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The alignment of the Fermi level of a metal electrode within the gap of the hi ghest occupied (HOMO) and lowest unoccupied orbital (LUMO) of a molecule is a key quantity in molecular electronics, which can vary the electron transparency of…

Materials Science · Physics 2009-11-11 R. Stadler , K. W. Jacobsen

The alignment of molecular levels with the Fermi energy in single molecule junctions is a crucial factor in determining their conductance or the observability of quantum interference effects. In the present study which is based on density…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Robert Stadler

The alignment of the frontier orbital energies of an adsorbed molecule with the substrate Fermi level at metal-organic interfaces is a fundamental observable of significant practical importance in nanoscience and beyond. Typical density…

Mesoscale and Nanoscale Physics · Physics 2017-03-07 Zhenfei Liu , David A. Egger , Sivan Refaely-Abramson , Leeor Kronik , Jeffrey B. Neaton

Based on density functional calculations, the relationship between magnetism or superconductivity and electronic states around Fermi level were derived, and the location of the Fermi level in nonmagnetic "form" of Laves-phase compounds is…

Materials Science · Physics 2007-05-23 Xing-Qiu Chen , Shu-Lan Wang , Xue-Yong Ding , Xiang-Xun Xue

We review the binding and energy level alignment of $\pi$-conjugated systems on metals, a field which during the last two decades has seen tremendous progress both in terms of experimental characterization as well as in the depth of…

Materials Science · Physics 2020-05-01 Antoni Franco-Cañellas , Steffen Duhm , Alexander Gerlach , Frank Schreiber

First-principles calculations of polar semiconductor nanorods reveal that their dipole moments are strongly influenced by Fermi level pinning. The Fermi level for an isolated nanorod is found to coincide with a significant density of…

Mesoscale and Nanoscale Physics · Physics 2012-06-08 Philip W. Avraam , Nicholas D. M. Hine , Paul Tangney , Peter D. Haynes

Hybridized molecule/metal interfaces are ubiquitous in molecular and organic devices. The energy level alignment (ELA) of frontier molecular levels relative to the metal Fermi level (EF) is critical to the conductance and functionality of…

Materials Science · Physics 2017-07-03 Yifeng Chen , Isaac Tamblyn , Su Ying Quek

Using photoemission spectroscopy, we determine the relationship between electronic energy level alignment at a metal-molecule interface and single-molecule junction transport data. We measure the position of the highest occupied molecular…

Mesoscale and Nanoscale Physics · Physics 2010-06-28 M. Dell'Angela , G. Kladnik , A. Cossaro , A. Verdini , M. Kamenetska , I. Tamblyn , S. Y. Quek , J. B. Neaton , D. Cvetko , A. Morgante , L. Venkataraman

The dependence of the transport properties on the specific location of the Fermi level in molecular electronics devices is studied by using electrodes of different materials. The zero-bias transport properties are shown to depend…

Mesoscale and Nanoscale Physics · Physics 2008-12-06 V. M. García-Suárez , C. J. Lambert

We describe the proximity effect in a short disordered metallic junction between three superconducting leads. Andreev bound states in the multi-terminal junction may cross the Fermi level. We reveal that for a quasi-continuous metallic…

Mesoscale and Nanoscale Physics · Physics 2015-11-13 C. Padurariu , T. Jonckheere , J. Rech , R. Mélin , D. Feinberg , T. Martin , Yu. V. Nazarov

In materials science, point defects play a crucial role in materials properties. This is particularly well known for the wide band gap insulators where the defect formation/compensation determines the equilibrium Fermi level and generally…

Materials Science · Physics 2023-11-29 Harshan Reddy Gopidi , Lovelesh Vashist , Oleksandr I. Malyi

To explore the origin of the Fermi level pinning in germanium we investigate the Ge(001) and Ge(001):H surfaces. The absence of relevant surface states in the case of Ge(001):H should unpin the surface Fermi level. This is not observed. For…

We present a theoretical study of the electronic transport through single-molecule junctions incorporating a Pt6 metal cluster bound within an organic framework. We show that the insertion of this molecule between a pair of electrodes leads…

Mesoscale and Nanoscale Physics · Physics 2013-02-27 Linda A. Zotti , Edmund Leary , Maria Soriano , Juan Carlos Cuevas , Juan Jose Palacios

The conductance of a molecular junction is commonly determined by either charge-transfer-doping, where alignment of the Fermi energy to the molecular levels is achieved, or tunnelling through the tails of molecular resonances within the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 R. Gutierrez , G. Fagas , K. Richter , F. Grossmann , R. Schmidt

Graphene devices require electric contacts with metals, particularly with gold. Scanning tunneling spectroscopy studies of electron local density of states performed on mono-, bi- and tri- graphene layer deposited on metallic conductive…

Materials Science · Physics 2009-01-05 Z. Klusek , P. Dabrowski , P. Kowalczyk , W. Kozlowski , P. Blake , M. Szybowicz , T. Runka , W. Olejniczak

Choosing self-assembled monolayers (SAM) of fluorine terminated oligophenylenes adsorbed on gold as illustration, we show that a single level (molecular orbital, MO) model can excellently reproduce full I-V curves measured for large area…

Mesoscale and Nanoscale Physics · Physics 2024-03-11 Ioan Baldea

Properties of the distribution of single-particle levels adjacent to the Fermi surface in finite Fermi systems are studied, focusing on the case in which these levels are degenerate. The interaction of the quasiparticles occupying these…

Strongly Correlated Electrons · Physics 2009-11-11 V. A. Khodel , J. W. Clark , Haochen Li , M. V. Zverev

Fermi arcs represent the surface states at the boundary of a three-dimensional topological semimetal with the vacuum, illustrating the notion of bulk-boundary correspondence playing out in real materials. Their special character is tied up…

Mesoscale and Nanoscale Physics · Physics 2025-10-22 Ipsita Mandal

The "density-density" correlation function of conduction electrons in metal is investigated. It is shown, that the asymptotic behaviour of the CF depends on the shape and the local geometry of the Fermi surface. In particular, the exponent…

Condensed Matter · Physics 2009-10-22 D. I. Golosov , M. I. Kaganov

The quantum phase transitions of metals have been extensively studied in the rare-earth "heavy electron" materials, the cuprates, and related compounds. The Fermi surface of the metal often has different shapes in the states well away from…

Strongly Correlated Electrons · Physics 2007-05-23 Ribhu K. Kaul , Alexei Kolezhuk , Michael Levin , Subir Sachdev , T. Senthil
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