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We study the Stokes-Einstein (SE) and the Stokes-Einstein-Debye (SED) relations using molecular dynamics simulations of the extended simple point charge model of water. We find that both the SE and SED relations break down at low…

Statistical Mechanics · Physics 2007-06-01 Marco G. Mazza , Nicolas Giovambattista , H. Eugene Stanley , Francis W. Starr

We study the motion of a tracer particle injected in facilitated models which are used to model supercooled liquids in the vicinity of the glass transition. We consider the East model, FA1f model and a more general class of non-cooperative…

Statistical Mechanics · Physics 2015-06-16 Oriane Blondel , Cristina Toninelli

The theories of Brownian motion, the Debye rotational diffusion model, and hydrodynamics together provide us with the Stokes--Einstein--Debye (SED) relation between the rotational relaxation time of the $\ell$-th degree Legendre polynomials…

Soft Condensed Matter · Physics 2019-06-03 Takeshi Kawasaki , Kang Kim

It is widely believed that the breakdown of the Stokes-Einstein (SE) relation between the translational diffusivity and the shear viscosity in supercooled liquids is due to the development of dynamic heterogeneity i.e. the presence of both…

Statistical Mechanics · Physics 2015-06-12 Shiladitya Sengupta , Smarajit Karmakar

The Stokes-Einstein (SE) relation between the self-diffusion and shear viscosity coefficients operates in sufficiently dense liquids not too far from the liquid-solid phase transition. By considering four simple model systems with very…

Soft Condensed Matter · Physics 2021-10-27 Sergey Khrapak , Alexey Khrapak

Molecular dynamics simulations have been performed on TIP4P/2005 supercooled water to investigate the molecular diffusion and shear viscosity at various timescales and assess the Stokes-Einstein (SE) and Stokes-Einstein-Debye (SED)…

Soft Condensed Matter · Physics 2019-08-12 Takeshi Kawasaki , Kang Kim

The Stokes-Einstein (SE) relation is commonly regarded as being breakdown in supercooled water. However, this conclusion is drawn upon testing the validities of some variants of the SE relation rather than its original form, and it appears…

Soft Condensed Matter · Physics 2021-11-24 Gan Ren , Yanting Wang

The breakdown of the Stokes-Einstein (SE) relation between diffusivity and viscosity at low temperatures is considered to be one of the hallmarks of glassy dynamics in liquids. Theoretical analyses relate this breakdown with the presence of…

Statistical Mechanics · Physics 2015-06-12 Shiladitya Sengupta , Smarajit Karmakar , Chandan Dasgupta , Srikanth Sastry

In this Research Note the Zwanzig's formulation of the Stokes-Einstein (SE) relation for simple atomistic fluids is re-examined. It is shown that the value of the coefficient in SE relation depends on the ratio of the transverse and…

Soft Condensed Matter · Physics 2020-04-22 Sergey Khrapak

The Stokes-Einstein (SE) relation has been widely applied to quantitatively describe the Brownian motion. Notwithstanding, here we show that even for a simple fluid, the SE relation may not be completely applicable. Namely, although the SE…

Statistical Mechanics · Physics 2021-03-17 Hanqing Zhao , Hong Zhao

Stokes-Einstein (SE) relation, which relates diffusion constant with the viscosity of a liquid at high temperatures in equilibrium, is violated in the supercooled temperature regime. Whether this relation is obeyed in nonequilibrium active…

Soft Condensed Matter · Physics 2023-06-21 Anoop Mutneja , Smarajit Karmakar

The Debye-Stokes-Einstein (DSE) model of rotational diffusion predicts that the rotational correlation times $\tau_{l}$ vary as $[l(l+1)]^{-1}$, where $l$ is the rank of the orientational correlation function (given in terms of the Legendre…

Soft Condensed Matter · Physics 2009-11-11 Prasanth P. Jose , Dwaipayan Chakrabarti , Biman Bagchi

The Stokes-Einstein-Debye (SED) relation is proposed to be breakdown in supercooled liquids by many studies. However, the conclusions are usually drawn by testing some variants of the SED relation rather than its original form. In this…

Soft Condensed Matter · Physics 2024-04-23 Gan Ren

Molecular Dynamics simulations of high density hard sphere fluids clearly show a breakdown of the Stokes-Einstein equation (SE). This result has been conjectured to be due to the presence of mobile particles, i.e., ones which have the…

Materials Science · Physics 2009-11-11 Sanat K. Kumar , Grzegorz Szamel , Jack F. Douglas

The Stokes-Einstein relation (SER) is one of the most robust and widely employed results from the theory of liquids. Yet sizable deviations can be observed for self-solvation, which cannot be explained by the standard hydrodynamic…

Statistical Mechanics · Physics 2018-06-15 Benoit Charbonneau , Patrick Charbonneau , Grzegorz Szamel

Motivated by the modeling of three-dimensional fluid turbulence, we define and study a class of stochastic partial differential equations (SPDEs) that are randomly stirred by a spatially smooth and uncorrelated in time forcing term. To…

Probability · Mathematics 2021-12-24 Gabriel B. Apolinário , Laurent Chevillard , Jean-Christophe Mourrat

One of hallmark features of glass forming ultraviscous liquids is the decoupling between translational and orientational dynamics. This report presents studies of this phenomenon in glycerol, a canonical molecular glass former, heading for…

The breakdown of the Stokes-Einstein (SE) law in fragile glassformers is examined by Molecular-Dynamics simulations of atomic liquids and polymers and consideration of the experimental data concerning the archetypical OTP glassformer. All…

Soft Condensed Matter · Physics 2018-05-09 F. Puosi , A. Pasturel , N. Jakse , D. Leporini

Hydrodynamic interactions are important for diverse fluids especially those with low Reynold's number such as microbial and particle-laden suspensions, and proteins diffusing in membranes. Unfortunately, while far-field (asymptotic)…

Soft Condensed Matter · Physics 2023-02-10 Noman Hanif Barbhuiya , A. G. Yodh , Chandan K. Mishra

The violation of Stokes--Einstein (SE) relation $D\sim (\eta/T)^{-1}$ between the shear viscosity $\eta$ and the translational diffusion constant $D$ at temperature $T$ is of great importance for characterizing anomalous dynamics of…

Soft Condensed Matter · Physics 2017-08-22 Takeshi Kawasaki , Kang Kim
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