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We investigate the statistical mechanics of a torsionally constrained polymer. The polymer is modeled as a fluctuating rod with bend stiffness A kT and twist stiffness C kT. In such a model, thermal bend fluctuations couple geometrically to…

Soft Condensed Matter · Physics 2009-10-30 J. David Moroz , Philip Nelson

We consider the rupture dynamics of a homopolymer chain pulled at one end at a constant loading rate. Our model of the breakable polymer is related to the Rouse chain, with the only difference that the interaction between the monomers is…

Soft Condensed Matter · Physics 2009-10-29 S. Fugmann , I. M. Sokolov

Unconcatenated, unknotted polymer rings in the melt are subject to strong interactions with neighboring chains due to the presence of topological constraints. We study this by computer simulation using the bond-fluctuation algorithm for…

Statistical Mechanics · Physics 2009-10-31 M. Mueller , J. P. Wittmer , M. E. Cates

We present a molecular dynamics study of the effects of confinement on the lubrication and flow properties of ionic liquids. We use a coarse-grained salt model description of ionic liquid as a lubricant confined between finite solid plates…

Soft Condensed Matter · Physics 2018-11-08 Miljan Dašić , Konstantinos Gkagkas , Igor Stanković

The non-linear response of entangled polymers to shear flow is complicated. Its current understanding is framed mainly as a rheological description in terms of the complex viscosity. However, the full picture requires an assessment of the…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas , Philipp Gutfreund , Max Wolff

We show that the injection of polymer chains into nanochannels becomes easier as the channel becomes narrower. This counter intuitive result arises because of a decrease in the diffusive time scale of the chains with increasing confinement.…

Soft Condensed Matter · Physics 2012-07-16 Rodrigo Ledesma-Aguilar , Takahiro Sakaue , Julia M. Yeomans

We use the bond fluctuation model to study the contraction process of two polymer loops with $N$ segments that are connected each to the bottom and top part of a Feringa engine. The change in the size of the molecules as well as the folding…

Chemical Physics · Physics 2022-07-04 Michael Lang , Cornelia Schuster , Ron Dockhorn , Martin Wengenmayr , Jens-Uuwe Sommer

We use the method of dimensional reduction to show that a branching polymer with excluded volume interaction confined between two flat plates has, in the thermodynamic limit, a confinement free energy and density profile that is the same as…

Statistical Mechanics · Physics 2009-11-13 Rouzbeh Ghafouri , Joseph Rudnick , Robijn Bruinsma

We present exact spatio-temporal correlation functions of a Rouse polymer chain submerged in a fluid having planar mixed flow, in the steady state. Using these correlators, determination of the time scale distribution functions associated…

Statistical Mechanics · Physics 2011-09-06 Dipjyoti Das , Sanjib Sabhapandit , Dibyendu Das

We present an analytical and computational study characterizing the structural and dynamical properties of an active filament confined in cylindrical channels. We first outline the effects of the interplay between confinement and polar…

Soft Condensed Matter · Physics 2024-10-09 José Martín-Roca , Emanuele Locatelli , Valentino Bianco , Paolo Malgaretti , Chantal Valeriani

Nanoscale and microscale confinement of biopolymers naturally occurs in cells and has been recently achieved in artificial structures designed for nanotechnological applications. Here, we present an extensive theoretical investigation of…

Soft Condensed Matter · Physics 2007-06-13 Frederik Wagner , Gianluca Lattanzi , Erwin Frey

We study by Monte Carlo simulations and scaling analysis two models of pairs of confined and dense ring polymers in two dimensions. The pair of ring polymers are modelled by squared lattice polygons confined within a square cavity and they…

Soft Condensed Matter · Physics 2022-01-05 EJ Janse van Rensburg , E Orlandini

There has been substantial progress in understanding confinement in a class of four-dimensional SU(N) gauge theories using semiclassical methods. These models have one or more compact directions, and much of the analysis is based on the…

High Energy Physics - Theory · Physics 2014-10-08 Michael C. Ogilvie

The persistence length of macromolecules is one of their basic characteristics, describing their intrinsic local stiffness. However, it is difficult to extract this length from physical properties of the polymers, different recipes may give…

Soft Condensed Matter · Physics 2013-03-12 Hsiao-Ping Hsu , Wolfgang Paul , Kurt Binder

The shape of a polymer plays an important role in determining its interactions with other molecules and with the environment, and is in turn affected by both of them. As a consequence, in the literature the shape properties of a chain in…

Soft Condensed Matter · Physics 2017-07-26 Alberto S. Sassi , Salvatore Assenza , Paolo De Los Rios

We have examined the behaviors of a knotted linear polymer in narrow tubes using Langevin dynamics simulation to investigate the knot localization property in one-dimensional (1D) geometry. We have found that the knot is strongly localized…

Soft Condensed Matter · Physics 2012-06-05 Chihiro H. Nakajima , Takahiro Sakaue

We report the results of Monte Carlo simulations investigating the effect of a spherical confinement within a simple model for a flexible homopolymer. We use the parallel tempering method combined with multi-histogram reweighting analysis…

Soft Condensed Matter · Physics 2012-12-27 M. Marenz , J. Zierenberg , H. Arkin , W. Janke

We introduce an efficient, scalable Monte Carlo algorithm to simulate cross-linked architectures of freely-jointed and discrete worm-like chains. Bond movement is based on the discrete tractrix construction, which effects conformational…

Soft Condensed Matter · Physics 2010-12-27 Henry E. Amuasi , Cornelis Storm

The dynamics of ring polymer melts are studied via molecular dynamics simulations of the Kremer-Grest bead-spring model. Rouse mode analysis is performed in comparison with linear polymers by changing the chain length. Rouse-like behavior…

Soft Condensed Matter · Physics 2021-09-23 Shota Goto , Kang Kim , Nobuyuki Matubayasi

We introduce a class of models of semiflexible polymers. The latter are characterized by a strong rigidity, the correlation length associated to the gradient-gradient correlations, called the persistence length, being of the same order as…

Probability · Mathematics 2011-08-25 Ostap Hryniv , Yvan Velenik