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We investigate a temperature-based model, called extended two-temperature model (eTTM), that describes the electronic non-equilibrium and its effect on energy dissipation in metals after ultrashort laser excitation. We derive and discuss…

Materials Science · Physics 2023-08-03 Markus Uehlein , Sebastian T. Weber , Baerbel Rethfeld

The famous Two-Temperature Model (TTM) used extensively in the investigations of energy relaxation in photo-excited systems originated in the seminal work of M. I. Kaganov, I. M. Lifshitz, and L. V. Tanatarov (KLT) in 1957. The idea that…

Strongly Correlated Electrons · Physics 2024-10-28 Navinder Singh

A model calculation is given for the energy relaxation of a non-equilibrium distribution of hot electrons prepared in a metallic sample that has been subjected to homogeneous photo-excitation by a femtosecond laser pulse. The model assumes…

Statistical Mechanics · Physics 2009-11-11 Navinder Singh

The simulation of non-equilibrium electron distributions is essential for capturing light-metal interactions and therefore the study of photoabsorption, photocatalysis, laser ablation, and many other phenomena. Current methodologies, such…

Materials Science · Physics 2025-03-13 M. Uehlein , H. T. Snowden , C. Seibel , T. Held , S. T. Weber , R. J. Maurer , B. Rethfeld

The non-equilibrium dynamics of electrons is of a great experimental and theoretical value providing important microscopic parameters of the Coulomb and electron-phonon interactions in metals and other cold plasmas. Because of the…

Superconductivity · Physics 2008-11-19 V. V. Kabanov , A. S. Alexandrov

We apply the powerful method of memory function formalism to investigate non-equilibrium electron relaxation in graphene. Within the premises of Two Temperature Model (TTM), explicit expressions of the imaginary part of the Memory Function…

Strongly Correlated Electrons · Physics 2019-09-04 Luxmi Rani , Pankaj Bhalla , Navinder Singh

Ultrafast laser excitation of a metal causes correlated, highly nonequilibrium dynamics of electronic and ionic degrees of freedom, which are however only poorly captured by the widely-used two-temperature model. Here we develop an…

Materials Science · Physics 2017-12-06 Pablo Maldonado , Karel Carva , Martina Flammer , Peter M. Oppeneer

The out-of-equilibrium dynamics of electrons and phonons upon laser excitation are often described by the two-temperature model, which assumes that both subsystems are separately in thermal equilibrium. However, recent experiments show that…

Materials Science · Physics 2021-01-04 Ulrike Ritzmann , Peter M. Oppeneer , Pablo Maldonado

The advent of pump-probe spectroscopy techniques paved the way to the exploration of the ultrafast dynamics of electrons and phonons in crystalline solids. Following photo-absorption of a pump pulse and the initial electronic…

Materials Science · Physics 2023-07-14 Fabio Caruso , Dino Novko

Time- and angle-resolved photoemission spectroscopy (TR-ARPES) accesses the electronic structure of solids under optical excitation, and is a powerful technique for studying the coupling between electrons and collective modes. One approach…

The electrons and phonons in metal films after ultra-short pulse laser heating are in highly non-equilibrium states not only between the electron sub-system and the phonon sub-system but also within the electron sub-system. An…

Materials Science · Physics 2014-08-05 Jun Zhou , Nianbei Li , Ronggui Yang

Ferromagnetic transition in double-exchange systems is studied by non-equilibrium relaxation technique combined with Monte Carlo calculations. Critical temperature and critical exponents are estimated from relaxation of the magnetic moment.…

Strongly Correlated Electrons · Physics 2009-11-07 Yukitoshi Motome , Nobuo Furukawa

We present a theoretical study of the ultrafast electron dynamics in transition metals using ultrashort pulsed laser beams. The significant influence of the contribution of the dynamics of produced nonthermal electrons to electron…

Materials Science · Physics 2016-12-14 George D. Tsibidis

A short overview of theoretical models for the description of the relaxation processes in metals excited by a short laser pulse is presented. The main effort is given to description of different processes which are taking place after…

Strongly Correlated Electrons · Physics 2020-05-20 V. V. Kabanov

Based on the momentum-resolved Boltzmann equation, we provide self-consistent numerical calculations of the dynamics of conduction electrons in thin noble metal films after linear and non-linear optical excitations with infrared and…

Mesoscale and Nanoscale Physics · Physics 2025-04-29 Jonas Grumm , Malte Selig , Holger Lange , Andreas Knorr

The theory and experiments concerned with the electron-ion thermal relaxation and melting of overheated crystal lattice constitute the subject of this paper. The physical model includes two-temperature equation of state, many-body…

This paper describes the effects of electronic nonequilibrium in a simulation of ultrafast laser irradiation of materials. The simulation scheme based on tight-binding molecular dynamics, in which the electronic populations are traced with…

Materials Science · Physics 2023-12-29 Nikita Medvedev

The two-temperature model (2TM) introduced by Kaganov, Lifshitz, and Tanatarov is widely used to describe the energy relaxation in the electron-phonon system of a metallic film. At the same time, the accuracy of the description of the…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 A. I. Bezuglyj , V. A. Shklovskij

Real-time probing of electrons can uncover intricate relaxation mechanisms and many-body interactions hidden in strongly correlated materials. While experimenters have used ultrafast optical pump-probe methods in bulk materials, laser…

Mesoscale and Nanoscale Physics · Physics 2024-01-23 H. M. Yoo , M. Korkusinski , D. Miravet , K. W. Baldwin , K. West , L. Pfeiffer , P. Hawrylak , R. C. Ashoori

We develop ion-ion pair potentials for Al, Na and K for densities and temperatures relevant to the warm-dense-matter (WDM) regime. Furthermore, we emphasize non-equilibrium states where the ion temperature $T_i$ differs from the electron…

Materials Science · Physics 2015-03-19 Louis Harbour , M. W. Chandre Dharma-wardana , Dennis D. Klug , Laurent J. Lewis
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