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To gain insight into the peculiar temperature dependence of the thermoelectric material SnSe, we employ many-body perturbation theory and explore the influence of the electron-phonon interaction on its electronic and transport properties.…

Materials Science · Physics 2019-05-23 Fabio Caruso , Maria Troppenz , Santiago Rigamonti , Claudia Draxl

This article derives an electron-phonon interaction suitable for interpreting ultrasonic attenuation measurements in the ruthenate and cuprate superconductors. The huge anisotropy found experimentally (Lupien et al., 2001) in Sr2RuO4 in the…

Superconductivity · Physics 2009-11-07 M. B. Walker , M. F. Smith , K. V. Samokhin

We report the results of comprehensive study of the critical dynamics of the prototype perovskite antiferroelectric PbZrO$_3$. The combination of inelastic X-ray and diffuse X-ray scattering techniques and Brillouin light scattering was…

Although the rutile structure of TiO$_2$ is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly…

Materials Science · Physics 2015-08-19 Tian Lan , C. W. Li , O. Hellman , D. Kim , J. A. Muñoz , H. Smith , D. L. Abernathy , B. Fultz

We present a first principles investigation of the lattice dynamics and electron-phonon coupling of the high-T_c superconductor YBa_2Cu_3O_7 within the framework of density functional perturbation theory using a mixed-basis pseudopotential…

Superconductivity · Physics 2009-11-07 K. -P. Bohnen , R. Heid , M. Krauss

Copper borate Cu$_3$(BO$_3$)$_2$ is a complex compound with a layered crystallographic structure in which the Jahn-Teller active and magnetic copper Cu$^{2+}$ ions occupy sixteen nonequivalent positions in the unit cell displaying…

We investigate the interplay of electron-phonon (EP) coupling and strong electronic correlations in the frame of the two-dimensional (2D) Holstein t-J model (HtJM), focusing on polaronic ordering phenomena for the quarter-filled band case.…

Strongly Correlated Electrons · Physics 2009-10-28 G. Wellein , H. Fehske , H. Büttner , A. R. Bishop

A strong electron-phonon interaction arises from the modulation of the superexchange interaction by phonons. As is studied in Phys. Rev. B 70, 184514 (2004), Cu-O bond stretching modes can be soft around (pm pi/a, 0) and (0, pm pi/a), with…

Superconductivity · Physics 2015-06-25 Fusayoshi J. Ohkawa

We investigate lattice dynamics in LaCoO$_3$ using inelastic neutron and x-ray scattering over $T = 2\mbox{-}650\,\mathrm{K}$, spanning the spin-state crossover at $T_{1} \approx 100\,\mathrm{K}$ and the insulator--metal transition at…

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

Materials Science · Physics 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch

The temperature and zone dependence of the lattice dynamics in Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ is characterized using neutron inelastic scattering. A strong correlation between the diffuse and phonon scattering is measured. The lattice…

Materials Science · Physics 2009-11-10 C. Stock , H. Luo , D. Viehland , J. F. Li , I. Swainson , R. J. Birgeneau , G. Shirane

Hartree-Fock calculations are presented of a theoretical model describing the Sr/CaRuO$_4$ family of compounds. Both commensurate and incommensurate magnetic states are considered, along with orbital ordering and the effect of lattice…

Strongly Correlated Electrons · Physics 2015-06-24 Satoshi Okamoto , Andrew J. Millis

We have investigated the phonon and the magnetic excitations in LaCoO3 by inelastic neutron scattering measurements. The acoustic phonon dispersions show some characteristic features of the folded Brillouin zone (BZ) for the rhombohedrally…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Kobayashi , Thant Sin Naing , M. Suzuki , M. Akimitsu , K. Asai , K. Yamada , J. Akimitsu , P. Manuel , J. M. Tranquada , G. Shirane

The lattice dynamics of members of the M2Mo6Se6 family of materials with guest ions M = K, Rb, Cs, In, and Tl has been studied using inelastic x-ray scattering and Raman spectroscopy at room temperature, as well as by ab-initio…

Hybrid organic-inorganic semiconductors feature complex lattice dynamics due to the ionic character of the crystal and the softness arising from non-covalent bonds between molecular moieties and the inorganic network. Here we establish that…

The lattice dynamics in CuGeO$_3$ has been analyzed by the combination of inelastic neutron scattering studies and lattice dynamical model calculations. We report an almost complete set of dispersion curves along the three orthorhombic…

Strongly Correlated Electrons · Physics 2025-09-11 M. Braden , W. Reichardt , B. Hennion , G. Dhalenne , A. Revcoleschi

We report a phonon density of states measurement of $\alpha$-ZnCl$_{2}$ using the coherent inelastic neutron scattering technique and a lattice dynamical calculation in four crystalline phases of ZnCl$_{2}$ using a transferable interatomic…

Materials Science · Physics 2007-05-23 A. Sen , Mala N. Rao , R Mittal , S. L. Chaplot

Slow dynamics of energy transfer between different phonon modes under the resonance conditions is considered. It may result in new effects in the inelastic and quasielastic neutron scattering spectra.

Materials Science · Physics 2009-11-10 M. I. Katsnelson , A. V. Trefilov

$\rm Sr_2IrO_4$ is an archetypal spin-orbit-coupled Mott insulator and has been extensively studied in part because of a wide range of predicted novel states. Limited experimental characterization of these states thus far brings to light…

Strongly Correlated Electrons · Physics 2020-09-14 Feng Ye , Christina Hoffmann , Wei Tian , Hengdi Zhao , G. Cao

Inelastic x-ray scattering and $ab$-$initio$ calculation are applied to investigate the lattice dynamics and electron-phonon coupling of the ternary silicide superconductor CaAlSi ($P/bar{6}m2$). A soft c-axis polarized mode is clearly…

Superconductivity · Physics 2009-11-13 S. Kuroiwa , A. Q. R. Baron , T. Muranaka , R. Heid , K. -P. Bohnen , J. Akimitsu
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