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We develop a new theory for associating fluids with multiple association sites. The theory accounts for small bond angle effects such as steric hindrance, ring formation and double bonding. The theory is validated against monte carlo…

Soft Condensed Matter · Physics 2013-08-19 B. D. Marshall , W. G. Chapman

While the realistically modeling of the thermodynamic behavior of fluids usually demands elaborated atomistic models, much have been learned from simplified ones. Here, we investigate a model where point-like particles (with activity $z_0$)…

Soft Condensed Matter · Physics 2019-07-15 Nathann T. Rodrigues , Tiago J. Oliveira

Micrometre sized colloidal particles can be viewed as large atoms with tailorable size, shape and interactions. These building blocks can assemble into extremely rich structures and phases, in which the thermal motions of particles can be…

Soft Condensed Matter · Physics 2017-11-10 Bo Li , Di Zhou , Yilong Han

Inverse patchy colloids are nano- to micro-scale particles with a surface divided into differently charged regions. This class of colloids combines directional, selective bonding with a relatively simple particle design: owing to the…

Soft Condensed Matter · Physics 2021-01-22 Emanuela Bianchi , Peter D. J. van Oostrum , Christos N. Likos , Gerhard Kahl

We report a computer-simulation study of the equilibrium phase diagram of a three-dimensional system of particles with a repulsive step potential. Using free-energy calculations, we have determined the equilibrium phase diagram of this…

Soft Condensed Matter · Physics 2009-11-13 Yu. D. Fomin , Daan Frenkel , N. V. Gribova , V. N. Ryzhov , S. M. Stishov

We study a model in which particles interact with short-ranged attractive and long-ranged repulsive interactions, in an attempt to model the equilibrium cluster phase recently discovered in sterically stabilized colloidal systems in the…

Soft Condensed Matter · Physics 2009-11-10 Francesco Sciortino , Stefano Mossa , Emanuela Zaccarelli , Piero Tartaglia

Phase separation, i.e., the coexistence of two different phases, is observed in many systems away from the coexistence curve of a first-order transition, leading to a stable heterogeneous phase or region. Examples include various quantum…

Strongly Correlated Electrons · Physics 2016-04-27 T. R. Kirkpatrick , D. Belitz

We investigate the ground state of the two-dimensional polarized Fermi gas with spin-orbit coupling and construct the phase diagram at zero temperature. We find there exist phase separation when the binding energy is low. As the binding…

Quantum Gases · Physics 2012-02-27 Xiaosen Yang , Shaolong Wan

We study analytically the structural properties of a system with a short-range attraction and a competing long-range screened repulsion. This model contains the essential features of the effective interaction potential among charged…

Soft Condensed Matter · Physics 2009-11-11 M. Tarzia , A. Coniglio

We study the phase behaviour of a fluid composed of particles which interact via a pair potential that is repulsive for large inter-particle distances, is attractive at intermediate distances and is strongly repulsive at short distances…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer , C. Ionescu , D. Pini , L. Reatto

We critically discuss the application of the Wertheim's theory to classes of complex associating fluids that can be today engineered in the laboratory as patchy colloids and to the prediction of their peculiar gas-liquid phase diagrams. Our…

Soft Condensed Matter · Physics 2016-01-06 Riccardo Fantoni , Giorgio Pastore

We deeply investigate a simple model representative of the recently synthesized Janus particles, i.e. colloidal spherical particles whose surface is divided into two areas of different chemical composition. When the two surfaces are…

Soft Condensed Matter · Physics 2009-12-21 Francesco Sciortino , Achille Giacometti , Giorgio Pastore

In this paper, we develop a thermodynamic perturbation theory to describe the self-assembly of patchy colloids which exhibit both patch-patch attractions as well as patch / non-patch attractions. That is, patches attract other patches as…

Soft Condensed Matter · Physics 2017-09-14 Bennett D. Marshall

Using self-consistent field and density-functional theories, we first investigate colloidal self-assembling of colloid/polymer films confined between two soft surfaces grafted by polymers. With the increase of colloidal concentrations, the…

Soft Condensed Matter · Physics 2007-05-23 Chun-lai Ren , Yu-qiang Ma

Patchy particles are a class of colloids with functionalized surfaces. Through surface functionalization, the strength and directionality of the colloidal interactions are tunable allowing control over coordination of the particle.…

Soft Condensed Matter · Physics 2013-10-21 Cristóvão Dias , Nuno Araújo , Margarida Telo da Gama

A simulation model is presented, comprising elastic spheres with a short range attraction. Besides conservative forces, radial- and shear friction, and radial noise are added. The model can be used to simulate colloids, granular solids and…

Soft Condensed Matter · Physics 2008-11-19 Robert D. Groot , Simeon D. Stoyanov

Motivated by the idea that intrinsically disordered proteins (IDPs) condense into liquid-like droplets within cells, we carry out Monte Carlo simulations of a polymer lattice model to study the relationship between charge patterning and…

Soft Condensed Matter · Physics 2019-12-11 Nicholas A. S. Robichaud , Ivan Saika-Voivod , Stefan Wallin

The behaviour of two-dimensional patchy particles with 5 and 7 regularly-arranged patches is investigated by computer simulation. For higher pressures and wider patch widths, hexagonal crystals have the lowest enthalpy, whereas at lower…

Soft Condensed Matter · Physics 2012-03-22 Marjolein N. van der Linden , Jonathan P. K. Doye , Ard A. Louis

The global phase behavior of the lattice restricted primitive model with nearest neighbor exclusion has been studied by grand canonical Monte Carlo simulations. The phase diagram is dominated by a fluid (or charge-disordered solid) to…

Soft Condensed Matter · Physics 2009-11-11 Alexandre Diehl , Athanassios Z. Panagiotopoulos

Mean-field calculations for the two dimensional electron gas (2DEG) in a large magnetic field with a partially filled Landau level with index $N\geq 2$ consistently yield ``stripe-ordered'' charge-density wave ground-states, for much the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Eduardo Fradkin , Steven A. Kivelson