English
Related papers

Related papers: Low lying excitations of the Dynamical Jahn-Teller…

200 papers

We determine the low-energy spectrum and the eigenstates for a two-bosonic mode nonlinear model by applying the In\"{o}n\"{u}-Wigner contraction method to the Hamiltonian algebra. This model is known to well represent a Bose-Einstein…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 P. Buonsante , R. Franco , V. Penna

We discuss a hopping model of electrons between idealized molecular sites with local orbital degeneracy and dynamical Jahn-Teller effect, for crystal field environments of sufficiently high symmetry. For the Mott-insulating case (one…

Strongly Correlated Electrons · Physics 2009-10-31 Giuseppe Santoro , Leonardo Guidoni , Alberto Parola , Erio Tosatti

A threefold degenerate electronic state is Jahn-Teller unstable with respect to symmetry lowering distortions, which transform as the five quadrupolar modes. The solution of the corresponding vibronic Hamiltonian is constructed using the…

Chemical Physics · Physics 2020-05-14 Arnout Ceulemans

Alkali-doped fullerides exhibit a wealth of unusual phases that remain controversial by nature. Here we report a cryogenic scanning tunneling microscopy study of the sub-molecular structural and electronic properties of expanded fullerene…

Superconductivity · Physics 2020-02-26 Sha Han , Meng-Xue Guan , Can-Li Song , Yi-Lin Wang , Ming-Qiang Ren , Sheng Meng , Xu-Cun Ma , Qi-Kun Xue

We present experiments demonstrating trajectory-dependent electronic excitations at low ion velocities, where ions are expected to primarily interact with delocalized valence electrons. The energy loss of H$^+$, H$_2 ^+$, He$^+$, B$^+$,…

Materials Science · Physics 2020-12-03 Svenja Lohmann , Radek Holeňák , Daniel Primetzhofer

In this paper, motivated by the experimental evidence of rapidly rotating $C_{60}$ molecules in fullerite, we study the low-energy electronic states of rotating fullerene within a continuum model. In this model, the low-energy spectrum is…

Mesoscale and Nanoscale Physics · Physics 2014-05-27 Jonas R. F. Lima , Julio Brandao , Marcio M. Cunha , F. Moraes

The electronic structure of Ce2 is studied in a valence bond model with two 4f electrons localized at two cerium sites. It is shown that the low-lying energy spectrum of the simplest cerium chemical bond is determined by peculiarities of…

Materials Science · Physics 2015-05-28 A. V. Nikolaev

The properties of the polaron and bipolaron are explored in the 1D Jahn-Teller model with dynamical quantum phonons. The ground-state properties of the polaron and bipolaron are computed using a recently developed variational method.…

Strongly Correlated Electrons · Physics 2009-11-07 S. El Shawish , J. Bonca , Li-Chung Ku , S. A. Trugman

Starting from a multipole expansion of intra- molecular Coulomb interactions, we present configuration interaction calculations of the molecular energy terms of the hole configurations hu^m, m=2-5, of C60^{m+} cations, of the electron…

Materials Science · Physics 2015-06-24 A. V. Nikolaev , K. H. Michel

Using a semiclassical continuum model of an electron in a deformable molecular crystal, some properties of multicomponent generalizations of the polaron--``vector polarons''-- are elucidated. Analytical solutions for the case of two…

Materials Science · Physics 2007-06-13 Dennis P. Clougherty

The low-temperature orthorhombic (LTO) phase transition in La$_{2-x}$Sr$_x$CuO$_4$ can be interpreted as a dynamic Jahn-Teller effect, in which the degenerate electronic states are associated with the large densities of states at the two…

Condensed Matter · Physics 2009-10-22 R. S. Markiewicz

The static and dynamic electric multipolar polarizabilities and second hyperpolarizabilities of the H$_2^+$, D$_2^+$, and HD$^+$ molecular ions in the ground and first excited states are calculated nonrelativistically using explicitly…

Atomic Physics · Physics 2014-09-23 Li-Yan Tang , Zong-Chao Yan , Ting-Yun Shi , James F. Babb

We report on THz time-domain spectroscopy on multiferroic GeV4S8, which undergoes orbital ordering at a Jahn-Teller transition at 30.5 K and exhibits antiferromagnetic order below 14.6 K. The THz experiments are complemented by dielectric…

Strongly Correlated Electrons · Physics 2017-10-25 S. Reschke , Zhe Wang , F. Mayr , E. Ruff , P. Lunkenheimer , V. Tsurkan , A. Loidl

We investigate the accuracy of first-principles many-body theories at the nanoscale by comparing the low energy excitations of the carbon fullerenes C_20, C_24, C_50, C_60, C_70, and C_80 with experiment. Properties are calculated via the…

Materials Science · Physics 2009-11-13 Murilo L. Tiago , P. R. C. Kent , Randolph Q. Hood , Fernando A. Reboredo

We study the electronic states of isolated fullerene anions C$^{n-}_{60}$ ($1\le n \le 6$) taking into account the effective interaction between electrons due to exchange of intramolecular phonons. If the vibronic coupling is strong enough…

Condensed Matter · Physics 2010-03-25 L. Bergomi , Th. Jolicoeur

We develop a geometric construction to prove the inevitability of the electronic ground-state (adiabatic) Berry phase for a class of Jahn-Teller models with maximal continuous symmetries and N > 2 intersecting electronic states. Given that…

Quantum Physics · Physics 2018-01-12 Raphael F. Ribeiro , Joel Yuen-Zhou

In this paper, we discuss the dissociative electron attachment process in Methane. Kinetic energy and angular distributions of H^{-} and CH_{2}^{-} fragment anions across the broad resonance about 10 eV is reported. Angular distribution of…

Chemical Physics · Physics 2010-07-30 N. Bhargava Ram , E. Krishnakumar

Understanding the optical properties of color centers in silicon carbide is essential for their use in quantum technologies, such as single-photon emission and spin-based qubits. In this work, first-principles calculations were employed…

Detailed neutron scattering measurements on the bond frustrated magnet ZnCr2S4 reveal a rich H-T phase diagram. The field dependence of the two subsequent antiferromagnetic transitions follows closely that of recently reported structural…

Strongly Correlated Electrons · Physics 2014-06-03 D. Hsieh , Y. W. Li , S. Watauchi , Chang Liu , Q. Huang , R. J. Cava , J. W. Lynn , M. Z. Hasan

Vibrational-excitation cross sections of ground electronic state of carbon dioxide molecule by electron-impact through the CO2-(2\Pi) shape resonance is considered in the separation of the normal modes approximation. Resonance curves and…

Chemical Physics · Physics 2016-11-01 V. Laporta , J. Tennyson , R. Celiberto