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We report experimental measurements of electronic Raman scattering under resonant conditions by electrons in individual single-walled carbon nanotubes (SWNTs). The inelastic Raman scattering at low frequency range reveals a single particle…

Mesoscale and Nanoscale Physics · Physics 2014-05-12 Xi Chen , Bairen Zhu , Anmin Zhang , Hualing Zeng , Qingming Zhang , Xiaodong Cui

We present experimental measurements of the electronic contribution to the Raman spectra of individual metallic single-walled carbon nanotubes (MSWNTs). Photoexcited carriers are inelastically scattered by a continuum of low-energy…

Mesoscale and Nanoscale Physics · Physics 2011-10-20 Hootan Farhat , Stéphane berciaud , Martin Kalbac , Riichiro Saito , Tony F. Heinz , Mildred S. Dresselhaus , Jing Kong

The electronic Raman scattering (ERS) features of single-walled carbon nanotubes (SWNTs) can reveal a wealth of information about their electronic structures, but have previously been thought to appear exclusively in metallic (M-) but not…

Mesoscale and Nanoscale Physics · Physics 2021-01-01 Yuecong Hu , Shaochuang Chen , Daqi Zhang , Xin Cong , Sida Sun , Jiangbin Wu , Feng Yang , Juan Yang , Ping-heng Tan , Yan Li

We present a high sensitivity single-monochromator Raman spectrometer which allows operation with a tunable laser source. The instrument is based on the modification of a commercial Raman spectrometer; such instruments operate with…

Materials Science · Physics 2011-07-08 Gábor Fábián , Christian Kramberger , Alexander Friedrich , Ferenc Simon , Thomas Pichler

Raman spectroscopy reveals chemically specific information and provides label-free insight into the molecular world. However, the signals are intrinsically weak and call for enhancement techniques. Here, we demonstrate Purcell enhancement…

We experimentally quantify the Raman scattering from individual carbyne chains confined in double-walled carbon nanotubes. We find that the resonant differential Raman cross section of confined carbyne is on the order of $10^{-22}$…

Mesoscale and Nanoscale Physics · Physics 2020-08-18 Cla Duri Tschannen , Georgy Gordeev , Stephanie Reich , Lei Shi , Thomas Pichler , Martin Frimmer , Lukas Novotny , Sebastian Heeg

The dipole-dipole interactions between excitons are of paramount importance in the nanoscale structures. When two excitons are placed together they can exchange the energy can manifest in the resonant Raman cross sections. We provide…

Mesoscale and Nanoscale Physics · Physics 2024-04-09 Anna Wroblewska , Niclas S. Mueller , Mariusz Zdrojek , Stephanie Reich , Georgy Gordeev

Quantum electrodynamics theory of the resonance Raman scattering is developed for an atom in a close proximity to a carbon nanotube. The theory predicts a dramatic enhancement of the Raman intensity in the strong atomic coupling regime to…

Mesoscale and Nanoscale Physics · Physics 2015-12-07 I. V. Bondarev

With the empirical bond polarizability model, the nonresonant Raman spectra of the chiral and achiral single-wall carbon nanotubes (SWCNTs) under uniaxial and torsional strains have been systematically studied by \textit{ab initio} method.…

Mesoscale and Nanoscale Physics · Physics 2007-07-31 Gang Wu , Jian Zhou , Jinming Dong

We present a systematic theoretical study of the Raman scattering effect for a two-level atomic system in near proximity of an ultrathin dielectric film with an embedded parallel array of periodically aligned single-wall semiconducting…

Mesoscale and Nanoscale Physics · Physics 2026-04-21 SK Firoz Islam , Michael Dean Pugh , Igor V. Bondarev

Electron scattering rates in metallic single-walled carbon nanotubes are studied using an atomic force microscope as an electrical probe. From the scaling of the resistance of the same nanotube with length in the low and high bias regimes,…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Ji-Yong Park , Sami Rosenblatt , Yuval Yaish , Vera Sazonova , Hande Ustunel , Stephan Braig , T. A. Arias , Piet W. Brouwer , Paul L. McEuen

Resonant Raman scattering of degenerate interacting two-channel quantum wire is studied. {\it All} collective excitations of two-channel quantum wire are shown to give rise to peaks in the polarized Raman spectra near resonance. If there…

Strongly Correlated Electrons · Physics 2009-11-07 Hyun C. Lee

In this work we investigate the role of exciton resonances in coherent anti-Stokes Raman scattering (er-CARS) in single walled carbon nanotubes (SWCNTs). We drive the nanotube system in simultaneous phonon and excitonic resonances, where we…

Mesoscale and Nanoscale Physics · Physics 2023-11-06 Georgy Gordeev , Lucas Lafeta , Benjamin Scott Flavel , Ado Jorio , Leandro M. Malard

Raman spectroscopy is used to probe the structure and electronic properties of nanotubes dispersed in a liquid phase. We show that the radial breathing modes are upshifted in suspensions due to the molecular pressure of the solvent. On the…

Other Condensed Matter · Physics 2016-08-16 Nicolas Izard , Alain Pénicaud , Eric Anglaret

A suspended carbon nanotube can act as a nanoscale resonator with remarkable electromechanical properties and the ability to detect adsorption on its surface at the level of single atoms. Understanding adsorption on nanotubes and other…

Mesoscale and Nanoscale Physics · Physics 2012-09-05 Zenghui Wang , Jiang Wei , Peter Morse , J. Gregory Dash , Oscar E. Vilches , David H. Cobden

Low-frequency Raman scattering experiments have been performed on thin films consisting of nickel-silver composite nanoparticles embedded in alumina matrix. It is observed that the Raman scattering by the quadrupolar modes, strongly…

Condensed Matter · Physics 2007-05-23 H. Portales , L. Saviot , E. Duval , M. Gaudry , E. Cottancin , M. Pellarin , J. Lerme , M. Broyer

Resonant Raman scattering is investigated in monolayer WS$_2$ at low temperature with the aid of an unconventional spectroscopy technique, $i.e.$, Raman scattering excitation (RSE). The RSE spectrum is made up by sweeping the excitation…

Mesoscale and Nanoscale Physics · Physics 2017-07-13 Maciej R. Molas , Karol Nogajewski , Marek Potemski , Adam Babinski

We exploit the near field enhancement of nano-antennas to investigate the Raman spectra of otherwise not optically detectable carbon nanotubes (CNTs). We demonstrate that a top-down fabrication approach is particularly promising when…

Mesoscale and Nanoscale Physics · Physics 2015-07-01 Nicola Paradiso , Fatemeh Yaghobian , Christoph Lange , Tobias Korn , Christian Schüller , Rupert Huber , Christoph Strunk

The interest of micro and tip-enhanced Raman spectroscopy to analyze nanosized and nanostructured materials, chiefly semiconductors, oxides and pristine or functionalized carbon nanotubes, is reviewed at the light of the contributions to…

Materials Science · Physics 2007-06-07 Philippe Colomban , Gwénael Gouadec

We explain quantitatively why resonant Raman scattering spectroscopy, an extensively used experimental tool in studying elementary electronic excitations in doped low dimensional semiconductor nanostructures, always produces an observable…

Strongly Correlated Electrons · Physics 2009-10-31 S. Das Sarma , Daw-Wei Wang
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