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Linear response methods are applied to identify the increase in electron-phonon coupling in elemental yttrium that is responsible for its high superconducting critical temperature Tc, which reaches nearly 20 K at 115 GPa. While the…

Superconductivity · Physics 2007-05-23 Z. P. Yin , S. Y. Savrasov , W. E. Pickett

The highest superconducting temperature T$_c$ observed in any elemental metal (Li with T$_c$ ~ 20 K at pressure P ~ 40 GPa) is shown to arise from critical (formally divergent) electron-phonon coupling to the transverse T$_1$ phonon branch…

Superconductivity · Physics 2009-11-11 Deepa Kasinathan , J. Kunes , A. Lazicki , H. Rosner , C. S. Yoo , R. T. Scalettar , W. E. Pickett

The phonon dispersion and the electron-phonon interaction for the $\beta$-Po and the bcc high pressure phases of tellurium are computed with density-functional perturbation theory. Our calculations reproduce and explain the experimentally…

The lattice dynamical properties of Li$_x$BC are calculated for several values of $x$ using density functional perturbation theory. We find that the electron-phonon coupling parameter $\lambda$ increases monotonically with decreasing $x$ to…

Superconductivity · Physics 2009-11-07 J. K. Dewhurst , S. Sharma , C. Ambrosch-Draxl , B. Johansson

We observe strong softening of optical phonon modes in superconducting (Tc = 4.2 K) boron doped diamond near the Brillouin zone center using inelastic x-ray scattering from a CVD-grown highly oriented sample. The magnitude of the softening,…

We calculate Tc map in region of weak electron-phonon coupling based on simple phonon spectrum. By using linear-response method and density functional theory, we calculate phonon spectra and Eliashberg functions of simple metals under…

Superconductivity · Physics 2010-08-18 Fan Wei , Y. L. Li , J. L. Wang , L. J. Zou , Z. Zeng

Recent experiments [Schaeffer 2015] have shown that lithium presents an extremely anomalous isotope effect in the 15-25 GPa pressure range. In this article we have calculated the anharmonic phonon dispersion of $\mathrm{^7Li}$ and…

Superconductivity · Physics 2017-11-15 Miguel Borinaga , Unai Aseginolaza , Ion Errea , Matteo Calandra , Francesco Mauri , Aitor Bergara

Motivated by unexpected reports of a 26 K superconducting transition in elemental titanium at high pressure, we carry out an accurate ab-initio study of its properties to understand the rationale for this observation. The critical…

Superconductivity · Physics 2023-08-29 Antonio Sanna , Camilla Pellegrini , Simone di Cataldo , Giannni Profeta , Lilia Boeri

Understanding the phase stability of elemental lithium (Li) is crucial for optimizing its performance in lithium-metal battery anodes, yet this seemingly simple metal exhibits complex polymorphism that requires proper accounting for quantum…

Materials Science · Physics 2025-02-24 Yiheng Shen , Wei Xie

Lithium transition metal phospho-olivines are useful electrode materials, owing to their stability, high safety, low cost and cyclability. We report phonon studies using neutron inelastic scattering experiments, ab-initio density functional…

Materials Science · Physics 2014-08-19 Prabhatasree Goel , M. K. Gupta , R. Mittal , S. Rols , S. J. Patwe , S. N. Achary , A. K. Tyagi , S. L. Chaplot

Possible variations in the dynamical behaviour of LiYF$_{4}$ due to its several structural changes under pressure are examined by making use of the complementary techniques of quasi-harmonic lattice dynamics and molecular dynamics…

Materials Science · Physics 2007-05-23 A. Sen , S. L. Chaplot , R. Mittal

Density functional perturbation theory calculations of alpha-quartz using extended norm conserving pseudopotentials have been used to study the elastic properties and phonon dispersion relations along various high symmetry directions as a…

Materials Science · Physics 2007-05-23 N. Choudhury , S. L. Chaplot

Possible variations in the dynamical behaviour of LiYF$_{4}$ due to its structural changes following several pressure-induced phase transitions are examined by making use of the complementary techniques of quasi-harmonic lattice dynamics…

Materials Science · Physics 2007-05-23 A. Sen , S. L. Chaplot , R. Mittal

Recently reported structural complexity and superconducting transition in lithium under pressure has increased the interest in light alkalis, otherwise considered as simple metals and well known systems under normal conditions. In this work…

Materials Science · Physics 2007-05-23 A. Rodriguez-Prieto , A. Bergara

The mechanisms for strong electron-phonon coupling predicted for hydrogen-rich alloys with high superconducting critical temperature ($T_c$) are examined within the Migdal-Eliashberg theory. Analysis of the functional derivative of $T_c$…

Superconductivity · Physics 2017-09-28 K. Tanaka , J. S. Tse , H. Liu

We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe$_2$. We observe a complete softening of a transverse optic phonon at the L point, i.e. q = (0.5, 0, 0.5), at T ~…

Strongly Correlated Electrons · Physics 2015-05-28 F. Weber , S. Rosenkranz , J. -P. Castellan , R. Osborn , G. Karapetrov , R. Hott , R. Heid , K. -P. Bohnen , A. Alatas

The intermetallic compound TlBi$_2$ crystallizes in the MgB$_2$ structure and becomes superconducting below 6.2 K. Considering that both Tl and Bi have heavy atomic masses, it is puzzling why TlBi$_2$ is a conventional phonon-mediated…

Superconductivity · Physics 2023-12-27 Aiqin Yang , Xiangru Tao , Yundi Quan , Peng Zhang

We present temperature dependent inelastic neutron scattering measurments, accompanied byab-initio calculations of phonon spectra and elastic properties as a function of pressure to understand anharmonicity of phonons and to study the…

Using electronic structure calculation we study the superconducting properties of the theoretically-devised superconductor MS1-LiB (LiB). We calculate the electron-phonon coupling ($\lambda=0.62$) and the phonon frequency logarithmic…

Superconductivity · Physics 2007-05-23 Matteo Calandra , Aleksey N. Kolmogorov , Stefano Curtarolo

We have studied the lattice dynamics, electron-phonon coupling, and superconducting properties of $\alpha$-MoB$_2$, as a function of applied pressure, within the framework of density functional perturbation theory using a mixed-basis…

Superconductivity · Physics 2023-10-31 Marco-Antonio Carmona-Galván , Rolf Heid , Omar De la Peña-Seaman
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