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Electron transport properties of C$_{20}$ molecules suspended between gold electrodes are investigated using first-principles calculations. Our study reveals that the conductances are quite sensitive to the number of C$_{20}$ molecules…

Condensed Matter · Physics 2009-11-10 Megumi Otani , Tomoya Ono , Kikuji Hirose

The first electrical conductivity measurements of monoatomic carbon chains are reported in this study. The chains were obtained by unraveling carbon atoms from graphene ribbons while an electrical current flowed through the ribbon and,…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 O. Cretu , A. R. Botello-Mendez , I. Janowska , C. Pham-Huu , J. -C. Charlier , F. Banhart

C60 fullerene has been studied extensively, as it is considered to be a good candidate for building single-molecule junctions. Here, we theoretically demonstrate that the conductance of single-molecule junctions based on a newly discovered…

Mesoscale and Nanoscale Physics · Physics 2015-11-19 Chengbo Zhu , Xiaolin Wang

We have investigated the electronic properties of a C_60 molecule in between carbon nanotube leads. This problem has been tackled within a quantum chemical treatment utilizing a density functional theory-based LCAO approach combined with…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 G. Cuniberti , R. Gutierrez , G. Fagas , F. Grossmann , K. Richter , R. Schmidt

Applying a first-principles computational approach, we have systematically analyzed the effects of [2+2] cycloaddition oligomerization of fullerene C60 chains on their junction electronic and charge transport properties. For hypothetical…

Mesoscale and Nanoscale Physics · Physics 2014-07-09 Han Seul Kim , Jhinhwan Lee , Yong-Hoon Kim

Superconductivity in the new polymerized C60 fullerite clathrate doped with simple metals was investigated through density functional theory methods. The phonon dispersion curves were systematically computed for the clathrate structures…

Single-walled carbon nanotubes (SWCNTs) in their pristine form have high thermal conductivity whose further improvement has attracted a lot of interest. Some theoretical studies have suggested that the thermal conductivity of a $(10,10)$…

Materials Science · Physics 2020-02-11 Haikuan Dong , Zheyong Fan , Ping Qian , Tapio Ala-Nissila , Yanjing Su

The charge flow from a single C60 molecule to another one has been probed. The conformation and electronic states of both molecules on the contacting electrodes have been characterized using a cryogenic scanning tunneling microscope. While…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Guillaume Schull , Thomas Frederiksen , Mads Brandbyge , Richard Berndt

We study the transport of electrons through a long quantum wire connecting two bulk leads. As the electron density in the wire is lowered, the Coulomb interactions lead to short-range crystalline ordering of electrons. In this Wigner…

Mesoscale and Nanoscale Physics · Physics 2010-07-23 K. A. Matveev

Recent experiments have shown that C60 can be positively field-doped. In that state, fullerene exhibits a higher resistivity and a higher superconducting temperature than the corresponding negatively doped state. A strong intramolecular…

Superconductivity · Physics 2009-11-07 Nicola Manini , Andrea Dal Corso , Michele Fabrizio , Erio Tosatti

Single molecule transistors (SMTs) are currently attracting enormous attention as possible quantum information processing devices. An intrinsic limitation to the prospects of these however is associated to the presence of a small number of…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 C. B. Winkelmann , N. Roch , W. Wernsdorfer , V. Bouchiat , F. Balestro

We offer a new theoretical interpretation for the effect of enhanced electron density at $^7$Be nucleus encapsulated in fullerene C$_{60}$. Our {\it{ab initio}} Hartree-Fock calculations show that electron density at the $^7$Be nucleus in…

Nuclear Theory · Physics 2010-04-06 E. V. Tkalya , A. V. Bibikov , I. V. Bodrenko

We study the conductance of an interconnect between two graphene leads formed by a single-atom carbon chain. Its dependence on the chemical potential and the number of atoms in the chain is qualitatively different from that in the case of…

Mesoscale and Nanoscale Physics · Physics 2011-09-12 Wei Chen , A. V. Andreev , G. F. Bertsch

The quasi-hexagonal phase of the two-dimensional fullerene network (qHPC$_{60}$), recently synthesized, has emerged as a stable carbon-based material with distinct structural and electronic features. In this work, we employed density…

We study the interplay of intrinsic-electronic and environmental factors on long-range charge transport across molecular chains with up to $N\sim 80$ monomers. We describe the molecular electronic structure of the chain with a tight-binding…

Mesoscale and Nanoscale Physics · Physics 2022-09-21 Francisco Lai Liang , Dvira Segal

We present a theoretical study of the conductance and thermopower of single-molecule junctions based on C60 and C60-terminated molecules. We first analyze the transport properties of gold-C60-gold junctions and show that these junctions can…

Mesoscale and Nanoscale Physics · Physics 2012-06-08 S. Bilan , L. A. Zotti , F. Pauly , J. C. Cuevas

We investigate the accuracy of first-principles many-body theories at the nanoscale by comparing the low energy excitations of the carbon fullerenes C_20, C_24, C_50, C_60, C_70, and C_80 with experiment. Properties are calculated via the…

Materials Science · Physics 2009-11-13 Murilo L. Tiago , P. R. C. Kent , Randolph Q. Hood , Fernando A. Reboredo

Electronic structure and transport properties of the fullerene C$_{82}$ and the metallofullerene Gd@C$_{82}$ are investigated with density functional theory and the Landauer-Buttiker formalism. The ground state structure of Gd@C$_{82}$ is…

Other Condensed Matter · Physics 2007-05-23 Laxmidhar Senapati , Joshua Schrier , K. Birgitta Whaley

We present first principles calculations of current-voltage characteristics (IVC) and conductance of Au(111):S2-cumulene-S2:Au(111) molecular wire junctions with realistic contacts. The transport properties are calculated using full…

Mesoscale and Nanoscale Physics · Physics 2010-09-30 J. Prasongkit , A. Grigoriev , G. Wendin , Rajeev Ahuja

We explore the possibility to trap polynitrogen clusters inside C60 fullerene cage, opening a new direction of developing nitrogen-rich high energy materials. We found that a maximum of 13 nitrogen atoms can be encapsulated in a C60 cage.…

Mesoscale and Nanoscale Physics · Physics 2009-08-25 Hitesh Sharma , Isha Garg , Keya Dharamvir , V. K. Jindal
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