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We studied the step dynamics during crystal sublimation and growth in the limit of fast surface diffusion and slow kinetics of atom attachment-detachment at the steps. For this limit we formulate a model free of the quasi-static…

Chemical Physics · Physics 2009-11-13 Bogdan Ranguelov , Stoyan Stoyanov

The kinetics of monoatomic steps in diffusion-controlled crystal growth and evaporation processes are investigated analytically using a Green's function approach. Integro-differential equations of motion for the steps are derived; and a…

Condensed Matter · Physics 2009-10-22 Fong Liu , H. Metiu

The dynamics of steps on crystal surfaces is considered. In general, the meandering of the steps obeys a subdiffusive behaviour. The characteristic asymptotic time laws depend on the microscopic mechanism for detachment and attachment of…

Condensed Matter · Physics 2009-10-31 W. Selke , M. Bisani

Step pattern stability of the vicinal surfaces during growth was analyzed using various surface kinetic models. It was shown that standard analysis of the vicinal surfaces provides no indication on the possible step coalescence and…

The quasistatic approximation is a useful but questionable simplification for analyzing step instabilities during the growth/evaporation of vicinal surfaces. Using this approximation, we characterized in Part I of this work the effect on…

Materials Science · Physics 2021-08-25 L. Guin , M. E. Jabbour , L. Shaabani-Ardali , N. Triantafyllidis

Step meandering instability in a Burton-Cabrera-Frank (BCF)-type model for the growth of an isolated, atomically high step on a crystal surface is analyzed. It is assumed that the growth is sustained by the molecular precursors deposition…

Materials Science · Physics 2015-06-18 Mikhail Khenner

It is shown that step moving to meet solution flow can be unstable against lateral perturbations. The instability of long-wavelength perturbations occurs at values of the solution flow intensity less than some critical value depending on…

Condensed Matter · Physics 2009-10-28 Serge Yu. Potapenko

The steps at the crystal surfaces could be transparent for the migrating adatoms. In the case of significant transparency the velocity of a given step in a given moment is affected by detachment of atoms from rather distant steps in rather…

Other Condensed Matter · Physics 2008-10-15 Bogdan Ranguelov , Stoyan Stoyanov

The decay of a crystalline cone below the roughening transition is studied. We consider local mass transport through surface diffusion, focusing on the two cases of diffusion limited and attachment-detachment limited step kinetics. In both…

Materials Science · Physics 2009-10-31 Navot Israeli , Daniel Kandel

High and low temperature relaxation of crystal steps are described in a unified picture, using a continuum model based on a modified expression of the step free energy. Results are in agreement with experiments and Monte Carlo simulations…

Statistical Mechanics · Physics 2009-11-07 O. Pierre-Louis

The features for the unsteady process of thermal equilibration ("the fast motions") in a one-dimensional harmonic crystal lying in a viscous environment (e.g., a gas) are under investigation. It is assumed that initially the displacements…

Statistical Mechanics · Physics 2021-02-16 Serge N. Gavrilov , Anton M. Krivtsov

We compare two distincts models of evaporative cooling of a magnetically guided atomic beam: a continuous one, consisting in approximating the atomic distribution function by a truncated equilibrium distribution, and a discrete-step one, in…

Other Condensed Matter · Physics 2016-08-16 Thierry Lahaye , David Guéry-Odelin

Step meandering during growth of gallium nitride (0001) surface is studied using kinetic Monte Carlo method. Simulated growth process, conducted in N-rich conditions are therefore controlled by Ga atoms surface diffusion. The model employs…

Statistical Mechanics · Physics 2011-10-24 Magdalena A. Załuska-Kotur , Filip Krzyżewski , Stanisław Krukowski

We discuss the growth process of a crystalline phase out of a metastable over-compressed liquid that is brought into contact with a crystalline substrate. The process is modeled by means of molecular dynamics. The particles interact via the…

Soft Condensed Matter · Physics 2014-08-07 Francesco Turci , Tanja Schilling

Epitaxial growth on a surface vicinal to a high-symmetry crystallographic plane occurs through the propagation of atomic steps, a process called step-flow growth. In some instances, the steps tend to form close groups (or bunches), a…

Materials Science · Physics 2021-08-25 L. Guin , M. E. Jabbour , N. Triantafyllidis

A microscopic model for thermal excitation of vibrational ground state of a molecule interacting with a condensed medium is developed. The master equation for evolution of occupancies of the vibrational levels is derived. The rate constant…

Statistical Mechanics · Physics 2011-03-04 V. I. Teslenko , D. Y. Iatsenko

We expand on a recent study of a lattice model of interacting particles [Phys. Rev. Lett. 111, 110601 (2013)]. The adsorption isotherm and equilibrium fluctuations in particle number are discussed as a function of the interaction. Their…

Statistical Mechanics · Physics 2014-11-20 T. Becker , K. Nelissen , B. Cleuren , B. Partoens , C. Van den Broeck

The kinetics and microstructure of solid-phase crystallization under continuous heating conditions and random distribution of nuclei are analyzed. An Arrhenius temperature dependence is assumed for both nucleation and growth rates. Under…

Materials Science · Physics 2017-04-26 J. Farjas , P. Roura

For low to moderate supersaturations, crystals grow by lateral build-up of new layers. The edges of the layers are known as "steps". We consider the rate of step advance on a flat crystal face under the influence of bulk diffusion in the…

Other Condensed Matter · Physics 2014-04-03 Rasmus Persson

The discerning behavior of living systems relies on accurate interactions selected from the lot of molecular collisions occurring in the cell. To ensure the reliability of interactions, binding partners are classically envisioned as finely…

Molecular Networks · Quantitative Biology 2016-09-28 Denis Michel , Benjamin Boutin , Philippe Ruelle
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