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The electronic properties of thin metallic films deviate from the corresponding bulk ones when the film thickness is comparable with the wavelength of the electrons at the Fermi level due to quantum size effects (QSE). QSE are expected to…

Materials Science · Physics 2009-11-07 L. Floreano , D. Cvetko , F. Bruno , G. Bavdek , A. Cossaro , R. Gotter , A. Verdini , A. Morgante

We show from density-functional calculations that Pb(100) thin films exhibit quantum size effect with a bilayer periodicity in film energies, film relaxations, and work functions, which originate from different symmetry of the stacking…

Materials Science · Physics 2017-03-27 Dengke Yu , Matthias Scheffler , Mats Persson

Quantum manifestations of various properties of metallic thin films by quantum size effect (QSE) have been studied intensively. Here, using first-principles calculations, we show quantum manifestation in dielectric properties of Al(111)…

Materials Science · Physics 2015-06-19 Wenmei Ming , Steve Blair , Feng Liu

We have studied Pb thin films as a function of the thickness up to 60 monolayers (MLs) using ab initio first principles and model calculations. Magic heights corresponding to a modulated oscillatory pattern of the energy of Pb(111) films…

Materials Science · Physics 2024-02-13 A. Ayuela , E. Ogando , N. Zabala

A theoretical study of the surface energy-loss function of freestanding Pb(111) thin films is presented, starting from the single monolayer case. The calculations are carried applying the linear response theory, with inclusion of the…

Materials Science · Physics 2013-04-11 X. Zubizarreta , E. V. Chulkov , V. M. Silkin

The Pb/Si(111) thin films were simulated within the density functional theory (DFT). The well-known Perdew-Burke-Ernzerhof (PBE) version of the generalized gradient approximation (GGA) and its recent nonempirical successor Wu-Cohen (WC)…

Mesoscale and Nanoscale Physics · Physics 2009-11-23 M. Rafiee , S. Jalali Asadabadi

Using first-principles calculations, we have systematically studied the quantum size effects of ultrathin Pb(111) films on the adsorption energies and diffusion energy barriers of oxygen atoms. For the on-surface adsorption of oxygen atoms…

Chemical Physics · Physics 2015-05-14 Ziyu Hu , Yu Yang , Bo Sun , Xiaohong Shao , Wenchuan Wang , Ping Zhang

We report the thickness-dependent (in terms of atomic layers) oscillation behavior of the perpendicular upper critical field $H_{c2\perp}$ in the ultra-thin lead films at the reduced temperature ($t=T/T_c$). Distinct oscillations of the…

Superconductivity · Physics 2007-05-23 Xin-Yu Bao , Yan-Feng Zhang , Yupeng Wang , Jin-Feng Jia , Qi-Kun Xue , X. C. Xie , Zhong-Xian Zhao

The quantum size effect on the in-plane paramagnetic critical field in Pb nanofilms is investigated with the use of the spin-generalized Bogolubov-de Gennes equations. It is shown that the critical field oscillates as a function of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 P. Wójcik , M. Zegrodnik

The magnetoconductive properties of ultrathin Pb films deposited on Si(111) are measured and compared with density-functional electronic band-structure calculations on two-dimensional, free-standing, 1 to 8 monolayers thick Pb(111) slabs. A…

Materials Science · Physics 2009-11-07 I. Vilfan , M. Henzler , O. Pfennigstorf , H. Pfnuer

In nano-structures such as thin films electron confinement results in the quantization of energy levels in the direction perpendicular to the film. The discretization of the energy levels leads to the oscillatory dependence of many…

Mesoscale and Nanoscale Physics · Physics 2018-08-09 Thomas Späth , Matthias Popp , Carmen Pérez León , Michael Marz , Regina Hoffmann-Vogel

Morphological instability of a planar surface ([111], [011], or [001]) of an ultra-thin metal film is studied in a parameter space formed by three major effects (the quantum size effect, the surface energy anisotropy and the surface stress)…

Materials Science · Physics 2020-12-03 Mikhail Khenner

The optical properties of periodic electromagnetic metamaterials are considered as functions of their relative unit cell size $d / \lambda$. The reflection $R$ and transmission $T$ coefficients are numerically calculated for some realistic…

Optics · Physics 2023-01-10 Victor V. Gozhenko

Conductivity of quantized multilayer metal films is analyzed with an emphasis on scattering by rough interlayer interfaces. Three different types of quantum size effect (QSE) in conductivity are predicted. Two of these QSE are similar to…

Mesoscale and Nanoscale Physics · Physics 2009-01-09 I. V. Ponomarev , A. E. Meyerovich

We analyze topographic scanning force microscopy images together with Kelvin probe images obtained on Pb islands and on the wetting layer on Si(111) for variable annealing times. Within the wetting layer we observe negatively charged…

Mesoscale and Nanoscale Physics · Physics 2020-01-16 Th. Späth , M. Popp , R. Hoffmann-Vogel

The extrinsic size effect in Piezoresponse Force Microscopy of ferroelectric and piezoelectric thin films on non-polar dielectric substrate is analyzed. Analytical expressions for effective piezoresponse, object transfer function…

Materials Science · Physics 2009-11-13 Anna N. Morozovska , Sergei V. Svechnikov , Eugene A. Eliseev , Sergei V. Kalinin

We have carried out first-principles calculation of Mg(0001) free-standing thin films to study the oscillatory quantum size effect exhibited in the surface energy, work function, interlayer relaxation, and adsorption energy of the atomic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Ping Zhang

a-Nb(x)Si(1-x) thin films with thicknesses down to 25 {\AA} have been structurally characterized by TEM (Transmission Electron Microscopy) measurements. As-deposited or annealed films are shown to be continuous and homogeneous in…

Superconductivity · Physics 2013-04-29 O. Crauste , A. Gentils , F. Couëdo , Y. Dolgorouky , L. Bergé , S. Collin , C. A. Marrache-Kikuchi , L. Dumoulin

The quantum size effect (QSE) and strain effect are two key factors influencing the surface morphology of thin films, which can increase film surface roughness through QSE-induced thickness oscillation and strain-induced island formation,…

The electrical conductance and RHEED intensities as a function of the coverage have been measured during Pb depositions at 105 K on Si(111)-(6x6)Au with up to 4.2 ML of annealed Pb. The experiments show the strong influence of used…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Z. Korczak , T. Kwapinski
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