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Ab initio self-consistent total energy calculations using second order Moller-Plesset perturbation theory and Hay-Wadt effective core potentials for gallium and arsenic have been used to investigate the chemisorption of atomic oxygen on the…

Condensed Matter · Physics 2007-05-23 Michael L. Mayo , Asok K. Ray

In this paper, we discuss the dissociative electron attachment process in Methane. Kinetic energy and angular distributions of H^{-} and CH_{2}^{-} fragment anions across the broad resonance about 10 eV is reported. Angular distribution of…

Chemical Physics · Physics 2010-07-30 N. Bhargava Ram , E. Krishnakumar

Using first-principles calculations, we systematically study the potential energy surfaces and dissociation processes of the hydrogen molecule on the Mg(0001) surface. It is found that during the dissociative adsorption process with the…

Materials Science · Physics 2015-05-13 Yanfang Li , Yu Yang , Bo Sun , Hong-Zhou Song , Yinghui Wei , Ping Zhang

The geometric, electronic, energetic, and dynamic properties of 1-propanol adsorbed on the Si(001)-2x1 surface are studied from first principles by use of a slab approach. The 1-propanol molecule initially interacts with the Si surface…

Materials Science · Physics 2009-11-11 Jian-Ge Zhou , Frank Hagelberg , Chuanyun Xiao

The Work function (f)is fundamental for chemistry and electronics. Additionally, f can be used to examine the validity of the theoretical surfaces by comparing it with experimental f, even in the absence of long-range orders. In the…

Materials Science · Physics 2025-07-10 Yukio Watanabe , S. Miyauchi , S. Kaku , T. Yamada , A. Horiguchi

A comparative first principles pseudopotential study of the adsorption and migration profiles of single Pt and Au atoms on the stoichiometric and reduced TiO2 rutile (110) surfaces is presented. Pt and Au behave similarly with respect to…

Materials Science · Physics 2009-11-10 Hakim Iddir , Serdar Ogut , Nigel D. Browning , Mark M. Disco

A new classical potential for methyl-thiol on a Au(111) surface has been developed using density functional theory electronic structure calculations. Energy surfaces between methyl-thiol and a gold surface were investigated in terms of…

Materials Science · Physics 2007-10-24 Byoungseon Jeon , Joel D. Kress , Niels Grønbech-Jensen

We investigate the atomic and electronic structure of a single layer of pentacene on the Au(111) surface using density functional theory. To find the candidate structures we strain match the pentacene crystal geometry with the Au(111)…

Materials Science · Physics 2013-08-06 Kurt Stokbro , Søren Smidstrup

The characterization and applications of topological insulators depend critically on their protected surface states, which, however, can be obscured by the presence of trivial dangling bond states. Our first principle calculations show that…

Materials Science · Physics 2014-12-25 Yin Shi , Meng Wu , Fan Zhang , Ji Feng

The adsorption of the chiral molecule lactate on the intrinsically chiral noble metal surfaces Pt(321), Au(321) and Ag(321) is studied by Density Functional Theory calculations. We use the oPBE-vdW functional which includes van der Waals…

Materials Science · Physics 2015-06-17 J. -H. Franke , D. S. Kosov

The interactions of atomic and molecular hydrogen with bare interstellar dust grain surfaces are important for understanding H2 formation at relatively high temperatures (>20 K). We investigate the diffusion of physisorbed H atoms and the…

Astrophysics of Galaxies · Physics 2019-11-14 Masashi Tsuge , Tetsuya Hama , Yuki Kimura , Akira Kouchi , Naoki Watanabe

We present a first-principles study of the atomic hydrogen adsorption onto the Be(10\={1}0) thin film. There are two types of Be(10\={1}0) surfaces according to the interlayer spacing between the surface and its nearest-neighbor layer. We…

Materials Science · Physics 2007-05-23 Ping Zhang , Hong-Zhou Song

Using helium-3 atom scattering, we have studied the adsorption kinetics, the structure and the diffusional dynamics of atomic hydrogen on the surface of a graphene monolayer on Ni(111). Diffraction measurements reveal a 4$^\circ$ rotated…

Mesoscale and Nanoscale Physics · Physics 2022-12-15 Emanuel Bahn , Anton Tamtögl , John Ellis , William Allison , Peter Fouquet

The structure and dynamics of atomic oxygen adsorbed on Ag(410) and Ag(210) surfaces have been investigated using density functional theory. Our results show that the adsorption configuration in which O adatoms decorate the upper side of…

Materials Science · Physics 2009-11-10 N. Bonini , A. Kokalj , A. Dal Corso , S. de Gironcoli , S. Baroni

Atomic and molecular scattering at semiconductor interfaces plays a central role in surface chemistry and catalysis, yet predictive simulations remain challenging due to strong nonadiabatic effects causing the breakdown of the…

Materials Science · Physics 2026-01-16 Xiaohan Dan , Zhuoran Long , Tianyin Qiu , Jan Paul Menzel , Qiang Shi , Victor S. Batista

The results of DFT GGA calculations on oxygen molecules adsorbed upon the (001) surface of uranium mononitride (UN) are presented and discussed. We demonstrate that O2 molecules oriented parallel to the substrate can dissociate either (i)…

Materials Science · Physics 2010-09-01 Yuri F. Zhukovskii , Dmitry Bocharov , Eugene A. Kotomin

A key step towards building single molecule machines is to control the rotation of molecules and nanostructures step by step on a surface. Here, we used the tunneling electrons coming from the tip of a scanning tunneling microscope to…

Mesoscale and Nanoscale Physics · Physics 2020-05-19 Frank Eisenhut , Jörg Meyer , Justus Krüger , Robin Ohmann , Gianaurelio Cuniberti , Francesca Moresco

A pi-conjugated {C}3h-oligomer involving three dithienylethylene branches bridged at the meta positions of a central benzenic core has been synthesized and deposited either on the Si(100) surface or on the HOPG surface. On the silicon…

Stable organic radicals serve as model systems for investigating metal-free magnetic phenomena at (sub)nanometer length scales. We have investigated at the single-molecule level the stable $\pi$-radical 2,2-diphenyl-1-picrylhydrazyl (DPPH)…

Instrumentation and Detectors · Physics 2021-01-13 Radovan Vranik , Vitalii Stetsovych , Simon Feigl , Stefan Müllegger

The adsorption of pentacene on Cu(221), Cu(511) and Cu(911) is investigated using density functional theory (DFT) with the self-consistent inclusion of van der Waals (vdW) interactions. Cu(211) is a vicinal of Cu(111) while Cu(511) and…

Materials Science · Physics 2016-09-21 Jeronimo Matos , Abdelkader Kara
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