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Catalysis has entered everyday life through a number of technological processes relying on different catalytic systems. The increasing demand for such systems requires rationalization of the use of their expensive components, like noble…

Materials Science · Physics 2019-10-29 A. S. Dobrota , I. A. Pašti , A. Z. Jovanović , B. Johansson , N. V. Skorodumova

Atomic scale nanowires attract enormous interest in a wide range of fields. On the one hand, due to their quasi-one-dimensional nature, they can act as a experimental testbed for exotic physics: Peierls instability, charge density waves,…

Materials Science · Physics 2014-03-13 Danny E. P. Vanpoucke

We report scanning tunneling microscopy observations of Ge deposited on the Si(111)-7x7 surface for a sequence of sub-monolayer coverages. We demonstrate that Ge atoms replace so-called Si adatoms. Initially, the replacements are random,…

Materials Science · Physics 2007-05-23 Y. L. Wang , H. -J. Gao , H. M. Guo , Sanwu Wang , Sokrates T. Pantelides

We report an experimental refinement of the local charge density at the Si (111) 7x7 surface utilizing a combination of x-ray and high energy electron diffraction. By perturbing about a bond-centered pseudoatom model, we find experimentally…

Materials Science · Physics 2015-05-13 J. Ciston , A. Subramanian , I. K. Robinson , L. D. Marks

The segregation behavior of the bimetallic alloys PtPd and CoCr in the case of bare surfaces and in the presence of an oxygen ad-layer has been studied by means of first-principles modeling based on density-functional theory (DFT). For both…

First principles calculations based on density functional theory are having an incerasing impact on our understanding of molecule-surface interactions. For example, calculations of the multi-dimensional potential energy surface have…

Materials Science · Physics 2007-05-23 O. Gulseren , D. M. Bird , S. E. Humphreys

We report the growth process, structure, and electronic states of 1 unit layer (u.l.) of a Ce-Pt intermetallic compound on Pt(111) using scanning tunneling microscopy/spectroscopy (STM/STS) and low-energy electron diffraction. An ordered…

Strongly Correlated Electrons · Physics 2021-10-27 Koichiro Ienaga , Sunghun Kim , Toshio Miyamachi , Fumio Komori

We study theoretically the low-temperature phases of a two-component atomic Fermi gas with attractive s-wave interactions under conditions of rapid rotation. We find that, in the extreme quantum limit, when all particles occupy the lowest…

Mesoscale and Nanoscale Physics · Physics 2007-11-17 Gunnar Moller , Nigel R. Cooper

In this work, we use the first-principle density-functional approach to study the electronic structure of a H atom adsorbed on the ideal Pt(111) and vicinal Pt(211) and Pt(331) surfaces. Full three-dimensional potential-energy surfaces (3D…

Materials Science · Physics 2009-08-04 T. Vehviläinen , P. Salo , T. Ala-Nissila , S. C. Ying

We have performed the numerical modeling of Ge(111)-(2x1) surface electronic properties in vicinity of P donor impurity atom located near the surface. We have found a notable increase of surface $LDOS$ around surface dopant near the bottom…

Mesoscale and Nanoscale Physics · Physics 2013-02-08 S. V. Savinov , A. I. Oreshkin , S. I. Oreshkin

Recently, a novel low-energy collective excitation has been predicted to exist at metal surfaces where a quasi two-dimensional (2D) surface-state band coexists with the underlying three-dimensional (3D) continuum. Here we present a model in…

Materials Science · Physics 2009-11-10 J. M. Pitarke , V. U. Nazarov , V. M. Silkin , E. V. Chulkov , E. Zaremba , P. M. Echenique

Stable oxygen sites on a PdO film over a Pd(100) thin structures with a (sqrt{5} times sqrt{5}) R27^circ surface-unit cell are determined using the first-principles electronic structure calculations with the generalized gradient…

Materials Science · Physics 2015-05-14 K. Kusakabe , K. Harada , Y. Ikuno , H. Nagara

To help provide insight into the remarkable catalytic behavior of the oxygen/silver system for heterogeneous oxidation reactions, purely sub-surface oxygen, and structures involving both on-surface and sub-surface oxygen, as well as…

Materials Science · Physics 2009-11-10 Wei-Xue Li , Catherine Stampfl , Matthias Scheffler

We report a first-principles Wannier function study of the electronic structure of PdTe. Its electronic structure is found to be a broad three-dimensional Fermi surface with highly reduced correlations effects. In addition, the higher…

Superconductivity · Physics 2013-09-13 Chinedu E. Ekuma , Chia-Hui Lin , Juana Moreno , Wei Ku , Mark Jarrell

A nearly-free-electron (NFE) model to describe STM spectroscopy of (111) metal surfaces with Kondo impurities is presented. Surface states are found to play an important role giving a larger contribution to the conductance in the case of…

Strongly Correlated Electrons · Physics 2009-11-10 J. Merino , O. Gunnarsson

We summarize and discuss some of the available experimental and theoretical data important for understanding the role played by subsurface sites in dissociative chemisorption calculations for the H$_2$/Pd(111) system. Then we use a…

chem-ph · Physics 2009-10-28 Ole Martin Løvvik , Roar Aspesæter Olsen

We realized and experimentally tested a conceptually new kind of electrically thin absorbers of electromagnetic waves. The idea is to utilize a single layer of precisely designed meta-atoms. This allows one to design an absorber with…

The modular nature and unique electronic properties of two-dimensional (2D) covalent organic frameworks (COFs) make them an attractive option for applications in catalysis, optoelectronics, and spintronics. The fabrications of such devices…

Materials Science · Physics 2021-04-15 Joseph Frimpong , Zhen-Fei Liu

Perfluoropentacene (PFP), an $n$-type organic semiconductor, is deposited at monolayer and bilayer coverage on Cu(111). Scanning tunneling microscopy at various bias voltages is used to investigate the geometric and electronic structure of…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 S. Smalley , P. Darancet , J. R. Guest , J. A. Smerdon

We study the adsorption geometry of 3,4,9,10-perylene-tetracarboxylic-dianhydride (PTCDA) on Ag(111) and Cu(111) using X-ray standing waves. The element-specific analysis shows that the carbon core of the molecule adsorbs in a planar…

Materials Science · Physics 2011-04-13 A. Gerlach , S. Sellner , F. Schreiber , N. Koch , J. Zegenhagen