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We study analytically a continuum model for phase-separation in binary polymer blends based on the Flory-Huggins-De Gennes free energy, by means of the self-consistent large-$n$ limit approach. The model is solved for values of the…

Statistical Mechanics · Physics 2009-10-30 Claudio Castellano , Federico Corberi

The evolution of the microstructure due to spinodal decomposition in phase separated mixtures has a strong impact on the final material properties. In the late stage of coarsening, the system is characterized by the growth of a single…

Soft Condensed Matter · Physics 2021-12-09 Björn König , Olivier J. J. Ronsin , Jens Harting

We propose an exactly solvable self-consistent kinetic model of polymerization-induced phase separation (PIPS) via spinodal decomposition. Using modified Cahn-Hilliard and Glotzer-Coniglio theories for early and late stages of spinodal…

Condensed Matter · Physics 2007-05-23 Valeriy V. Ginzburg , Noel A. Clark

We study the possibility of the spinodal decomposition in the induction period of the polymer crystallization. This phenomenon was first reported in an X-ray scattering experiment, and has still been controversial due to various experiments…

Soft Condensed Matter · Physics 2017-05-02 Hiroshi Yokota , Toshihiro Kawakatsu

By extending the Sanchez-Lacombe lattice-fluid model for mixtures to the case of polymer blends containing solid fillers, we calculate the excess thermodynamic quantities arising from the presence of fillers. These results are then used to…

Soft Condensed Matter · Physics 2026-01-16 A. I. Chervanyov

A MATLAB program has been developed for simulation of polymer blend self-assembly with nano-scaled features. The Cahn-Hilliard equation is implemented to calculate the free energy profile of the polymer blends. The Flory-Huggins type of…

Materials Science · Physics 2010-07-09 Yingrui Shang , David Kazmer

The co-solvency method is a method for the size controlled preparation of nanoparticles like polymersomes, where a poor co-solvent is mixed into a homogeneous copolymer solution to trigger precipitation of the polymer. The size of the…

Soft Condensed Matter · Physics 2018-04-10 Simon Kessler , Friederike Schmid , Klaus Drese

The paper presents a model of lateral phase separation in a two component material surface. The resulting fourth order nonlinear PDE can be seen as a Cahn-Hilliard equation posed on a time-dependent surface. Only elementary tangential…

Numerical Analysis · Mathematics 2020-03-18 Vladimir Yushutin , Annalisa Quaini , Maxim Olshanskii

The Cahn-Hilliard system has been used to describe a wide number of phase separation processes, from co-polymer systems to lipid membranes. In this work the convergence properties of a closest-point based scheme is investigated. In place of…

Numerical Analysis · Mathematics 2017-02-28 Prerna Gera , David Salac

We investigate how the dynamics of a single chain influences the kinetics of early stage phase separation in a symmetric binary polymer mixture. We consider quenches from the disordered phase into the region of spinodal instability. On a…

Statistical Mechanics · Physics 2009-11-07 E. Reister , M. Mueller , K. Binder

A simple expression for the composition dependence of the Flory-Huggins interaction parameter of polymer/solvent systems reported earlier is used to model the demixing of polymer solutions into two liquid phases. To this end the system…

Soft Condensed Matter · Physics 2007-05-23 Sergej Stryuk , Bernhard A. Wolf

Phase transition kinetics of aqueous hydroxypropyl cellulose solution was studied by using turbidimetric monitoring and mathematical modelling techniques. Based on the nonlinear Cahn-Hilliard equation with a mobility depending on the…

Soft Condensed Matter · Physics 2021-12-21 V. I. Kovalchuk

Monte Carlo computer simulations are used to study the conformational free energy of a folded polymer confined to a long cylindrical tube. The polymer is modeled as a hard-sphere chain. Its conformational free energy $F$ is measured as a…

Soft Condensed Matter · Physics 2018-02-07 James M. Polson , Aidan F. Tremblett , Zakary R. N. McLure

We consider the modification of the Cahn-Hilliard equation when a time delay process through a memory function is taken into account. We then study the process of spinodal decomposition in fast phase transitions associated with a conserved…

High Energy Physics - Phenomenology · Physics 2009-11-11 T. Koide , G. Krein , Rudnei O. Ramos

We derive an expression for the free energy of the blends of block copolymers expressed as a functional of the density distribution of the monomer of each block. The expression is a generalization of the Flory-Huggins-de Gennes theory for…

Soft Condensed Matter · Physics 2007-05-23 Takashi Uneyama , Masao Doi

The Flory-Huggins theory is a well-established lattice model that is commonly used to study the mixing of distinct chemical species. It can successfully predict phase separation phenomena in blends of incompatible materials. However, it is…

Materials Science · Physics 2025-12-19 Maxime Siber , Olivier J. J. Ronsin , Jens Harting

The kinetic separation of repulsive active Brownian particles into a dense and a dilute phase is analyzed using a systematic coarse-graining strategy. We derive an effective Cahn-Hilliard equation on large length and time scales, which…

Soft Condensed Matter · Physics 2014-06-02 Thomas Speck , Julian Bialké , Andreas M. Menzel , Hartmut Löwen

If a binary liquid mixture, composed of two alternative species with equal amounts, is quenched from a high temperature to a low temperature, below the critical point of demixing, then the mixture will phase separate through a process known…

Statistical Mechanics · Physics 2022-02-04 Thomas J. Longo , Mikhail A. Anisimov

The filtration membranes are often elaborated through a phase separation process where a polymer rich phase and a polymer poor phase spontaneously form through spinodal decomposition. One process that is still not well understood from a…

We consider a system which consists of a Cahn-Hilliard equation coupled with a Cahn-Hilliard-Oono equation in a bounded domain of $\mathbb{R}^d$, $d = 2, 3$. This system accounts for macrophase and microphase separation in a polymer mixture…

Analysis of PDEs · Mathematics 2022-03-25 Andrea Di Primio , Maurizio Grasselli
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