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The electronic structure of the $(2\sqrt{2}\times\sqrt{2})R45^{\circ}$ O/Cu(001) system has been calculated using locally self-consistent, real space multiple scattering technique based on first principles. Oxygen atoms are found to perturb…

Materials Science · Physics 2009-11-07 S. Stolbov , T. S. Rahman

Representing polyether-salt systems by chains of interacting coordination shells, defined by the cation and by its nearest ligands, we derive the interaction potential between closest shells -- the inter-shells potential -- in terms of…

chem-ph · Physics 2009-10-28 L. D. Carlos , A. L. L. Videira

Electron-electron correlation forms the basis of difficulties encountered in many-body problems. Accurate treatment of the correlation problem is likely to unravel some nice physical properties of matter embedded in this correlation. In an…

Quantum Physics · Physics 2022-03-24 Eric Ouma Jobunga

Energies of a certain class of fullerene molecules (elongated, contracted, and regular icosahedral fullerenes) are numerically calculated using a microscopic description of carbon-carbon bonding. It is shown how these results can be…

Soft Condensed Matter · Physics 2009-11-11 Antonio Siber

A new model with a new Hamiltonian is offered as the means for studying properties of a system of strongly correlated electrons. Consideration of the simplest possible situation, namely a system on non-interacting electrons in a two-leg…

General Physics · Physics 2018-01-30 Valentin Voroshilov

We use variational quantum Monte Carlo to calculate the density-functional exchange-correlation hole n_{xc}, the exchange-correlation energy density e_{xc}, and the total exchange-correlation energy E_{xc}, of several electron gas systems…

Materials Science · Physics 2009-10-31 Maziar Nekovee , W. M. C. Foulkes , R. J. Needs

We explore several random phase approximation (RPA) correlation energy variants within the adiabatic-connection fluctuation-dissipation theorem approach. These variants differ in the way the exchange interactions are treated. One of these…

Chemical Physics · Physics 2014-04-08 János G. Angyán , Ru-Fen Liu , Julien Toulouse , Georg Jansen

A general formalism is used to express the long-range potential energies in inverse powers of the separation distance between two like atomic or molecular systems with $P$ symmetries. The long-range molecular interaction coefficients are…

Atomic Physics · Physics 2007-08-01 J. -Y. Zhang , Z. -C. Yan , D. Vrinceanu , J. F. Babb , H. R. Sadeghpour

Certain classes of strongly correlated systems promise high thermopower efficiency, but a full understanding of correlation effects on the Seebeck coefficient is lacking. This is partly due to limitations of Boltzmann-type approaches. One…

Strongly Correlated Electrons · Physics 2020-12-15 R. Nourafkan , A. -M. S. Tremblay

Electron correlation effects are essential for an accurate ab initio description of molecules. A quantitative a priori knowledge of the single- or multi-reference nature of electronic structures as well as of the dominant contributions to…

Quantum Physics · Physics 2012-12-18 Katharina Boguslawski , Paweł Tecmer , Örs Legeza , Markus Reiher

We calculate the `exact' potential corresponding to a one-dimensional interacting system of two electrons with a specific, tailored density. We use one-dimensional density-functional theory with a local-density approximation (LDA) on the…

Other Condensed Matter · Physics 2015-05-13 J. P. Coe , I. D'Amico

The dynamic response of an interacting electron system is determined by an extension of the relaxation-time approximation forced to obey local conservation laws for number, momentum and energy. A consequence of these imposed constraints is…

Strongly Correlated Electrons · Physics 2009-11-07 G. S. Atwal , N. W. Ashcroft

The exciton on a single polydiacetylene chain is considered in a Wannier approach, taking into account the surrounding polarizable medium. The electron-hole Coulomb interaction potential is explictly obtained for a quantum wire of circular…

Strongly Correlated Electrons · Physics 2007-05-23 Francois Dubin , Michel Schott

We have calculated the correlation energy of the homogeneous electron gas (HEG) and the dissociation energy curves of molecules with covalent bonds from a novel implementation of the adiabatic connection fluctuation dissipation (ACFD)…

Strongly Correlated Electrons · Physics 2015-06-22 Nicola Colonna , Maria Hellgren , Stefano de Gironcoli

The effect of the exchange-correlation potential in ab initio electron transport calculations is investigated by constructing optimized effective potentials (OEP) using different energy functionals or the electron density from second-order…

Mesoscale and Nanoscale Physics · Physics 2009-08-23 San-Huang Ke , Harold U. Baranger , Weitao Yang

Theoretical descriptions of the spectrum of electronic excitations in real metals have not yet reached a fully predictive, "first-principles" stage. In this paper we begin by presenting brief highlights of recent progress made in the…

Materials Science · Physics 2007-05-23 Adolfo G. Eguiluz , Wolf-Dieter Schoene

Considering the interactions of two arbitrary particles, we obtain an internal energy expression of the complex system having long-range interactions. Based on the postulate of "equal-probability principle" for all microstates, the…

Statistical Mechanics · Physics 2017-01-19 Yanxiu Liu , Cheng Xu , Zhifu Huang , Bihong Lin , Jincan Chen

Motivated by recent suggestions --to split the electron-electron interaction into a short-range part, to be treated within the density functional theory, and a long-range part, to be handled by other techniques-- we compute, with a…

Materials Science · Physics 2009-11-10 Lorenzo Zecca , Paola Gori-Giorgi , Saverio Moroni , Giovanni B. Bachelet

A functional $E_{xc}[\rho(\r,\epsilon)]$ is presented, in which the exchange and correlation energy of an electron gas depends on the local density of occupied states. A simple local parametrization scheme is proposed, entirely from first…

Materials Science · Physics 2009-11-10 Jose M. Soler

The interaction energy of the two-dimensional electron system in the region of fractional quantum Hall effect is considered within the Chern-Simons composite fermion approach. In the limit when Coulomb interaction is very small comparing to…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 P. Sitko