Related papers: Frustration in Coupled Rattler System: KOs2O6
We use the density functional theory and lattice dynamics calculations to investigate the properties of potassium superoxide KO$_2$ in which spin, orbital, and lattice degrees of freedom are interrelated and determine the low-temperature…
Kagome materials are emerging platforms for studying charge and spin orders. In this work, we have revealed a rich lattice instability in a $\mathbb{Z}_2$ kagome metal ScV$_6$Sn$_6$ by first-principles calculations. Beyond verifying the…
Here we resolve the real-space nature of the high-temperature, short-range charge correlations in the kagome metal ScV$_6$Sn$_6$. Diffuse scattering appears along a frustrated wave vector $\textbf{q}_H=(\frac{1}{3},\frac{1}{3},\frac{1}{2})$…
We have applied ab initio molecular dynamics (MD) simulations to study metal-metal coupling on the alkali-metal sublattice in the {\beta}-pyrochlore osmates, AOs2O6 (A = K, Rb, Cs) at 300 K. We find that the alkali-metal atoms (rattlers)…
As an instance of geometrical frustration with non-magnetic degrees of freedom, we explore the physics of local spin $S\geq 1$ moments on the pyrochlore lattice that interact via pure quadrupolar couplings. In the presence of spin-orbit…
If magnetic frustration is most commonly known for undermining long-range order, as famously illustrated by spin liquids, the ability of matter to develop new collective mechanisms in order to fight frustration is no less fascinating,…
A wide variety of experimental results and theoretical investigations in recent years have convincingly demonstrated that several transition metal oxides and other materials, have dominant states that are not spatially homogeneous. This…
We propose and experimentally explore a method for realizing frustrated lattice models using a Bose-Einstein condensate held in an optical square lattice. A small lattice distortion opens up an energy gap such the lowest band splits into…
Pyrochlore systems ($A_{2}B_{2}O_{7}$) with $A$-site rare-earth local moments and $B$-site $5d$ conduction electrons offer excellent material platforms for the discovery of exotic quantum many-body ground states. Notable examples include…
Geometric frustration gives rise to vast manifolds of degenerate ground states and competing orders in spin and charge systems. Typically, classical ground states are governed by a local ``zero-sum constraint" that relieves frustrated…
The intertwined charge, spin, orbital, and lattice degrees of freedom could endow 5d compounds with exotic properties. Current interest is focused on electromagnetic interactions in these materials, whereas the important role of lattice…
We study the phase diagram of a topological string-net type lattice model in the presence of geometrically frustrated interactions. These interactions drive several phase transitions that reduce the topological order, leading to a rich…
Noise-enhanced chaos in a doped, weakly coupled GaAs/Al_{0.45}Ga_{0.55}As superlattice has been observed at room temperature in experiments as well as in the results of the simulation of nonlinear transport based on a discrete tunneling…
Rattling dynamics have been identified as fundamental to superconductivity in defect pyrochlore osmates and aluminium vanadium intermetallics, as well as low thermal conductivity in clathrates and filled skutterudites. Combining inelastic…
We explore the magnetic phases in a Kondo lattice model on the geometrically frustrated Shastry-Sutherland lattice at metallic electron densities, searching for noncollinear and noncoplanar spin textures. Motivated by experimental…
We use rigorous group-theoretic techniques and molecular dynamics to investigate the connection between structural symmetry and ionic conductivity in the garnet family of solid Li-ion electrolytes. We identify new ordered phases and…
Orthorhombic pseudobrookites CoTi$_2$O$_5$ and FeTi$_2$O$_5$ have a low-symmetry crystal structure comprising magnetic Co$^{2+}$/Fe$^{2+}$ ions and nonmagnetic Ti$^{4+}$ ions, where the orbital-nondegenerate Co$^{2+}$/Fe$^{2+}$ ions form…
The electron-phonon interaction is of central importance for the electrical and thermal properties of solids, and its influence on superconductivity, colossal magnetoresistance, and other many-body phenomena in correlated-electron materials…
Active systems are comprised of constituents with interactions that are generically non-reciprocal in nature. Such non-reciprocity often gives rise to situations where conflicting objectives exist, such as in the case of a predator pursuing…
Generally, one has two strategies to achieve magnetic frustration: through geometric means or interactions with different length scales. As the former leads to much simpler theoretical treatments it is favored and so magnetic sublattices…