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Colloidal particles or nanoparticles, with equal affinity for two fluids, are known to adsorb irreversibly to the fluid-fluid interface. We present large-scale computer simulations of the demixing of a binary solvent containing such…

Soft Condensed Matter · Physics 2007-05-23 K. Stratford , R. Adhikari , I. Pagonabarraga , J. -C. Desplat , M. E. Cates

We study the adsorption of charged patchy particle models (CPPMs) on a thin film of a like-charged and dense polyelectrolyte (PE) brush (of 50 monomers per chain) by means of implicit-solvent, explicit-salt Langevin dynamics computer…

Soft Condensed Matter · Physics 2017-01-11 Cemil Yigit , Matej Kanduc , Matthias Ballauff , Joachim Dzubiella

We study the coupling between the structural dynamics and rheological response of charged colloidal monolayers at water/oil interfaces, driven into steady shear by a microdisk rotating at a controlled angular velocity. The flow causes…

Soft Condensed Matter · Physics 2015-09-14 Ivo Buttinoni , Zachary A. Zell , Todd M. Squires , Lucio Isa

Due to the complex interplay between surface adsorption and hydrodynamic interactions, representative microscopic mechanisms of colloidal membrane fouling are still not well understood. Numerical simulations overcome experimental…

Computational Physics · Physics 2018-03-22 Johannes Lohaus , Yannic Martin Perez , Matthias Wessling

We investigate the behavior of colloidal suspensions with different volume fractions confined between parallel walls under a range of steady shears. We model the particles using molecular dynamics (MD) with full hydrodynamic interactions…

Soft Condensed Matter · Physics 2014-09-18 Frances E. Mackay , Kyle Pastor , Mikko Karttunen , Colin Denniston

We experimentally and theoretically investigate the collective behavior of three colloidal particles that are driven by a constant force along a toroidal trap. Due to hydrodynamic interactions, a characteristic limit cycle is observed. When…

Soft Condensed Matter · Physics 2016-08-31 Christoph Lutz , Michael Reichert , Holger Stark , Clemens Bechinger

Recently a novel class of responsive uncharged polymer brushes has been proposed [Klushin et al, J. Chem. Phys. 154, 074904 (2021)] where the brush-forming chains have an affinity to the substrate. For sufficiently strong surface…

We consider a system of colloidal particles embedded in a paranematic -- an isotropic phase of a nematogenic medium above the temperature of the nematic-to-isotropic transition. In this state, the nematic order is induced by the boundary…

Analysis of PDEs · Mathematics 2025-08-08 Dmitry Golovaty , Jamie Taylor , Raghavendra Venkatraman , Arghir Zarnescu

Previous experiments have shown that spherical colloidal particles relax to equilibrium slowly after they adsorb to a liquid-liquid interface, despite the large interfacial energy gradient driving the adsorption. The slow relaxation has…

Soft Condensed Matter · Physics 2016-11-08 Anna Wang , Ryan McGorty , David M. Kaz , Vinothan N. Manoharan

Polyelectrolyte (PE) brushes are widely used in biomaterials and nanotechnology to regulate surface properties and interactions. Here, we apply the electrostatic correlation augmented self-consistent field theory to investigate the…

Soft Condensed Matter · Physics 2024-08-16 Chao Duan , Rui Wang

We study the motion of charged particles constrained to arbitrary two-dimensional curved surfaces but interacting in three-dimensional space via the Coulomb potential. To speed-up the interaction calculations, we use the parallel compute…

Classical Physics · Physics 2012-12-07 Thomas Müller , Jörg Frauendiener

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer

We simulated irreversible aggregation of non-interacting particles and of particles interacting via repulsive and attractive potentials explicitly implementing the rotational diffusion of aggregating clusters. Our study confirms that the…

Soft Condensed Matter · Physics 2019-03-26 Swetlana Jungblut , Jan-Ole Joswig , Alexander Eychmüller

We use computer simulations to study highly dense systems of granular particles that are driven by oscillating forces. We implement different dissipation mechanisms that are used to extract the injected energy. In particular, the action of…

Soft Condensed Matter · Physics 2016-10-27 Ronny Moebius , Claus Heussinger

In sandstorms and thunderclouds, turbulence-induced collisions between solid particles and ice crystals lead to inevitable triboelectrification. The charge segregation is usually size-dependent, with small particles charged negatively and…

Fluid Dynamics · Physics 2023-12-11 Xuan Ruan , Matthew T. Gorman , Rui Ni

Designable media can control properties of nanocomposite materials by spatially organizing nanoparticles. Here we theoretically study particle organization by ultrathin polymer films of grafted chains (``brushes''). Polymer-soluble…

Soft Condensed Matter · Physics 2009-11-07 Jaeup U. Kim , Ben O'Shaughnessy

We investigate a set of design principles that link specific features of interparticle interactions to predictable structural and dynamic outcomes in two-dimensional self-assembly, a framework relevant to soft matter and biological…

Soft Condensed Matter · Physics 2026-01-06 Cecilia Bores , Antonio Diaz-Pozuelo , Enrique Lomba

The aim of this paper is to discuss the mathematical modeling of Brownian active particle systems, a recently popular paradigmatic system for self-propelled particles. We present four microscopic models with different types of repulsive…

Statistical Mechanics · Physics 2022-05-31 M. Bruna , M. Burger , A. Esposito , S. M. Schulz

If particles interact according to isotropic pair potentials that favor multiple length scales, in principle a large variety of different complex structures can be achieved by self-assembly. We present, motivate, and discuss a conjecture…

Soft Condensed Matter · Physics 2018-11-07 Erdal C. Oğuz , Aleksandar Mijailović , Michael Schmiedeberg

We consider the effect of atomic hydrogen exposure to a system of two undoped sheets of graphene grown near a silica surface (the first adsorbed to the surface and the second freestanding near the surface). In the absence of atomic hydrogen…

Materials Science · Physics 2012-01-26 Mathias Boström , Bo E. Sernelius