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We report on the electrostatic complexation between oppositely charged polymers and inorganic nanoparticles investigated by static and dynamical light scattering. The nanoparticles put under scrutiny were citrate-coated nanocrystals of…

Soft Condensed Matter · Physics 2007-09-10 J. -F. Berret

We report on the formation and the structural properties of supermicellar aggregates also called electrostatic complexes, made from mineral nanoparticles and polyelectrolyte-neutral block copolymers in aqueous solutions. The mineral…

Soft Condensed Matter · Physics 2007-09-10 Jean-Francois Berret , Kazuhiko Yokota , Mikel Morvan , Ralf Schweins

We report the formation of stable nanoparticle-polymer clusters obtained by electrostatic complexation. The nanoparticles placed under scrutiny are nanoceria (CeO2) coated by short poly(acrylic acid) moieties, whereas the polymers are…

Materials Science · Physics 2010-02-11 J. Fresnais , C. Lavelle , J. -F. Berret

Engineered nanoparticles made from noble metals, rare-earth oxides or semiconductors are emerging as the central constituents of future nanotech developments. In this review, a survey of the complexing strategies between nanoparticles and…

Materials Science · Physics 2011-08-25 J. -P. Chapel , J. -F. Berret

We report the presence of a correlation between the bulk and interfacial properties of electrostatic coacervate complexes. Complexes were obtained by co-assembly between cationic-neutral diblocks and oppositely charged surfactant micelles…

Soft Condensed Matter · Physics 2007-10-12 Ling Qi , Jean-Paul Chapel , Jean-Christophe Castaing , Jerome Fresnais , Jean-Francois Berret

During the last 3 years, our group has investigated extensively the complexation mechanism between neutral-polyelectrolyte block copolymers with oppositely charged species. These species are surfactant micelles, multivalent counterions and…

Soft Condensed Matter · Physics 2007-05-23 J. -F. Berret , P. Herve , M. Morvan , K. Yokota , M. Destarac , J. Oberdisse , I. Grillo , R. Schweins

When polyelectrolyte-neutral block copolymers are mixed in aqueous solutions with oppositely charged species, stable complexes are found to form spontaneously. The mechanism is based on electrostatics, and on the compensation between the…

When polyelectrolyte-neutral block copolymers are mixed in solutions to oppositely charged species (e.g. surfactant micelles, macromolecules, proteins etc), there is the formation of stable supermicellar aggregates combining both…

Soft Condensed Matter · Physics 2007-05-23 J. -F. Berret , K. Yokota , M. Morvan

The static electric dipole polarizability of $\mathrm{Na_N}$ clusters with even N has been calculated in a collective, axially averaged and a three-dimensional, finite-field approach for $2\le N \le 20$, including the ionic structure of the…

Atomic and Molecular Clusters · Physics 2009-10-31 S. Kümmel , T. Berkus , P. -G. Reinhard , M. Brack

In this review, we address the issue of the electrostatic complexation between charged-neutral diblock copolymers and oppositely charged nanocolloids. We show that nanocolloids such as surfactant micelles and iron oxide magnetic…

Soft Condensed Matter · Physics 2011-02-01 J. -F. Berret

The stability of two-component clusters consisting of light (Na or K) and heavy (Rb or Cs) alkali atoms formed on helium nanodroplets is studied by femtosecond laser ionization in combination with mass spectrometry. Characteristic stability…

Atomic and Molecular Clusters · Physics 2011-12-19 G. Droppelmann , M. Mudrich , C. P. Schulz , F. Stienkemeier

During the past years we have investigated the complexation between nanocolloids and oppositely charged polymers. The nanocolloids examined were ionic surfactant micelles and inorganic oxide nanoparticles. For the polymers, we used…

Soft Condensed Matter · Physics 2007-05-23 Jean-Francois Berret , Regis Cartier

A cluster consisting of many atoms or molecules may be considered, in some circustances, to be a single large molecule with a well defined polarizability. Once the polarizability of such a cluster is known, one can evaluate certain…

Materials Science · Physics 2009-11-11 Hye-Young Kim , Jorge O. Sofo , Darrell Velegol , Milton W. Cole , Gautam Mukhopadhyay

We report the co-assembly and adsorption properties of coacervate complexes made from polyelectrolyte-neutral block copolymers and oppositely charged nanocolloids. The nanocolloids put under scrutiny were ionic surfactant micelles and…

We report on the structural properties of mixed aggregates made from rare-earth inorganic nanoparticles (radius 20 Angstroms) and polyelectrolyte-neutral block copolymers in aqueous solutions. Using scattering experiments and Monte Carlo…

Soft Condensed Matter · Physics 2021-09-27 K. Yokota , M. Morvan , J. -F. Berret , J. Oberdisse

In recent years, there has been a renewed interest in complex coacervation, driven by concerted efforts to offer novel experimental and theoretical insights into electrostatic charge-induced association. While previous studies have…

Soft Condensed Matter · Physics 2024-10-30 Letícia Vitorazi , Jean-François Berret

Network analysis was used to study the structure and time evolution of driven three-dimensional complex plasma clusters. The clusters were created by suspending micron-size particles in a glass box placed on top of the rf electrode in a…

We report the formation of colloidal complexes resulting from the electrostatic co-assembly between anionic surfactants and cationic polyelectrolytes or block copolymers. Combining light and x-ray scattering experiments with cryogenic…

Soft Condensed Matter · Physics 2009-04-01 J. -F. Berret

We report on the complexation between charged-neutral block copolymers and oppositely charged surfactants studied by small-angle neutron scattering. Two block copolymers/surfactant systems are investigated, poly(acrylic…

Soft Condensed Matter · Physics 2007-05-23 Jean-Francois Berret

We review theoretical explanation of mechanisms of control of uniformity in growth of nanosize particles and colloids. The nanoparticles are synthesized as nanocrystals, by burst nucleation from solution. The colloids are self-assembled by…

Statistical Mechanics · Physics 2010-09-22 Vladimir Privman
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