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In the quest to increase battery performance, nanostructuring battery electrodes gives access to architectures with electrical conductivity and solid-state diffusion regimes not accessible with traditional electrodes based on aggregated…

We carry out first-principles calculations to demonstrate that the complex energy landscape and competing phases of HfO$_2$ can be understood from the four unstable flat phonon bands of an unconventional high-symmetry structure of HfO$_2$…

Materials Science · Physics 2025-07-09 Yubo Qi , Karin M. Rabe

We have studied potassium-intercalated bulk HfS$_2$ and HfSe$_2$ by combining transmission electron energy loss spectroscopy, angle-resolved photoemission spectroscopy and density functional theory calculations. Calculations of the…

Mesoscale and Nanoscale Physics · Physics 2020-07-01 Carsten Habenicht , Jochen Simon , Manuel Richter , Roman Schuster , Martin Knupfer , Bernd Büchner

The structural, elastic and electronic properties of two-dimensional (2D) titanium carbide/nitride based pristine (Tin+1Cn/Tin+1Nn) and functionalized MXenes (Tin+1CnT2/Tin+1NnT2, T stands for the terminal groups: -F, -O and -OH, n = 1, 2,…

Materials Science · Physics 2018-07-06 Ning Zhang , Yu Hong , Sanaz Yazdanparast , Mohsen Asle Zaeem

The single crystal elastic constants, polycrystalline elastic moduli and related properties of orthorhombic MgSiN$_{2}$, MgGeN$_{2}$ and MgSnN$_{2}$ have been calculated using density functional theory and compared to the related wurtzite…

Materials Science · Physics 2018-08-29 Mikael Råsander , Michelle A. Moram

Hafnium carbides are studied by a systematic search for possible stable stoichiometric compounds in the Hf-C system at ambient pressure using variable-composition ab initio evolutionary algorithm implemented in the USPEX code. In addition…

We investigate the structural, electronic, and magnetic properties of the hypothetical compound BaFePn2 (Pn = As and Sb), which is isostructural to the parent compound of the high temperature superconductor LaFeAsO1-xFx. Using density…

Superconductivity · Physics 2013-05-29 J. H. Shim , K. Haule , G. Kotliar

We study the stability and electronic structure of previously unexplored two-dimensional (2D) ternary compounds BNP$_2$ and C$_2$SiS. Using $ab$ $initio$ density functional theory, we have identified four stable allotropes of each ternary…

Materials Science · Physics 2020-11-11 Shixin Song , Jie Guan , David Tománek

First principles density functional calculations within the local spin density approximation (LSDA) and the generalized gradient approximation (GGA) are reported for pyrochlore Cd$_2$Os$_2$O$_7$ and Cd$_{2}$Re$_{2}$O$_7$. The transition…

Condensed Matter · Physics 2009-11-07 D. J. Singh , P. Blaha , K. Schwarz , J. O. Sofo

The electrical conductivity and Raman spectroscopy measurements have been performed on MoS$_2$ at high pressures up to 90 GPa and variable temperatures down to 5 K. We find that the temperature dependence of the resistance in a metallic…

Materials Science · Physics 2018-06-27 Zi-Yu Cao , Jia-Wei Hu , Alexander F. Goncharov , Xiao-Jia Chen

High electronic transport and reasonable chemical stability of molybdenum disulfide (MoS$_2$) make it very suitable for electrochemical applications. However, its energy storage capacity is still low compared with other nanostructures. In…

Applied Physics · Physics 2022-08-19 Marzieh Rashidi , Foad Ghasemi

Motivated by the recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ under high pressure, we explore its potential charge and spin instabilities through combined model analysis and first-principles calculations. Taking into account…

Superconductivity · Physics 2025-01-24 Xuejiao Chen , Peiheng Jiang , Jie Li , Zhicheng Zhong , Yi Lu

The elemental two-dimensional (2D) materials such as graphene, silicene, germanene, and black phosphorus have attracted considerable attention due to their fascinating physical properties. Structurally they possess the honeycomb or…

Materials Science · Physics 2016-05-18 Ping Li , Weidong Luo

We present a theoretical study of the structure-property correlation in gallium ferrite, based on the first principles calculations followed by a subsequent comparison with the experiments. Local spin density approximation (LSDA+U) of the…

Materials Science · Physics 2011-07-27 Amritendu Roy , Somdutta Mukherjee , Rajeev Gupta , Rajendra Prasad , Sushil Auluck , Ashish Garg

Boron nitride (BN) is a material with outstanding technological promise because of its exceptional thermochemical stability, structural, electronic and thermal conductivity properties, and extreme hardness. Yet, the relative thermodynamic…

Materials Science · Physics 2018-12-13 Claudio Cazorla , Tim Gould

The structural behavior of UO2 under high pressure up to 300GPa has been studied by first-principles calculations with LSDA+U approximation. The results show that a pressure-induced structural transition to the cotunnite-type (orthorhombic…

Materials Science · Physics 2007-05-23 H. Y. Geng , Y. Chen , Y. Kaneta , M. Kinoshita

The lack of a bulk second-order nonlinearity (\c{hi}(2)) in silicon nitride (Si3N4) keeps this low-loss, CMOS-compatible platform from key active functions such as Pockels electro-optic (EO) modulation and efficient second harmonic…

The square-planar layered nickelates R$_{n+1}$Ni$_n$O$_{2n+2}$ (R= Nd, $n=4-7$) have been recently shown to be superconducting without the need for chemical doping or pressure. Here, we examine the electronic structure of the analog…

Strongly Correlated Electrons · Physics 2026-03-31 Alexander K. Gavrilov , Lidia C. Santander , Antia S. Botana

The existence of a new two dimensional CN2 structure was predicted using ab-initio molecular dynamics (AIMD) and density-functional theory calculations. It consists tetragonal and hexagonal rings with C-N and N-N bonds arranged in a…

Materials Science · Physics 2021-01-29 Qun Wei , Ying Yang , Alexander Gavrilov , Xihong Peng

The polymeric phase of nitrogen connected by the lower (than three) order N-N bonds has been long sought after for the potential application as high energy density materials. Here we report a hitherto unknown polymeric N$_2$H phase…

Materials Science · Physics 2015-03-16 Ketao Yin , Yanchao Wang , Hanyu Liu , Feng Peng , Lijun Zhang