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We present a detailed first-principles DFT study of the equation of state (EOS), energy-optimized geometries, phase stabilities and electronic properties of bulk crystalline Cu3N, CuN and CuN2 in a set of twenty different structural phases.…

Materials Science · Physics 2018-05-18 Mohammed S. H. Suleiman , Mahlaga P. Molepo , Daniel P. Joubert

We report an optical spectroscopy study on the single crystal of Na$_2$Ti$_2$As$_2$O, a sister compound of superconductor BaTi$_2$Sb$_2$O. The study reveals unexpectedly two density wave phase transitions. The first transition at 320 K…

Strongly Correlated Electrons · Physics 2015-06-18 Y. Huang , H. P. Wang , R. Y. Chen , X. Zhang , P. Zheng , Y. G. Shi , N. L. Wang

In this work we explore the phase diagram of the binary Nb-S system from ambient pressures up to 250 GPa using $ab$ $initio$ evolutionary crystal structure prediction. We find several new stable compositions and phases, especially in the…

Materials Science · Physics 2021-01-13 Roman Lucrezi , Christoph Heil

The development of advanced materials with high specific energy is crucial for enabling sustainable energy storage solutions, particularly in applications such as lithium-air batteries. Lithium peroxide (Li$_{2}$O$_{2}$) is a key discharge…

Nitriding introduces nitrides into the surface of steels, significantly enhancing the surface me-chanical properties. By combining the variable composition evolutionary algorithm and first-principles calculations based on density functional…

Materials Science · Physics 2024-11-27 Ergen Bao , Jinbin Zhao , Qiang Gao , Ijaz Shahid , Hui Ma , Yixiu Luo , Peitao Liu , Yan Sun , Xing-Qiu Chen

We present a detailed quantum oscillatory study on the Dirac type-II semimetallic candidates PdTe$_{2}$ and PtTe$_{2}$ \emph{via} the temperature and the angular dependence of the de Haas-van Alphen (dHvA) and Shubnikov-de Haas (SdH)…

The electronic band structures along with Fermi surface, anisotropy, Vickers hardness, analysis of Mulliken populations, optical and thermodynamic properties were studied for the first time. The optimized unit cell parameters are compared…

Materials Science · Physics 2018-08-22 P. Barua , M. M. Hossain , M. A. Ali , M. M. Uddin , S. H. Naqib , A. K. M. A. Islam

We present an ab initio full-potential linearized augmented plane-wave (FLAPW) study of the structural and electronic properties of the two bulk unstable compounds FeSi (CsCl structure) and FeSi$_2$ (CaF$_2$ structure) which have recently…

Condensed Matter · Physics 2007-05-23 K. A. Mader , H. von Kanel , A. Baldereschi

Noting the structural relationships between phases of carbon and boron carbide with phases of boron nitride and boron subnitride, we investigate their mutual solubilities using a combination of first principles total energies supplemented…

Materials Science · Physics 2016-04-13 Hantao Zhang , Sanxi Yao , Michael Widom

Two-dimensional materials have attracted tremendous attention for their fascinating electronic, optical, chemical and mechanical properties. However, the band gaps of most 2D materials reported are smaller than 2.0 eV, which greatly…

Materials Science · Physics 2018-02-14 Hang Xiao , Xiaoyang Shi , Feng Hao , Xiangbiao Liao , Yayun Zhang , Xi Chen

Plutonium dioxide is of high technological importance in nuclear fuel cycle and is particularly crucial in long-term storage of Pu-based radioactive waste. Using first-principles density-functional theory, in this paper we systematically…

Materials Science · Physics 2011-09-29 Ping Zhang , Bao-Tian Wang , Xian-Geng Zhao

We have investigated the pressure-induced phase transition and superconducting properties of niobium disulfide (NbS$_2$) based on the density functional theory. The structures of NbS$_2$ at pressures from 0 to 200 GPa were predicted using…

Superconductivity · Physics 2014-10-31 Zhong-Li Liu , Ling-Cang Cai , Xiu-Lu Zhang

The physical mechanisms behind the reduction of the bulk modulus of a high-pressure cubic TiO2 phase are confirmed by first-principles calculations. An unusual and abrupt change occurs in the dependence of energy on pressure at 43 GPa,…

Materials Science · Physics 2010-08-16 Xiang-Feng Zhou , Xiao Dong , Guang-Rui Qian , Lixin Zhang , Yonjun Tian , Hui-Tian Wang

In the present work we have proposed the method that allows one to easily estimate hardness and bulk modulus of known or hypothetical solid phases from the data on Gibbs energy of atomization of the elements and corresponding covalent…

Materials Science · Physics 2011-02-08 Vladimir A. Mukhanov , Oleksandr O. Kurakevych , Vladimir L. Solozhenko

The electronic and energy properties of beta-Si3N4 (a), Si{6-x}AlxOxN{8-x} (b) and the hypothetical ordered solid solutions Si{6-x}MgxO{2x}N{8-2x} (c), Si{6-x}MgxOxN{8-2x}Sx (d), Si{6-x}MgxOxN{8-x} (e), Si{6-x}Mg{x/2}Al{x/2}OxN{8-x} (f) are…

Materials Science · Physics 2007-05-23 S. V. Okatov

Polynitrogen compounds have attracted great interest due to their potential applications as high energy density materials. Most recently, a rich variety of alkali polynitrogens (R_{x}N_{y}; R=Li, Na, and Cs) have been predicted to be stable…

Materials Science · Physics 2018-02-07 Brad A. Steele , Ivan I. Oleynik

Density-functional-theory-based electronic structure calculations are made to consider the novel electronic states of Ru-pnictides RuP and RuAs where the intriguing phase transitions and superconductivity under doping of Rh have been…

Strongly Correlated Electrons · Physics 2016-01-25 H. Goto , T. Toriyama , T. Konishi , Y. Ohta

NiS2, a compound characterized by its pyrite structure, uniquely bridges the realms of strong correlation physics and topology. While bulk NiS2 is known to be a Mott or charge-transfer insulator, its surface displays anomalous metallic…

We investigate energetically favorable structures of ABO$_2$N oxynitrides as functions of pressure and strain via swarm-intelligence-based structure prediction methods, DFT lattice dynamics and first-principles molecular dynamics. We…

Materials Science · Physics 2021-06-11 Li Zhu , Hiroyuki Takenaka , R. E. Cohen

We have synthesized four iron-based oxyarsenide superconductors Rb$Ln_2$Fe$_4$As$_4$O$_2$ ($Ln$ = Sm, Tb, Dy and Ho) resulting from the intergrowth of RbFe$_2$As$_2$ and $Ln$FeAsO. It is found that the lattice match between RbFe$_2$As$_2$…

Superconductivity · Physics 2017-04-05 Zhi-Cheng Wang , Chao-Yang He , Si-Qi Wu , Zhang-Tu Tang , Yi Liu , Guang-Han Cao