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Related papers: Magnetocaloric Study of Spin Relaxation in `Frozen…

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We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

We have performed AC susceptibility and DC magnetic relaxation measurements on the spin ice system Dy$_2$Ti$_2$O$_7$ down to 0.08 K. The relaxation time of the magnetization has been estimated below 2 K down to 0.08 K. The spin dynamics of…

Strongly Correlated Electrons · Physics 2012-02-07 K. Matsuhira , C. Paulsen , E. Lhotel , C. Sekine , Z. Hiroi , S. Takagi

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

We have studied spin relaxation in the spin ice compound Dy2Ti2O7 through measurements of the a.c. magnetic susceptibility. While the characteristic spin relaxation time is thermally activated at high temperatures, it becomes almost…

Materials Science · Physics 2009-11-10 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , Ari Mizel , P. Schiffer

The intrinsic noncollinear spin patterns in rare-earth pyrochlore are physically interesting, hosting many emergent properties, e.g. spin ice and monopole-type excitation. Recently, the magnetic monopole excitation of spin ice systems was…

Materials Science · Physics 2015-12-18 Lin Lin , Y. L. Xie , J. -J. Wen , Shuai Dong , Z. B. Yan , J. -M. Liu

An adiabatic demagnetization process is studied in Gd2Ti2O7, a geometrically frustrated antiferromagnet on a pyrochlore lattice. In contrast to conventional paramagnetic salts, this compound can exhibit a temperature decrease by a factor of…

Strongly Correlated Electrons · Physics 2007-05-23 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , A. I. Golov , I. B. Berkutov , O. A. Petrenko , G. Balakrishnan , M. E. Zhitomirsky

We report the magneto-dielectric response of single crystals of the spin-ice compound Dy2Ti2O7 down to 0.26 K. The dielectric constant under zero magnetic field exhibits a clear decrease reflecting the development of the local two-spins-in,…

Strongly Correlated Electrons · Physics 2009-11-11 Masafumi Saito , Ryuji Higashinaka , Yoshiteru Maeno

We have studied the low temperature a.c. magnetic susceptibility of the diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y or Lu. We…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , Ari Mizel , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

When degenerate states are separated by large energy barriers, the approach to thermal equilibrium can be slow enough that physical properties are defined by the thermalization process rather than the equilibrium. The exploration of…

The Shastry-Sutherland lattice is a prototypical frustrated quantum magnet. It is notable for its exactly solvable dimer-singlet ground state and hosts a wealth of magnetic phenomena under external fields. Here, this work investigates the…

We have studied spin freezing in the diluted spin ice compound Dy2-xYxTi2O7 where the non-magnetic Y ions replace the magnetic Dy ions on the frustrated pyrochlore lattice. Magnetic a.c. and d.c. susceptibility data are presented with an…

Materials Science · Physics 2009-11-07 J. Snyder , J. S. Slusky , R. J. Cava , P. Schiffer

An external magnetic field induces large relative changes in the entropy of one-dimensional quantum spin systems at finite temperatures. This leads to a magnetocaloric effect, i.e. a change in temperature during an adiabatic…

Strongly Correlated Electrons · Physics 2007-05-23 M. E. Zhitomirsky , A. Honecker

We present an experimental determination of the isothermal magnetic susceptibility of the spin ice materials Dy2Ti2O7 and Ho2Ti2O7 in the temperature range 1.8-300 K. The use of spherical crystals has allowed the accurate correction for…

Strongly Correlated Electrons · Physics 2013-09-02 L. Bovo , L. D. C. Jaubert , P. C. W. Holdsworth , S. T. Bramwell

We herein present the spin freezing dynamics of stuffed polycrystalline compound Dy$_2$Ti$_{1.8}$Mn$_{0.2}$O$_7$. In Dy$_2$Ti$_2$O$_7$, spin freezes with ice-like spin relaxations at a temperature around 3 K (T$_i$) along with another spin…

Materials Science · Physics 2022-05-10 Rajnikant Upadhyay , Manjari Shukla , Rachana Sain , Martin Tolkiehn , Chandan Upadhyay

Low temperature measurements of the ac magnetic susceptibility along the [110] direction of a single crystal of the dipolar spin ice material Ho2Ti2O7, in zero static field, are presented. While behavior that is qualitatively consistent…

Materials Science · Physics 2015-05-27 J. A. Quilliam , L. R. Yaraskavitch , H. A. Dabkowska , B. D. Gaulin , J. B. Kycia

Intensity distribution of the neutron magnetic scattering has been taken in the reciprocal space of a single crystal of the "spin ice" system Ho2Ti2O7 at the elastic energy position in the temperature (T) region between 0.4 K and 50 K. The…

We report vibrating coil magnetometry of the spin ice system Ho2Ti2O7 down to ~0.04 K for magnetic fields up to 5 T applied parallel to the [111] axis. History dependent behavior emerges below T*_0 ~ 0.6 K near zero magnetic field, in…

Strongly Correlated Electrons · Physics 2012-06-25 C. Krey , S. Legl , S. R. Dunsiger , M. Meven , J. S. Gardner , J. M. Roper , C. Pfleiderer

We have studied the field-dependent ac magnetic susceptibility of single crystals of Dy2Ti2O7 spin ice along the [111] direction in the temperature range 1.8 K - 7 K. Our data reflect the onset of local spin ice order in the appearance of…

Strongly Correlated Electrons · Physics 2015-06-12 M. J. Matthews , C. Castelnovo , R. Moessner , S. A. Grigera , D. Prabhakaran , P. Schiffer

We report the low-temperature magnetothermal properties and spin dynamics of a mixed pyrochlore, Dy2GaSbO7 through the coordination of measurements of dc magnetization, ac susceptibility, and heat capacity, and CF computation. In Dy2GaSbO7,…

Materials Science · Physics 2021-04-19 Saikat Nandi , Yatramohan Jana , Jahangir Alam , Pallab Bag , S. S. Islam , Ramesh Nath

Magneto-dielectric spectra of La0.95Ca0.05CoO3 covering the crossover of spin states reveals strong coupling of its spin and dipolar degrees of freedom. Signature of spin-state transition at 30K clearly manifests in magnetization, supported…

Materials Science · Physics 2016-02-29 Suchita Pandey , Jitender Kumar , A. M. Awasthi
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