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We develop a complete theoretical description of photoassociative Stimulated Raman Adiabatic Passage (STIRAP) near a Feshbach resonance in a thermal atomic gas. We show that it is possible to use low intensity laser pulses to directly…

Quantum Physics · Physics 2015-05-13 Elena Kuznetsova , Susanne F. Yelin , Marko Gacesa , Philippe Pellegrini , Robin Côté

We suggest and analyze a novel technique for efficient and robust creation of dense ultracold molecular ensembles in their ground rovibrational state. In our approach a molecule is brought to the ground state through a series of…

Quantum Physics · Physics 2009-11-13 Elena Kuznetsova , Philippe Pellegrini , Robin Côté , M. D. Lukin , S. F. Yelin

One possibility for the creation of ultracold, high-phase-space-density quantum gases of molecules in the rovibrational ground state relies on first associating weakly-bound molecules from quantum-degenerate atomic gases on a Feshbach…

We study the conversion of $^{40}$K and $^{87}$Rb atoms into stable molecules through the stimulated Raman adiabatic passage (STIRAP) in photoassociation assisted with Feshbach resonance. Starting with the mean-field Langrange density, we…

Soft Condensed Matter · Physics 2007-11-24 Li-Hua Lu , You-Quan Li

A narrow-linewidth, dual-wavelength laser system is vital for the creation of ultracold ground state molecules via stimulated Raman adiabatic passage (STIRAP) from a weakly bound Feshbach state. Here we describe how a relatively simple…

Atomic Physics · Physics 2015-05-21 P. D. Gregory , P. K. Molony , M. P. Köppinger , A. Kumar , Z. Ji , B. Lu , A. L. Marchant , S. L. Cornish

We produce ${^{84}\mathrm{Sr}_2}$ molecules using Bose-enhanced Raman photoassociation. We apply the stimulated Raman adiabatic passage (STIRAP) technique on a Bose-Einstein condensate (BEC) to produce more than $8 \times 10^3$ ultracold…

Quantum Gases · Physics 2017-12-05 Alessio Ciamei , Alex Bayerle , Benjamin Pasquiou , Florian Schreck

We report on the creation of ultracold 84Sr2 molecules in the electronic ground state. The molecules are formed from atom pairs on sites of an optical lattice using stimulated Raman adiabatic passage (STIRAP). We achieve a transfer…

Quantum Gases · Physics 2012-09-18 Simon Stellmer , Benjamin Pasquiou , Rudolf Grimm , Florian Schreck

We associate Sr atom pairs on sites of a Mott insulator optically and coherently into weakly-bound ground-state molecules, achieving an efficiency above 80\%. This efficiency is 2.5 times higher than in our previous work [S. Stellmer, B.…

Quantum Gases · Physics 2017-07-25 Alessio Ciamei , Alex Bayerle , Chun-Chia Chen , Benjamin Pasquiou , Florian Schreck

Collective two-color photoassociation of a freely-interacting 87Rb Bose-Einstein condensate is theoretically examined, focusing on stimulated Raman adiabatic passage (STIRAP) from an atomic to a stable molecular condensate. In particular,…

Atomic Physics · Physics 2016-09-08 Matt Mackie , Anssi Collin , Juha Javanainen

We theoretically examine Raman photoassociation of a Bose-Einstein condensate, revisiting stimulated Raman adiabatic passage (STIRAP). Due to collisional mean-field shifts, efficient molecular conversion requires strong coupling and low…

Atomic Physics · Physics 2007-05-23 Matt Mackie , Kari Harkonen , Anssi Collin , Kalle-Antti Suominen , Juha Javanainen

Many experimental platforms for quantum science depend on state control via laser fields. Frequently, however, the control fidelity is limited by optical phase noise. This is exacerbated in stabilized laser systems where high-frequency…

We report the achievement of stimulated Raman adiabatic passage (STIRAP) in the microwave frequency range between internal states of a Bose-Einstein condensate (BEC) magnetically trapped in the vicinity of an atom chip. The STIRAP protocol…

We present a study of two-photon pathways for the transfer of NaCs molecules to their rovibrational ground state. Starting from NaCs Feshbach molecules, we perform bound-bound excited state spectroscopy in the wavelength range from 900~nm…

The process of stimulated Raman adiabatic passage (STIRAP) provides a possible route for the generation of a coherent molecular Bose-Einstein condensate (BEC) from an atomic BEC. We analyze this process in a three-dimensional mean-field…

Statistical Mechanics · Physics 2009-11-07 P. D. Drummond , K. V. Kheruntsyan , D. J. Heinzen , R. H. Wynar

We report the binding energy of $^{87}$Rb$^{133}$Cs molecules in their rovibrational ground state measured using an offset-free optical frequency comb based on difference frequency generation technology. We create molecules in the absolute…

We identify a route for the production of $^{87}$Rb$^{133}$Cs molecules in the $\textrm{X} \, ^1\Sigma^+$ rovibronic ground state that is compatible with efficient mixing of the atoms in optical lattices. We first construct a model for the…

We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large…

We present a method for the creation and control of cold molecules that involves coherently combining Feshbach Resonances and STIRAP. We present analytical and numerical results showing how to optimize this process that can be implemented…

Atomic Physics · Physics 2019-10-09 Phillip Price , Susanne Yelin

We introduce a method for the coherent acceleration of atoms trapped in an optical lattice, using the well-known model for stimulated Raman adiabatic passage (STIRAP). Specifically, we show that small harmonic modulations of the optical…

Quantum Physics · Physics 2009-11-13 Benjamin P. Holder , Linda E. Reichl

One possible way to produce ultracold, high-phase-space-density quantum gases of molecules in the rovibronic ground state is given by molecule association from quantum-degenerate atomic gases on a Feshbach resonance and subsequent coherent…

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