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The results of fabrication and characterization of atomic structure of nanocrystalline thin layers of Y2O3 in cubic and monoclinic phases is reported. Experimental data demonstrate crystalline ordering in nanocrystalline films with average…

Materials Science · Physics 2022-12-28 D. W. Boukhvalov , D. A. Zatsepin , Yu. A. Kuznetsova , N. V. Gavrilov , A. F. Zatsepin

We present a general formalism of ultrafast diffractive voltammetry approach as a contact-free tool to investigate the ultrafast surface charge dynamics in nanostructured interfaces. As case studies, the photoinduced surface charging…

Chemical Physics · Physics 2015-06-17 Kiseok Chang , Ryan A. Murdick , Zhensheng Tao , Tzong-Ru T. Han , Chong-Yu Ruan

The diverse functionality emerging at oxide interfaces calls for a fundamental understanding of the mechanisms and control parameters of electronic reconstructions. Here, we explore the evolution of electronic phases in…

Strongly Correlated Electrons · Physics 2015-01-19 David Doennig , Rossitza Pentcheva

The mechanism responsible for the extraordinary interface conductivity of LaAlO$_{3}$ on SrTiO$_{3}$ and its insulator-metal transition remains controversial. Here, using density functional theory calculations, we establish a comprehensive…

Strongly Correlated Electrons · Physics 2015-07-21 Jun Zhou , Teguh Citra Asmara , Ming Yang , George A. Sawatzky , Yuan Ping Feng , Andrivo Rusydi

2D electron gases (2DEGs) formed at oxide interfaces provide a rich testbed for fundamental physics and device applications. While the discussion of the physical origins of this phenomenon continues, the recent discovery of oxide 2DEGs at…

Materials Science · Physics 2018-08-01 Dana Cohen-Azarzar , Maria Baskin , Lior Kornblum

The electronic structure of nanowires in contact with metallic electrodes of experimentally relevant sizes is calculated by incorporating the electrostatic polarization potential into the atomistic single particle Schr\"odinger equation. We…

Materials Science · Physics 2015-05-13 Denis O. Demchenko , Lin-Wang Wang

Novel two-dimensional electron systems at the interfaces and surfaces of transition-metal oxides recently have attracted much attention as they display tunable, intriguing properties that can be exploited in future electronic devices. Here…

The nanoscopic mass and charge distribution within the double layer at electrified interfaces plays a key role in electrochemical phenomena of huge technological relevance for energy production and conversion. However, in spite of its…

Chemical Physics · Physics 2019-05-29 Remi Khatib , Ashwinee Kumar , Stefano Sanvito , Marialore Sulpizi , Clotilde S. Cucinotta

Oxide growth with semiconductor-like accuracy has led to atomically precise thin films and interfaces that exhibit a plethora of phases and functionalities not found in the oxide bulk material. This yielded spectacular discoveries such as…

The electric double layer (EDL) formed around charged nanostructures at the liquid-solid interface determines their electrochemical activity and influences their electrical and optical polarizability. We experimentally demonstrate that…

Soft Condensed Matter · Physics 2020-04-29 Kevin Namink , Xuanhui Meng , Marc T. M. Koper , Philipp Kukura , Sanli Faez

We report on the transport characterization in dark and under light irradiation of three different interfaces: LaAlO3/SrTiO3, LaGaO3/SrTiO3, and the novel NdGaO3/SrTiO3 heterostructure. All of them share a perovskite structure, an…

Three-dimensional interconnected nanowire networks have recently attracted notable attention for the fabrication of new devices for energy harvesting/storage, sensing, catalysis, magnetic and spintronic applications and for the design of…

Electronic, lattice, and spin interactions at the interfaces between crystalline complex transition metal oxides can give rise to a wide range of functional electronic and magnetic phenomena not found in bulk. At hetero-interfaces, these…

Strongly Correlated Electrons · Physics 2017-08-03 S. Koohfar , A. S. Disa , M. Marshall , F. J. Walker , C. H. Ahn , D. P. Kumah

The role of electronic correlation effects for a realistic description of the electronic properties of LaAlO3/SrTiO3 heterostructures as covered by the on-site Coulomb repulsion within the GGA+U approach is investigated. Performing a…

Strongly Correlated Electrons · Physics 2017-01-30 I. I. Piyanzina , T. Kopp , Yu. V. Lysogorskiy , D. A. Tayurskii , V. Eyert

LaAlO3/SrTiO3 ad LaTiO3/SrTiO3 interfaces are known to host a strongly inhomogeneous (nearly) two-dimensional electron gas (2DEG). In this work we present three unconventional electronic mechanisms of electronic phase separation (EPS) in a…

Mesoscale and Nanoscale Physics · Physics 2015-05-08 N. Bovenzi , F. Finocchiaro , N. Scopigno , D. Bucheli , S. Caprara , G. Seibold , M. Grilli

A combined experimental and theoretical study of very-low-energy electron diffraction at the (0001) surface of 2H-NbSe2 is presented. Electron transmission spectra have been measured for energies up to 50 eV above the Fermi level with k||…

Strongly Correlated Electrons · Physics 2009-11-07 E. E. Krasovskii , W. Schattke , V. N. Strocov , R. Claessen

Recent advances in creating complex oxide heterostructures, interfaces formed between two different transition metal oxides, have heralded a new era of materials and physics research, enabling a uniquely diverse set of coexisting physical…

Mesoscale and Nanoscale Physics · Physics 2014-07-07 Joseph A. Sulpizio , Shahal Ilani , Patrick Irvin , Jeremy Levy

The electronic properties of devices based on two-dimensional materials are significantly influenced by interactions with substrate and electrode materials. Here, we use photoemission electron microscopy to investigate the real- and…

In this study we try to answer the qustion : What happens when explicit constraints are introduced such that the low energy, long wavelength modes of a system are unavailable ? This question has assumed some importance in recent years due…

Soft Condensed Matter · Physics 2009-11-11 Abhishek Chaudhuri

An ab initio downfolding method is formulated to construct low-dimensional models for correlated electrons. In addition to the band downfolding by constrained random phase approximation formulated for 3D models, screening away from the…

Strongly Correlated Electrons · Physics 2011-01-11 Kazuma Nakamura , Yoshihide Yoshimoto , Yoshiro Nohara , Masatoshi Imada