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Related papers: Quasiparticle self-consistent $GW$ method; a basis…

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Excited-state self-energy effects in the electronic structure of Cu, a prototype weakly correlated system containing states with different degrees of localization, are investigated with emphasis on the unoccupied states up to 40 eV above…

Strongly Correlated Electrons · Physics 2009-11-07 V. N. Strocov , R. Claessen , F. Aryasetiawan , P. Blaha , P. O. Nilsson

We present a method to calculate the electronic charge density of periodic solids in the GW approximation, using the space-time method. We investigate for the examples of silicon and germanium to what extent the GW approximation is…

Condensed Matter · Physics 2009-10-31 Martin M. Rieger , R. W. Godby

To obtain accurate independent-particle descriptions for ferromagnetic two-dimensional van der Waals materials, we apply the quasiparticle self-consistent $GW$ (QSGW) method to VI$_3$, CrI$_3$, CrGeTe$_3$, and Fe$_3$GeTe$_2$. QSGW provides…

Strongly Correlated Electrons · Physics 2020-06-09 Y. Lee , Takao Kotani , Liqin Ke

Modifications to the quasiparticle self-consistent GW (QSGW) method needed to correctly describe metal/vacuum interfaces and other systems having extended regions with small electron density are identified and implemented. The method's…

Materials Science · Physics 2010-03-30 Sergey V. Faleev , Oleg N. Mryasov , Thomas R. Mattsson

We introduce a systematic hierarchy of one-body Green's function methods derived from the $GW$ approximation, constructed by progressively reducing the dynamical content of the self-energy. Starting from the fully dynamical Dyson…

Chemical Physics · Physics 2026-04-10 Pierre-François Loos , Johannes Tölle

We present improved band structure calculations of the Mg-IV-N$_2$ compounds in the quasiparticle self-consistent $GW$ approximation. Compared to previous calculations (Phys. Rev. B 94, 125201 (2016)) we here include the effects of the…

Materials Science · Physics 2019-07-24 Sai Lyu , Walter R. L. Lambrecht

In principle, the Luttinger-Ward Green's function formalism allows one to compute simultaneously the total energy and the quasiparticle band structure of a many-body electronic system from first principles. We present approximate and exact…

Materials Science · Physics 2015-05-18 Sohrab Ismail-Beigi

We describe the following new features which significantly enhance the power of the recently developed real-space imaginary-time GW scheme (Rieger et al., Comp. Phys. Commun. 117, 211 (1999)) for the calculation of self-energies and related…

Condensed Matter · Physics 2009-10-31 L. Steinbeck , A. Rubio , L. Reining , M. Torrent , I. D. White , R. W. Godby

The electronic structure of surfaces and interfaces plays a key role in the properties of quantum devices. Here, we study the electronic structure of realistic Al/InAs/Al heterojunctions using a combination of density functional theory…

Mesoscale and Nanoscale Physics · Physics 2024-11-06 H. Ness , F. Corsetti , D. Pashov , B. Verstichel , G. W. Winkler , M. van Schilfgaarde , R. M. Lutchyn

We show how to construct an effective Hamiltonian whose dimension scales linearly with system size, and whose eigenvalues systematically approximate the excitation energies of GW theory. This is achieved by rigorously expanding the…

Chemical Physics · Physics 2023-07-18 Charles J. C. Scott , Oliver J. Backhouse , George H. Booth

The quasiparticle wavefunction of a many-electron system is traditionally defined as the eigenfunction of the quasiparticle eigenvalue equation involving the self-energy. In this article a new concept of a quasiparticle wavefunction is…

Strongly Correlated Electrons · Physics 2024-12-05 F. Aryasetiawan , K. Karlsson

The performance of many-body perturbation theory for calculating ground-state properties is investigated. We present fully numerical results for the electron gas in three and two dimensions in the framework of the GW approximation. The…

Condensed Matter · Physics 2009-10-31 P. Garcia-Gonzalez , R. W. Godby

The electronic band structures of BeSiN$_2$ and BeGeN$_2$ compounds are calculated using the quasiparticle self-consistent $GW$ method. The lattice parameters are calculated for the wurtzite based crystal structure commonly found in other…

Materials Science · Physics 2019-09-04 Sai Lyu , Walter R. L. Lambrecht

This paper describes an all-electron implementation of the self-consistent GW (sc-GW) approach -- i.e. based on the solution of the Dyson equation -- in an all-electron numeric atom-centered orbital (NAO) basis set. We cast Hedin's…

Materials Science · Physics 2013-08-12 Fabio Caruso , Patrick Rinke , Xinguo Ren , Angel Rubio , Matthias Scheffler

The calculation of quasi-particle spectra based on the GW approximation is extended to systems of hundreds of atoms, thus expanding the size range of current approaches by more than one order of magnitude. This is achieved through an…

Materials Science · Physics 2008-11-11 P. Umari , Geoffrey Stenuit , Stefano Baroni

We discuss the implementation of quasiparticle calculations for point defects on semiconductor surfaces and, as a specific example, present an ab initio study of the electronic structure of the As vacancy in the +1 charge state on the…

Materials Science · Physics 2007-05-23 Magnus Hedstrom , Arno Schindlmayr , Matthias Scheffler

Over the years, Hedin's $GW$ self-energy has been proven to be a rather accurate and simple approximation to evaluate electronic quasiparticle energies in solids and in molecules. Attempts to improve over the simple $GW$ approximation, the…

Computational Physics · Physics 2024-01-24 Fabien Bruneval , Arno Förster

The family of Green's function methods based on the $GW$ approximation has gained popularity in the electronic structure theory thanks to its accuracy in weakly correlated systems combined with its cost-effectiveness. Despite this,…

Chemical Physics · Physics 2023-08-31 Antoine Marie , Pierre-François Loos

Calculations of ground-state and excited-state properties of materials have been one of the major goals of condensed matter physics. Ground-state properties of solids have been extensively investigated for several decades within the…

Strongly Correlated Electrons · Physics 2009-10-30 F. Aryasetiawan , O. Gunnarsson

A GW approximation (GWA) method named U+GWA is proposed, where we can start GWA with more localized wave functions obtained by the local spin-density approximation (LSDA)+U method. Then GWA and U+GWA are applied to MnO, NiO, and V$_2$O$_3$…

Strongly Correlated Electrons · Physics 2008-10-18 S. Kobayashi , Y. Nohara , S. Yamamoto , T. Fujiwara
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