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We report the existence of a phase transition at high temperature in the 3D Kitaev candidate material, $\beta$-Li$_2$IrO$_3$. We show that the transition is bulk, intrinsic and orders a tiny magnetic moment with a spatially anisotropic…

We investigate the structural, magnetic and spin-state transitions, and magnetocaloric properties of Sr$_{2-x}$La$_x$CoNbO$_6$ ($x=$ 0--1) double perovskites. The structural transition from tetragonal to monoclinic phase at $x$ $\geqslant$…

Materials Science · Physics 2020-04-21 Ajay Kumar , R. S. Dhaka

Macroscopic magnetic properties and microscopic magnetic structure of Rb$_2$Mn$_3$(MoO$_4$)$_3$(OH)$_2$ (space group $Pnma$) are investigated by magnetization, heat capacity and single-crystal neutron diffraction measurements. The…

The low and high-temperature phases of V$_4$O$_7$ have been studied by \textit{ab initio} calculations. At high temperature, all V atoms are electronically equivalent and the material is metallic. Charge and orbital ordering, associated…

Strongly Correlated Electrons · Physics 2011-12-06 A. S. Botana , V. Pardo , D. Baldomir , A. V. Ushakov , D. I. Khomskii

Ultra-high resolution synchrotron diffraction data for $\rm GdBaCo_2O_{5.5}$ throw new light on the metal-insulator transition of Co$^{3+}$ Ba-cobaltites. An anomalous expansion of CoO$_6$ octahedra is observed at the phase transition on…

Materials Science · Physics 2016-08-16 C. Frontera , J. L. García-Muñoz , A. Llobet , M. A. G. Aranda

In this paper we have studied, by means of high-resolution neutron powder diffraction and magnetic susceptibility, the structural and magnetic features of selected samples of the HoBaCo2O5+delta layered cobaltite in the low oxygen content…

Materials Science · Physics 2009-11-13 Lorenzo Malavasi , Yuri Diaz-Fernandez , M. Cristina Mozzati , Clemens Ritter

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

The present study reports on the structural and magnetic phase transitions in Pr-doped polycrystalline Tb0.6Pr0.4MnO3, using high-resolution neutron powder diffraction (NPD) collected at SINQ spallation source (PSI), to emphasize the…

Materials Science · Physics 2021-07-07 Harshit Agarwal , Jose A Alonso , Ángel Muñoz , R J Choudhary , O N Srivastava , M A Shaz

Magnetic properties of the pyrovanadate CaCoV$_2$O$_7$ have been studied by means of the bulk magnetization and neutron powder diffraction measurements. Magnetic susceptibility in the paramagnetic phase shows Curie-Weiss behavior with…

Materials Science · Physics 2021-08-03 Ryo Murasaki , Kazuhiro Nawa , Daisuke Okuyama , Maxim Avdeev , Taku J Sato

The properties and mechanism of the magnetic phase transition of the perovskite-type Ti oxides, which is driven by the Ti-O-Ti bond angle distortion, are studied theoretically by using the effective spin and pseudospin Hamiltonian with…

Strongly Correlated Electrons · Physics 2007-05-23 Masahito Mochizuki , Masatoshi Imada

The spin ordering of La3/2Sr1/2NiO4 was investigated by magnetization measurements, and by unpolarized- and polarized-neutron diffraction. Spin ordering with an incommensurability epsilon ~ 0.445 is observed below T_so ~ 80 K. On cooling, a…

Strongly Correlated Electrons · Physics 2009-11-07 P. G. Freeman , A. T. boothroyd , D. Prabhakaran , D. Gonzalez , M. Enderle

We have studied the electronic structure of BaCoO$_3$ using soft x-ray absorption spectroscopy at the Co-$L_{2,3}$ and O-$K$ edges, magnetic circular dichroism at the Co-$L_{2,3}$ edges, as well as valence band hard x-ray photoelectron…

The Pr$_{0.50}$Sr$_{0.5}$0CoO$_3$ perovskite exhibits unique magnetostructural properties among the rest of ferromagnetic/metallic Ln$_{0.50}$Sr$_{0.50}$CoO$_3$ compounds. The sudden orthorhombic-tetragonal (Imma $\to$ I4/mcm) structural…

Several rare earth magnetic pyrochlore materials are well modeled by a spin-1/2 quantum Hamiltonian with anisotropic exchange parameters Js. For the Er2Ti2O7 material, the Js were recently determined from high-field inelastic neutron…

Strongly Correlated Electrons · Physics 2014-04-11 J. Oitmaa , R. R. P. Singh , A. G. R. Day , B. V. Bagheri , M. J. P. Gingras

We present a numerical study of magnetic ordering in spin ice on kagome, a two-dimensional lattice of corner-sharing triangles. The magnet has six ground states and the ordering occurs in two stages, as one might expect for a six-state…

Strongly Correlated Electrons · Physics 2012-11-21 Gia-Wei Chern , Oleg Tchernyshyov

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

A fully ab initio scheme based on quantum chemical wavefunction methods is used to investigate the correlated multiorbital electronic structure of a 3d-metal compound, LaCoO3. The strong short-range electron correlations, involving both Co…

Strongly Correlated Electrons · Physics 2009-11-13 L. Hozoi , U. Birkenheuer , H. Stoll , P. Fulde

We report the comprehensive experimental results identifying the magnetic spin ordering and the magnetization dynamics of a double perovskite Pr2CoFeO6 by employing the (dc and ac) magnetization, powder neutron diffraction (NPD) and X-ray…

We explore the spin states in the quantum spin chain compound SrCo$_{2}$V$_{2}$O$_{8}$ up to 14.9 T and down to 50 mK, using single-crystal neutron diffraction. Upon cooling in zero-field, antiferromagnetic (AFM) order of N\'eel type…

Strongly Correlated Electrons · Physics 2019-07-05 L. Shen , O. Zaharko , J. O. Birk , E. Jellyman , Z. He , E. Blackburn

BaCo2V2O8 is a nice example of a quasi-one-dimensional quantum spin system that can be described in terms of Tomonaga-Luttinger liquid physics. This is explored in the present study where the magnetic field-temperature phase diagram is…

Strongly Correlated Electrons · Physics 2015-06-11 E. Canévet , B. Grenier , M. Klanjšek , C. Berthier , M. Horvatić , V. Simonet , P. Lejay
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