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We present a differentiable formalism for learning free energies that is capable of capturing arbitrarily complex model dependencies on coarse-grained coordinates and finite-temperature response to variation of general system parameters.…

Computational Physics · Physics 2024-05-31 Blake R. Duschatko , Xiang Fu , Cameron Owen , Yu Xie , Albert Musaelian , Tommi Jaakkola , Boris Kozinsky

Recent years have seen an increasing integration of distributed renewable energy resources into existing electric power grids. Due to the uncertain nature of renewable energy resources, network operators are faced with new challenges in…

Distributed, Parallel, and Cluster Computing · Computer Science 2020-06-05 Hatem Khalloof , Wilfried Jakob , Shadi Shahoud , Clemens Duepmeier , Veit Hagenmeyer

This paper studies a training method to jointly estimate an energy-based model and a flow-based model, in which the two models are iteratively updated based on a shared adversarial value function. This joint training method has the…

Machine Learning · Statistics 2020-04-02 Ruiqi Gao , Erik Nijkamp , Diederik P. Kingma , Zhen Xu , Andrew M. Dai , Ying Nian Wu

Energy-based models (EBMs) are versatile density estimation models that directly parameterize an unnormalized log density. Although very flexible, EBMs lack a specified normalization constant of the model, making the likelihood of the model…

Machine Learning · Computer Science 2024-02-20 Louis Grenioux , Éric Moulines , Marylou Gabrié

This paper presents a control architecture in which a direct adaptive control technique is used within the model predictive control framework, using the concurrent learning based approach, to compensate for model uncertainties. At each time…

Optimization and Control · Mathematics 2015-02-02 Olugbenga Moses Anubi

We develop a method to fit high-temperature Gibbs free energy data for the development of interatomic potentials for atomic systems. The approach is based on Hamiltonian thermodynamic integration, enabling the identification of suitable…

Materials Science · Physics 2026-03-04 Liangrui Wei , Yang Sun

Alchemical binding free energy (BFE) calculations offer an efficient and thermodynamically rigorous approach to in silico binding affinity predictions. As a result of decades of methodological improvements and recent advances in computer…

Statistical Mechanics · Physics 2021-07-13 Pengfei Li , Zhijie Li , Yu Wang , Huaixia Dou , Brian K. Radak , Woody Sherman , Huafeng Xu

Incorporating computational fluid dynamics in the design process of jets, spacecraft, or gas turbine engines is often challenged by the required computational resources and simulation time, which depend on the chosen physics-based…

Computational Physics · Physics 2019-12-09 Cristina White , Daniela Ushizima , Charbel Farhat

We study the conformational equilibria of two peptides using a novel statistical mechanics approach designed for calculating free energy differences between highly dis-similar conformational states. Our results elucidate the contrasting…

Biological Physics · Physics 2007-05-23 F. Marty Ytreberg , Daniel M. Zuckerman

This paper investigates a new class of modifier-adaptation schemes to overcome plant-model mismatch in real-time optimization of uncertain processes. The main contribution lies in the integration of concepts from the areas of Bayesian…

The high computational demands of multiscale modeling necessitate advanced parallel and adaptive strategies. To address this challenge, we introduce an adaptive method that utilizes two microscale models based on an offline database for…

Distributed, Parallel, and Cluster Computing · Computer Science 2024-07-02 Sion Kim , Ezra Kissel , Karel Matous

With the help of metadynamics it is possible to calculate efficiently the free energy of systems displaying high energy barriers as a function of few selected "collective variables". In doing this, the contribution of all the other degrees…

Statistical Mechanics · Physics 2009-11-13 Guido Tiana

Automatic numerical algorithms attempt to provide approximate solutions that differ from exact solutions by no more than a user-specified error tolerance. The computational cost is often determined \emph{adaptively} by the algorithm based…

Numerical Analysis · Mathematics 2015-01-16 Nicholas Clancy , Yuhan Ding , Caleb Hamilton , Fred J. Hickernell , Yizhi Zhang

Estimating the free energy in molecular simulation requires, implicitly or explicitly, counting how many times the system is observed in a finite region. If the simulation is biased by an external potential, the weight of the configurations…

Chemical Physics · Physics 2021-12-22 Matteo Carli , Alessandro Laio

In this paper we present a hybrid neural network augmented physics-based modeling (APBM) framework for Bayesian nonlinear latent space estimation. The proposed APBM strategy allows for model adaptation when new operation conditions come…

Machine Learning · Computer Science 2022-09-16 Tales Imbiriba , Ahmet Demirkaya , Jindřich Duník , Ondřej Straka , Deniz Erdoğmuş , Pau Closas

An adaptive finite difference scheme for variable-order fractional-time subdiffusion equations in the Caputo form is studied. The fractional time derivative is discretized by the L1 procedure but using nonhomogeneous timesteps. The size of…

Numerical Analysis · Mathematics 2024-09-20 Joaquín Quintana-Murillo , Santos Bravo Yuste

An expression is derived for the classical free energy difference between two configurations of a system, in terms of an ensemble of finite-time measurements of the work performed in parametrically switching from one configuration to the…

Statistical Mechanics · Physics 2009-10-28 C. Jarzynski

This work proposes a methodology to find performance and energy trade-offs for parallel applications running on Heterogeneous Multi-Processing systems with a single instruction-set architecture. These offer flexibility in the form of…

Current model-free adaptive control (MFAC) can hardly deal with the time delay problem in multiple-input multiple-output (MIMO) systems. To solve this problem, a novel model-free adaptive predictive control (MFAPC) method is proposed.…

Systems and Control · Electrical Eng. & Systems 2023-11-21 Feilong Zhang

Hyperparameter selection is critical for stable and efficient convergence of heterogeneous federated learning, where clients differ in computational capabilities, and data distributions are non-IID. Tuning hyperparameters is a manual and…

Machine Learning · Computer Science 2025-10-07 Aayushya Agarwal , Larry Pileggi , Gauri Joshi