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In a retroreflective scheme atomic Raman diffraction adopts some of the properties of Bragg diffraction due to additional couplings to off-resonant momenta. As a consequence, double Raman diffraction has to be performed in a Bragg-type…

Quantum Physics · Physics 2022-09-08 Sabrina Hartmann , Jens Jenewein , Sven Abend , Albert Roura , Enno Giese

The study of strong electron correlations in transition metal oxides with modern microscopy and diffraction techniques unveiled a fascinating world of nanosize textures in the spin, charge, and crystal structure. Examples range from high…

Strongly Correlated Electrons · Physics 2007-05-23 G. Papavassiliou , M. Pissas , M. Belesi , M. Fardis , D. Stamopoulos , A. Kontos , M. Hennion , J. Dolinsek , J. P. Ansermet , C. Dimitropoulos

Some of the most exotic material properties derive from electronic states with short correlation length (~10-500 {\AA}), suggesting that the local structural symmetry may play a relevant role in their behavior. Here we discuss the combined…

Materials Science · Physics 2017-04-05 Gilberto Fabbris , Markus Hücker , Genda Gu , John M. Tranquada , Daniel Haskel

A method is described for using resonant x-ray scattering to separately quantify the charge (valence) modulation and the strain wave associated with a charge density wave. The essence of the method is a separation of the atomic form factor…

Strongly Correlated Electrons · Physics 2010-11-09 P. Abbamonte

We have performed a resonant x-ray scattering (RXS) study near the Co K edge on a single crystal of Ca3Co2O6. In the magnetically ordered phase a new class of weak reflections appears at the magnetic propagation vector tau (1/3,1/3,1/3).…

Strongly Correlated Electrons · Physics 2009-11-13 A. Bombardi , C. Mazzoli , S. Agrestini , M. R. Lees

We theoretically analyze the intensity of the resonant inelastic X-ray scattering (RIXS) based on Ansatz that the electron is fractionalized into two components. By fitting the angle resolved photoemission spectroscopy (ARPES) data of a…

Strongly Correlated Electrons · Physics 2021-07-26 Masatoshi Imada

The effect of x-rays on an orbital and charge ordered epitaxial film of a Pr$_{0.5}$Ca$_{0.5}$MnO$_{3}$ is presented. As the film is exposed to x-rays, the antiferromagnetic response increases and concomitantly the conductivity of the film…

Strongly Correlated Electrons · Physics 2012-10-11 M. Garganourakis , V. Scagnoli , S. W. Huang , U. Staub , H. Wadati , M. Nakamura , V. A. Guzenko , M. Kawasaki , Y. Tokura

We present a combined study of Ni $K$-edge resonant x-ray scattering and density functional calculations to probe and distinguish electronically driven ordering and lattice distortions in nickelate heterostructures. We demonstrate that due…

We theoretically investigate the origin of the resonant x-ray scattering (RXS) signal near the Ce $L_{III}$ absorption edge in the quadrupolar ordering phase of CeB$_6$, considering the intersite interaction between the $\Gamma_8$ states in…

Strongly Correlated Electrons · Physics 2009-11-07 Tatsuya Nagao , Jun-ichi Igarashi

Diffraction imaging of non-equilibrium dynamics at atomic resolution is becoming possible with X-ray free-electron lasers. However, there are unresolved problems with applying this method to objects that are confined in only one dimension.…

Strongly Correlated Electrons · Physics 2018-02-19 Kenneth R. Beyerlein

We report resonant x-ray scattering studies of charge and orbital order in Pr_{1-x}Ca_{x}MnO_3 with x=0.4 and 0.5. Below the ordering temperature, T_O=245 K, the charge and orbital order intensities follow the same temperature dependence,…

Strongly Correlated Electrons · Physics 2009-10-31 M. v. Zimmermann , J. P. Hill , Doon Gibbs , M. Blume , D. Casa , B. Keimer , Y. Murakami , Y. Tomioka , Y. Tokura

We study resonant x-ray scattering (RXS) at Np M_{4,5} edges in the triple-\textbf{k} multipole ordering phase in NpO_{2}, on the basis of a localized electron model. We derive an expression for RXS amplitudes to characterize the spectra…

Strongly Correlated Electrons · Physics 2015-06-25 Tatsuya Nagao , Jun-ichi Igarashi

We have grown epitaxial films a few atomic layers thick of iron oxides on ruthenium. We characterize the growth by low energy electron microscopy. Using selected area diffraction and intensity vs. voltage spectroscopy, we detect two…

Characterizing electrochemical energy conversion devices during operation is an important strategy for correlating device performance with the properties of cell materials under real operating conditions. While operando characterization has…

Applied Physics · Physics 2018-08-07 Jesse D. Benck , Daniel Rettenwander , Ariel Jackson , David Young , Yet-Ming Chiang

Linear polarization analysis of hard x-rays is employed to probe electronic anisotropies in metal-containing complexes with very high selectivity. We use the pronounced linear dichroism of nuclear resonant x-ray scattering to determine…

In layered manganites with orbital and charge orderings, the degeneracy of the Mn $4p$ orbitals as well as the $3d$ ones is lifted by the effects of the $4p$ bands and the local Coulomb interactions. We formulate the atomic scattering…

Strongly Correlated Electrons · Physics 2009-10-31 Sumio Ishihara , Sadamichi Maekawa

A recent polarized neutron diffraction experiment on the 5d2 rhenium double perovskite Ba2YReO6 held at a low temperature uncovered weak magnetic diffraction peaks. Data analysis inferred a significantly reduced Re dipole moment, and…

Strongly Correlated Electrons · Physics 2021-03-24 S. W. Lovesey , D. D. Khalyavin , G. van der Laan , G. J. Nilsen

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge density wave order,…

Strongly Correlated Electrons · Physics 2017-07-03 T. P. Devereaux , A. M. Shvaika , K. Wu , K. Wohlfeld , C. J. Jia , Y. Wang , B. Moritz , L. Chaix , W. -S. Lee , Z. -X. Shen , G. Ghiringhelli , L. Braicovich

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. In this work, we will investigate how RIXS can…

Superconductivity · Physics 2016-05-13 Pasquale Marra

The intercalation of alkali ions into layered materials has played an essential role in battery technology since the development of the first lithium-ion electrodes. Coulomb repulsion between the intercalants leads to ordering of the…

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