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The Zeeman-split spin-states of a single electron confined in a self-assembled quantum dot provide an optically-accessible spin qubit. For III-V materials the nuclear spins of the solid-state host provide an intrinsic noise source,…

Quantum Physics · Physics 2015-12-14 R. Stockill , C. Le Gall , C. Matthiesen , L. Huthmacher , E. Clarke , Maxime Hugues , M. Atature

We present pulsed electron-nuclear double resonance (ENDOR) experiments which enable us to characterize the coupling between bismuth donor spin qubits in Si and the surrounding spin bath of 29Si impurities which provides the dominant…

We evaluate free-induction decay for the transverse components of a localized electron spin coupled to a bath of nuclear spins via the Fermi contact hyperfine interaction. Our perturbative treatment is valid for special (narrowed) bath…

Mesoscale and Nanoscale Physics · Physics 2010-04-21 W. A. Coish , Jan Fischer , Daniel Loss

We report a first-principle theoretical study of the adiabatic decoherence undergone by a nuclear spin system in a solid, coupled to the phonon field through the dipolar interaction. The calculations are performed for a chain of weakly…

Statistical Mechanics · Physics 2016-03-09 F. D. Domínguez , C. E. González , H. H. Segnorile , R. C. Zamar

Despite the importance of isotopically purified samples in current experiments, there have been few corresponding studies of spin qubit decoherence using full quantum bath calculations. Isotopic purification eliminates the well-studied…

Quantum Physics · Physics 2016-01-06 J. E. Lang , R. Guichard , S. J. Balian , T. S. Monteiro

The nuclear spin, being much more isolated from the environment than its electronic counterpart, enables quantum experiments with prolonged coherence times and presents a gateway towards uncovering the intricate dynamics within an atom.…

Mesoscale and Nanoscale Physics · Physics 2023-09-08 Lukas M. Veldman , Evert W. Stolte , Mark P. Canavan , Rik Broekhoven , Philip Willke , Laëtitia Farinacci , Sander Otte

The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

Carbon nanoribbon or nanographene qubit arrays can facilitate quantum-to-quantum transduction between light, charge, and spin, making them an excellent testbed for fundamental science in quantum coherent systems and for the construction of…

Mesoscale and Nanoscale Physics · Physics 2023-08-01 Xiao Chen , James N. Fry , H. P. Cheng

Electron spins are amongst the most coherent solid-state systems known, however, to be used in devices for quantum sensing and information processing applications, they must be typically placed near interfaces. Understanding and mitigating…

We develop a theory for the spin-echo dynamics of a heavy hole in a quantum dot, accounting for both hyperfine- and electric-field-induced fluctuations. We show that a moderate applied magnetic field can drive this system to a…

Mesoscale and Nanoscale Physics · Physics 2012-12-19 Xiaoya Judy Wang , Stefano Chesi , William A. Coish

We introduce an integrability-based method enabling the study of semiconductor quantum dot models incorporating both the full hyperfine interaction as well as a mean-field treatment of dipole-dipole interactions in the nuclear spin bath. By…

Strongly Correlated Electrons · Physics 2014-10-24 Rianne van den Berg , Giuseppe Brandino , Omar El Araby , Robert Konik , Vladimir Gritsev , Jean-Sébastien Caux

We study theoretically spin decoherence and intrinsic spin noise in semiconductor quantum wires caused by an interplay of electron hopping between the localized states and the hyperfine interaction of electron and nuclear spins. At a…

Mesoscale and Nanoscale Physics · Physics 2016-09-13 A. V. Shumilin , E. Ya. Sherman , M. M. Glazov

We examine the logical qubit system of a pair of electron spins in double quantum dots. Each electron experiences a different hyperfine interaction with the local nuclei of the lattice, leading to a relative phase difference, and thus…

Mesoscale and Nanoscale Physics · Physics 2012-12-18 David Drummond , Leonid P. Pryadko , Kirill Shtengel

The time evolution of spin states of two electrons interacting with a nuclear spin bath in a quantum dot system is studied. The hyperfine interaction between the electrons and the nuclear spins is modeled by an isotropic Heisenberg…

Quantum Physics · Physics 2013-07-09 D. D. Bhaktavatsala Rao , V. Ravishankar , V. Subrahmanyam

Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…

Quantum Physics · Physics 2026-05-06 Timothy J. Krogmeier , James Bradley , Anthony W. Schlimgen , Kade Head-Marsden

The decoherence of a localized electron spin in a lattice of nuclear spins is an important problem for potential solid-state implementations of a quantum computer. We demonstrate that even at high fields, virtual electron spin-flip…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Neil Shenvi , Rogerio de Sousa , K. Birgitta Whaley

Bismuth (209Bi) is the deepest Group V donor in silicon and possesses the most extreme characteristics such as a 9/2 nuclear spin and a 1.5 GHz hyperfine coupling. These lead to several potential advantages for a Si:Bi donor electron spin…

In this paper, we study the electron spin decoherence of single defects in silicon carbide (SiC) nuclear spin bath. We find that, although the natural abundance of $^{29}\rm{Si}$ ($p_{\rm{Si}}=4.7\%$) is about 4 times larger than that of…

Mesoscale and Nanoscale Physics · Physics 2015-01-09 Li-Ping Yang , Christian Burk , Mattias Widmann , Sang-Yun Lee , Jörg Wrachtrup , Nan Zhao

Theoretical treatment of the electron spin echo envelope modulation (ESEEM) spectra from polarons in a semiconducting $\pi$- conjugated polymer is presented. The contact hyperfine coupling and the dipolar interaction between the polaron and…

Mesoscale and Nanoscale Physics · Physics 2017-06-14 V. V. Mkhitaryan , V. V. Dobrovitski

The interaction between a central qubit spin and a surrounding bath of spins is critical to spin-based solid state quantum sensing and quantum information processing. Spin-bath interactions are typically strongly anisotropic, and rapid…