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Mode-coupling theory (MCT) predicts arrest of colloids in terms of their volume fraction, and the range and depth of the interparticle attraction. We discuss how effective values of these parameters evolve under cluster aggregation. We…

Soft Condensed Matter · Physics 2009-11-10 K. Kroy , M. E. Cates , W. C. K. Poon

We numerically investigate the competition between phase separation and dynamical arrest in a colloidal system interacting via a short ranged attractive potential. Equilibrium fluid configurations are quenched at two different temperatures…

Soft Condensed Matter · Physics 2007-05-23 G. Foffi , C. De Michele , F. Sciortino , P. Tartaglia

Through Monte Carlo simulations and the Associating Lattice Gas Model, the phases of a two-dimensional fluid under hydrophilic confinement are evaluated. The model, in its unconfined version, reproduces the anomalous behavior of water…

We present some recent theory and simulation results addressing the phenomena of colloidal gelation at both high and low volume fractions, in the presence of short-range attractive interactions. We discuss the ability of mode-coupling…

Soft Condensed Matter · Physics 2009-11-10 M. E. Cates , M. Fuchs , K. Kroy , W. C. K. Poon , A. M. Puertas

We present further evidence that gelation is an arrested phase separation in attractive colloid-polymer mixtures, based on a method combining confocal microscopy experiments with numerical simulations recently established in {\bf Nature…

Soft Condensed Matter · Physics 2009-11-13 Emanuela Zaccarelli , Peter J. Lu , Fabio Ciulla , David. A. Weitz , Francesco Sciortino

We derive an extension of the mode coupling theory for the liquid-glass transition to a class of models of confined fluids, where the fluid particles evolve in a disordered array of interaction sites. We find that the corresponding…

Disordered Systems and Neural Networks · Physics 2007-05-23 V. Krakoviack

We introduce a simple spherical model whose structural properties are similar to the ones generated by models with directional interactions, by employing a binary mixture of large and small hard spheres, with a square-well attraction acting…

Disordered Systems and Neural Networks · Physics 2009-11-13 Emanuela Zaccarelli , Francesco Sciortino , Piero Tartaglia

We study -- using molecular dynamics simulations -- the temperature dependence of the dynamics in a dense short-ranged attractive colloidal glass to find evidence of the kinetic glass-glass transition predicted by the ideal Mode Coupling…

Disordered Systems and Neural Networks · Physics 2009-11-10 Emanuela Zaccarelli , Giuseppe Foffi , Francesco Sciortino , Piero Tartaglia

Patchy colloidal model with three and four equivalent patches, confined in the attractive random porous media, undergo re-entrant gas-liquid phase separation with the possibility for the liquid phase density to approach zero. This unusual…

Soft Condensed Matter · Physics 2022-05-11 Taras Hvozd , Yurij V. Kalyuzhnyi , Vojko Vlachy , Peter T. Cummings

We present mode-coupling theory (MCT) results for densely packed hard-sphere fluids confined between two parallel walls and compare them quantitatively to computer simulations. The numerical solution of MCT is calculated for the first time…

Soft Condensed Matter · Physics 2023-05-10 Gerhard Jung , Thomas Franosch

We report extensive numerical simulations in the {\it glass} region for a simple model of short-ranged attractive colloids, the square well model. We investigate the behavior of the density autocorrelation function and of the static…

Soft Condensed Matter · Physics 2009-11-10 Emanuela Zaccarelli , Francesco Sciortino , Piero Tartaglia

We report an extensive numerical study of a charged colloidal system with competing short-range depletion attraction and long-range electrostatic repulsion. By analizing the cluster properties, we identify two distinct regions in the phase…

Soft Condensed Matter · Physics 2009-03-18 Juan Carlos Fernandez Toledano , Francesco Sciortino , Emanuela Zaccarelli

We study a model in which particles interact with short-ranged attractive and long-ranged repulsive interactions, in an attempt to model the equilibrium cluster phase recently discovered in sterically stabilized colloidal systems in the…

Soft Condensed Matter · Physics 2009-11-10 Francesco Sciortino , Stefano Mossa , Emanuela Zaccarelli , Piero Tartaglia

We combine the hyper-netted chain approximation of liquid state theory with the mode-coupling theory of the glass transition to analyze the structure and dynamics of soft spheres interacting via harmonic repulsion. We determine the locus of…

Statistical Mechanics · Physics 2010-03-29 Ludovic Berthier , Elijah Flenner , Hugo Jacquin , Grzegorz Szamel

Simulations and Mode-Coupling Theory calculations, for a large range of the arm number $f$ and packing fraction $\eta$ have shown that the structural arrest and the dynamics of star polymers in a good solvent are extremely rich: the systems…

Soft Condensed Matter · Physics 2009-11-10 F. Lo Verso , L. Reatto , G. Foffi , P. Tartaglia , K. A. Dawson

We have developed a simulation model to describe particle adsorption to and desorption from liquid interfaces. Using this model we formulate a closed interfacial equation of state for repulsive elastic spheres. The effect of a long-range…

Soft Condensed Matter · Physics 2011-02-24 Robert D. Groot , Simeon D. Stoyanov

We report idealized mode-coupling theory results for the glass transition of ensembles of model fullerenes interacting via phenomenological two-body potentials. Transition lines are found for C60, C70 and C96 in the temperature-density…

Statistical Mechanics · Physics 2007-05-23 M. J. Greenall , Th. Voigtmann

We present molecular simulation data for viscosity, self-diffusivity, and the local structural ordering of (i) a hard-sphere fluid and (ii) a square-well fluid with short-range attractions. The latter fluid exhibits a region of dynamic…

Soft Condensed Matter · Physics 2007-09-06 William P. Krekelberg , Jeetain Mittal , Venkat Ganesan , Thomas M. Truskett

The kinetic glass transition in short-range attractive colloids is theoretically studied by time-convolutionless mode-coupling theory (TMCT). By numerical calculations, TMCT is shown to recover all the remarkable features predicted by the…

Disordered Systems and Neural Networks · Physics 2017-03-15 Takayuki Narumi , Michio Tokuyama

We compare glassy dynamics in two liquids that differ in the form of their interaction potentials. Both systems have the same repulsive interactions but one has also an attractive part in the potential. These two systems exhibit very…

Statistical Mechanics · Physics 2020-01-22 François P. Landes , Giulio Biroli , Olivier Dauchot , Andrea J. Liu , David R. Reichman