitive photoemission spectroscopy (PES), and ab initio…

Strongly Correlated Electrons · Physics 2013-07-25 J. Laverock , B. Chen , K. E. Smith , R. P. Singh , G. Balakrishnan , M. Gu , J. W. Lu , S. A. Wolf , R. M. Qiao , W. Yang , J. Adell

We study the transfer of spectral weight in the photoemission and optical spectra of strongly correlated electron systems. Within the LISA, that becomes exact in the limit of large lattice coordination, we consider and compare two models of…

Condensed Matter · Physics 2009-10-28 M. J. Rozenberg , G. Kotliar , H. Kajueter

Optical conductivity spectra of single crystals of Ca_1-xSr_xVO_3 have been studied to elucidate how the electronic behavior depends on the strength of the electron correlation without changing the nominal number of electrons per vanadium…

Strongly Correlated Electrons · Physics 2009-10-31 H. Makino , I. H. Inoue , M. J. Rozenberg , Y. Aiura , I. Hase , S. Onari

The ultrafast response of the prototype Mott-Hubbard system (V1-xCrx)2O3 was systematically studied with fs pump-probe reflectivity, allowing us to clearly identify the effects of the metal-insulator transition on the transient response.…

Strongly Correlated Electrons · Physics 2011-08-29 B. Mansart , D. Boschetto , S. Sauvage , A. Rousse , M. Marsi

The dynamical mean-field theory together with the non-crossing approximation is used to set up a novel scheme to study the electronic structure of strongly correlated electron systems. The non-interacting band structure is obtained from a…

Strongly Correlated Electrons · Physics 2007-05-23 M. B. Zoelfl , Th. Pruschke , J. Keller , A. I. Poteryaev , I. A. Nekrasov , V. I. Anisimov

Single crystals of the perovskite-type $3d^{1}$ metallic alloy system Ca$_{1-x}$Sr$_x$VO$_3$ were synthesized in order to investigate metallic properties near the Mott transition. The substitution of a Ca$^{2+}$ ion for a Sr$^{2+}$ ion…

Strongly Correlated Electrons · Physics 2009-10-31 I. H. Inoue , O. Goto , H. Makino , N. E. Hussey , M. Ishikawa

We have measured soft x-ray photoemission and O 1{\it s} x-ray absorption spectra of Ca$_{1-x}$Sr$_x$RuO$_3$ thin films prepared {\it in situ}. The coherent and incoherent parts have been identified in the bulk component of the…

Strongly Correlated Electrons · Physics 2009-11-10 M. Takizawa , D. Toyota , H. Wadati , A. Chikamatsu , H. Kumigashira , A. Fujimori , M. Oshima , Z. Fang , M. Lippmaa , M. Kawasaki , H. Koinuma

A phenomenological approach is presented that allows one to model, and thereby interpret, photoemission spectra of strongly correlated electron systems. A simple analytical formula for the self-energy is proposed. This self-energy describes…

Strongly Correlated Electrons · Physics 2009-11-07 Krzysztof Byczuk , Ralf Bulla , Ralph Claessen , Dieter Vollhardt

We study the electronic structure of Mott-Hubbard systems SrVO$_{3}$ and CaVO$_3$ with bulk and surface-sensitive high-resolution photoemission spectroscopy (PES), using a VUV laser, synchrotron radiation and a discharge lamp ($h\nu$ = 7 -…

Understanding the physics of strongly correlated electronic systems has been a central issue in condensed matter physics for decades. In transition metal oxides, strong correlations characteristic of narrow $d$ bands is at the origin of…

Strongly Correlated Electrons · Physics 2021-05-05 Mathieu Mirjolet , Francisco Rivadulla , Premysl Marsik , Vladislav Borisov , Roser Valenti , Josep Fontcuberta

We present parameter-free LDA+DMFT (local density approximation + dynamical mean field theory) results for the many-body spectra of cubic SrVO3 and orthorhombic CaVO3. Both systems are found to be strongly correlated metals, but not on the…

Strongly Correlated Electrons · Physics 2009-11-11 I. A. Nekrasov , G. Keller , D. E. Kondakov , A. V. Kozhevnikov , Th. Pruschke , K. Held , D. Vollhardt , V. I. Anisimov

We report the temperature dependence of transport and magnetic properties of La$_{1-x}$Ca$_x$VO$_3$ for x = 0.0, 0.1, 0.2, 0.3, 0.4 and 0.5. The system exhibits an insulator-to-metal transition concomitant with an…

Strongly Correlated Electrons · Physics 2008-02-03 K. Maiti , N. Y. Vasanthacharya , D. D. Sarma

Recent photoemission experiments have shown strong surface modifications in the spectra from vanadium oxides as (V,Cr)_2O_3 or (Sr,Ca)VO_3. The effective mass is enhanced at the surface and the coherent part of the surface spectrum is…

Strongly Correlated Electrons · Physics 2009-11-10 S. Schwieger , M. Potthoff , W. Nolting

We studied the electronic structure of the Ca1-xSrxVO3 series using a cluster model. Both the coherent and incoherent structures in photoemission correspond to well screened states. The coherent structure (3d1/u(C)) is mostly due to a…

Strongly Correlated Electrons · Physics 2007-05-23 R. J. O. Mossanek , M. Abbate , A. Fujimori

V2O3 is an archetypal system for the study of correlation induced, Mott-Hubbard metal-insulator transitions. Despite decades of extensive investigations, the accurate description of its electronic properties remains an open problem in the…

We report hard x-ray photoemission spectroscopy measurements of the electronic structure of the prototypical correlated oxide SrxCa1-xVO3. By comparing spectra recorded at different excitation energies, we show that 2.2 keV photoelectrons…

Strongly Correlated Electrons · Physics 2015-04-22 J. Laverock , J. Kuyyalil , B. Chen , R. P. Singh , G. Balakrishnan , B. Karlin , J. C Woicik , K. E. Smith

The doping and temperature dependent optical conductivity spectra of the quasi-two-dimensional Ca_{2-x}Sr_xRuO_4 (0.0=<x=<2.0) system were investigated. In the Mott insulating state, two electron correlation-induced peaks were observed…

Strongly Correlated Electrons · Physics 2009-11-07 J. S. Lee , Y. S. Lee , T. W. Noh , S. -J. Oh , Jaejun Yu , S. Nakatsuji , H. Fukazawa , Y. Maeno
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