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The localized-itinerant nature of Ce-4$f$ valence electrons in heavy fermion compound CeIn$_{3}$ under pressure is studied thoroughly by means of the combination of density functional theory and single-site dynamical mean-field theory. The…

Strongly Correlated Electrons · Physics 2016-08-17 Haiyan Lu , Li Huang

We present a simple, but very realistic, model for a description of pressure induced valence and metal-insulator transitions in mixed valence systems. It is based on the extended Falicov-Kimball model and the supposition that the key…

Strongly Correlated Electrons · Physics 2018-11-14 Pavol Farkasovsky

Pressure induced isostructural insulator to metal transition for SmS is characterised by the presence of an intermediate valence state at higher pressure which cannot be captured by the density functional theory. As a direct outcome of…

Strongly Correlated Electrons · Physics 2022-06-01 Debalina Banerjee , Evgeny Plekhanov , Ivan Rungger , Cedric Weber

A typical f-electron Kondo lattice system Ce exhibits the well-known isostructural transition, the so-called gamma-alpha transition, accompanied by an enormous volume collapse. Most interestingly, we have discovered that a topological-phase…

Strongly Correlated Electrons · Physics 2019-12-04 Junwon Kim , Dongchoon Ryu , Chang-Jong Kang , Kyoo Kim , Hongchul Choi , T. -S. Nam , B. I. Min

Valence instability is a key ingredient of the unusual properties of f electron materials, yet a clear understanding is lacking as it involves a complex interplay between f electrons and conduc- tion states. Here we propose a unified…

Transport properties of Ce$_{0.85}$F0.15SbS$_{2}$ and undoped CeOSbS$_{2}$ under high pressure were investigated experimentally and theoretically. Electrical resistivity measurements of the Ce$_{0.85}$F0.15SbS$_{2}$ single crystals were…

A combination of the density functional theory and the single-site dynamical mean-field theory is employed to study the pressure dependence of electronic structure for cubic phase californium. We predict that its 5$f$ electrons could…

Strongly Correlated Electrons · Physics 2019-01-09 Li Huang , Haiyan Lu

X-ray powder diffraction and electrical resistivity measurements were performed on the tetragonal compound CeCoSi under pressure to elucidate the phase boundary of the pressure-induced structural transition and the change in the 4$f$…

Electrical resistivity measurements on La$_{1-x}$Sm$_{x}$O$_{0.5}$F$_{0.5}$BiS$_{2}$ ($x$ = 0.1, 0.3, 0.6, 0.8) have been performed under applied pressures up to 2.6 GPa from 2 K to room temperature. The superconducting transition…

Superconductivity · Physics 2015-10-28 Y. Fang , D. Yazici , B. D. White , M. B. Maple

The pressure induced bcc to hcp transition in Fe has been investigated via ab-initio electronic structure calculations. It is found by the disordered local moment (DLM) calculations that the temperature induced spin fluctuations result in…

Materials Science · Physics 2013-12-04 S. Mankovsky , S. Polesya , H. Ebert , W. Bensch , O. Mathon , S. Pascarelli , J. Minar

The electronic property and magnetic susceptibility of Ce$_3$Pd$_3$Bi$_4$ were systemically investigated from 18 K to 290 K for varying values of cell-volume using dynamic mean-field theory coupled with density functional theory. By…

Strongly Correlated Electrons · Physics 2022-02-08 Chenchao Xu , Chao Cao , Jian-Xin Zhu

Pressure-induced polarization switching in ferroelectric thin films has emerged as a powerful method for domain patterning, allowing to create predefined domain patterns on free surfaces and under thin conductive top electrodes. However,…

Materials Science · Physics 2017-12-06 Ye Cao , Anna Morozovska , Sergei V. Kalinin

Properties of an extended periodic Anderson model with the f-c Coulomb interaction $\Ufc$ is studied as a model for \Ge and related compounds which is cosidered to exhibit a sharp valence change under pressure. The problem is treated by…

Strongly Correlated Electrons · Physics 2009-10-31 Y. Onishi , K. Miyake

We present results of hard X-ray angle-resolved photoemission spectroscopy and photoemission diffraction measurements performed on high-quality single crystals of the valence transition compound EuPd$_2$Si$_2$ for temperatures 25~K $\leq$ T…

CeCu$_2$Si$_2$ is an exemplary correlated electron metal that features two domes of unconventional superconductivity in its temperature-pressure phase diagram. The first dome surrounds an antiferromagnetic quantum critical point, whereas…

Strongly Correlated Electrons · Physics 2017-08-23 Y. Lai , S. M. Saunders , D. Graf , A. Gallagher , K. -W. Chen , F. Kametani , T. Besara , T. Siegrist , A. Shekhter , R. E. Baumbach

The pressure-induced structural phase transition in the intermediate-valence compound CeNi has been investigated by X-ray and neutron powder diffraction techniques. For the first time it is shown that the structure of the pressure-induced…

Strongly Correlated Electrons · Physics 2016-06-17 A. Mirmelstein , A. Podlesnyak , Antnio M. dos Santos , G. Ehlers , O. Kerbel , V. Matvienko , A. S. Sefat , B. Saparov , G. J. Halder , J. G. Tobin

We report on the most complete investigation to date of the 4f-electron properties at the gamma-alpha transition in elemental Ce by resonant inelastic x-ray scattering (RIXS). The Ce 2p3d-RIXS spectra were measured directly in the bulk…

Strongly Correlated Electrons · Physics 2016-08-16 Jean-Pascal Rueff , Jean-Paul Itié , M. Taguchi , C. F. Hague , J. -M. Mariot , R. Delaunay , J. -P. Kappler , N. Jaouen

A wide variety of superconducting oxides are used to test a general model of high pressure induced transition temperature (T c) changes. The T c 's vary from a low of 24 K to a high of 164 K. Although the model is capable of predicting both…

Superconductivity · Physics 2015-06-24 Mario Rabinowitz , T. McMullen

For describing the first-order isostructural valence phase transition in mixed valence compounds we develop a new approach based on the lattice Anderson model. We take into account the Coulomb interaction between localized f and conduction…

Strongly Correlated Electrons · Physics 2009-10-31 A. V. Goltsev , G. Bruls

The study of (quantum) phase transitions in heavy-fermion compounds relies on a detailed understanding of the microscopic control parameters that induce them. While the influence of external pressure is rather straight forward, atomic…

Strongly Correlated Electrons · Physics 2020-01-22 Jan M. Tomczak
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