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The phase behavior of asymmetrically interacting ABC star triblock copolymer melts is investigated by the self-consistent field theory (SCFT). Motivated by the experimental systems, in this study, we focus on the systems in which the…

Soft Condensed Matter · Physics 2015-08-25 Kai Jiang , Juan Zhang , Qin Liang

According to the universality hypothesis, the phase behavior of different block copolymer melt models having fixed composition depends solely on two parameters: the invariant chain length $\bar{N}$ and the effective interaction parameter…

Soft Condensed Matter · Physics 2024-08-16 Artem Petrov , Hejin Huang , Alfredo Alexander-Katz

Two-dimensional monodisperse linear polymer chains are known to adopt for sufficiently large chain lengths $N$ and surface fractions $\phi$ compact configurations with fractal perimeters. We show here by means of Monte Carlo simulations of…

Soft Condensed Matter · Physics 2025-08-04 J. P. Wittmer , A. Cavallo , A. Johner

We develop connections between the qualitative dynamics of Hamiltonian isotopies on a surface $\Sigma$ and their chain-level Floer theory using ideas drawn from Hofer-Wysocki-Zehnder's theory of finite energy foliations. We associate to…

Symplectic Geometry · Mathematics 2024-06-03 Dustin Connery-Grigg

We investigate the properties of a system of semi-diluted polymers in the presence of charged groups and counter-ions, by means of self-consistent field theory. We study a system of polyelectrolyte chains grafted to a similarly, as well as…

Soft Condensed Matter · Physics 2015-05-19 Gabriele Migliorini

A theoretical study on the phase behaviors of a polymer solution confined between two coaxial cylindrical walls is presented. For the case of a neutral inner cylinder, the spinodal point derived through the Gaussian fluctuation theory is…

Soft Condensed Matter · Physics 2009-09-23 Tongchuan Suo , Dadong Yan

Mesoscopic theory for soft-matter systems that combines density functional and statistical field theory is derived from the microscopic theory by a systematic coarse-graining procedure. Within the framework of this theory we obtain the…

Soft Condensed Matter · Physics 2013-05-29 A. Ciach

Inhomogeneous polymers play an important role in various cellular processes, both in nature and in biotechnological applications. At finite temperatures, inhomogeneous polymers exhibit non-trivial thermal fluctuations. In a broader context,…

Statistical Mechanics · Physics 2017-02-02 Yohai Bar-Sinai , Eran Bouchbinder

We study and predict the interfacial tension, solubility parameters and Flory-Huggins parameters of binary mixtures as functions of pressure and temperature, using multiscale numerical simulation. A mesoscopic approach is proposed for…

Chemical Physics · Physics 2016-02-19 E. Mayoral , E. Nahmad-Achar

Polymer networks formed by cross linking flexible polymer chains are ubiquitous in many natural and synthetic soft-matter systems. Current micromechanics models generally do not account for excluded volume interactions except, for instance,…

Soft Condensed Matter · Physics 2023-06-05 Pratik Khandagale , Timothy Breitzman , Carmel Majidi , Kaushik Dayal

We present a self-consistent field theory (SCFT) of semiflexible (wormlike) diblock copolymers, each consisting of a rigid and a flexible part. The segments of the polymers are otherwise identical, in particular with regard to their…

Soft Condensed Matter · Physics 2009-11-07 Dominik Düchs , D. E. Sullivan

Taking into account the well known correspondence between the field theoretical O(n)-vector model in the limit $n\to 0$ and the behavior of long-flexible polymer chains in a good solvent the investigation of ideal polymer chains adsorption…

Soft Condensed Matter · Physics 2012-09-25 Zoryana Usatenko

The paper presents a short overview of the theoretical, numerical and experimental works on the critical behavior of a dilute polymer solution of long-flexible polymer chains confined in semi-infinite space restricted by a surface or in a…

Soft Condensed Matter · Physics 2018-01-08 Zoryana Usatenko , Krzysztof S. Danel

More than half of a century has passed since the free energy of classical fluids defined by second Legendre transform was derived as a functional of density-density correlation function. It is now becoming an increasingly significant issue…

Statistical Mechanics · Physics 2018-12-05 Hiroshi Frusawa

The conformational properties of a semi-flexible polymer chain, anchored at one end in a uniform force field, are studied in a simple two-dimensional model. Recursion relations are derived for the partition function and then iterated…

Soft Condensed Matter · Physics 2009-11-07 A. Lamura , T. W. Burkhardt , G. Gompper

In the paper we investigate statistical and topological properties of fractional Brownian polymer chains, equipped with the short-range volume interactions. The attention is paid to statistical properties of collapsed conformations with the…

Soft Condensed Matter · Physics 2021-06-09 A. M. Astakhov , V. A. Avetisov , S. K. Nechaev , K. E. Polovnikov

We present numerical calculations of lamellar phases of block copolymers at patterned surfaces. We model symmetric di-block copolymer films forming lamellar phases and the effect of geometrical and chemical surface patterning on the…

Soft Condensed Matter · Physics 2016-02-18 Xingkun Man , David Andelman , Henri Orland

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

Field-theoretical method is efficient in predicting the assembling structures of polymeric systems. However, for the polymer/nanoparticle mixture, the continuous density description is not suitable to capture the realistic assembly of…

Soft Condensed Matter · Physics 2017-05-17 Hui-shu Li , Bo-kai Zhang , Jian Li , Wen-de Tian , Kang Chen

The properties of diluted symmetric A-B diblock copolymers at the interface between A and B homopolymer phases are studied by means of Monte Carlo (MC) simulations of the bond fluctuation model. We calculate segment density profiles as well…

Chemical Physics · Physics 2015-06-26 A. Werner , F. Schmid , K. Binder , M. Mueller
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