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Phase equilibria between regions of different thickness in thin liquid films stabilized by colloidal particles are investigated using a quasi-two-dimensional thermodynamic formalism. Appropriate equilibrium conditions for the film tension,…

Soft Condensed Matter · Physics 2009-11-11 J. Blawzdziewicz , E. Wajnryb

The dynamics of microphase separation and the orientation of lamellae in diblock copolymers is investigated in terms of a mean-field model. The formation of lamellar structures and their stable states are explored and it is shown that…

Soft Condensed Matter · Physics 2015-06-15 Vanessa Weith , Alexei Krekhov , Walter Zimmermann

Thin block copolymer films have attracted considerable academic attention because of their ability to self-assemble into various microstructures, many of which have potential technological applications. Despite the ongoing interest, little…

Soft Condensed Matter · Physics 2016-04-25 Bekele J. Gurmessa , Andrew B. Croll

Equilibration of polymer melts containing highly entangled long polymer chains in confinement or with free surfaces is a challenge for computer simulations. We approach this problem by first studying polymer melts based on the soft-sphere…

Soft Condensed Matter · Physics 2020-10-14 Hsiao-Ping Hsu , Kurt Kremer

In recent experiments, small, thick-walled vesicles with a narrow size distribution were formed from copolymers where the degree of polymerisation of the hydrophobic block, N_B, was significantly greater than that of the hydrophilic block,…

Soft Condensed Matter · Physics 2017-09-12 M. J. Greenall

According to the universality hypothesis, the phase behavior of different block copolymer melt models having fixed composition depends solely on two parameters: the invariant chain length $\bar{N}$ and the effective interaction parameter…

Soft Condensed Matter · Physics 2024-08-16 Artem Petrov , Hejin Huang , Alfredo Alexander-Katz

We present a generalized theory of microphase separation for charged-neutral diblock copolymer melt. Stability limit of the disordered phase for salt-free melt has been calculated using Random Phase Approximation (RPA) and self-consistent…

Soft Condensed Matter · Physics 2009-11-13 Rajeev Kumar , M. Muthukumar

We model a melt of monodisperse side-chain liquid crystalline polymers as a melt of comb copolymers in which the side groups are rod-coil diblock copolymers. We consider both excluded volume and Maier-Saupe interactions. The first acts…

Soft Condensed Matter · Physics 2007-05-23 Marcela Hernandez , Harry Westfahl Junior

A self consistent field theory for compressible polymer mixtures is developed by introducing elements of classical density functional theory into the framework of the Helfand theory. It is then applied to study free surfaces of binary (A,B)…

Condensed Matter · Physics 2009-10-28 F. Schmid

We study electronic properties of AA-stacked graphene bilayers. In the single-particle approximation such a system has one electron band and one hole band crossing the Fermi level. If the bilayer is undoped, the Fermi surfaces of these…

Strongly Correlated Electrons · Physics 2014-08-05 A. O. Sboychakov , A. V. Rozhkov , A. L. Rakhmanov , Franco Nori

We investigate the effects of chain flexibility on the self-assembly behavior of symmetric diblock copolymers (BCPs) when they are confined as a thin film between two surfaces. Employing worm-like chain (WLC) self-consistent field theory,…

Soft Condensed Matter · Physics 2023-08-07 Mingyang Chen , Yuguo Chen , Yanyan Zhu , Ying Jiang , David Andelman , Xingkun Man

In this paper we study a model describing a copolymer in a micro-emulsion. The copolymer consists of a random concatenation of hydrophobic and hydrophilic monomers, the micro-emulsion consists of large blocks of oil and water arranged in a…

Probability · Mathematics 2016-10-03 Frank den Hollander , Nicolas Pétrélis

We present numerical calculations of lamellar phases of di-block copolymers (BCP) confined between two surfaces, where the top surface is flat and the bottom one is corrugated. The corrugated substrate is assumed to have a single $q$-mode…

Soft Condensed Matter · Physics 2016-02-17 Xingkun Man , Jiuzhou Tang , Pan Zhou , Dadong Yan , David Andelman

The structure and chemistry of grain boundaries (GBs) are crucial in determining polycrystalline materials' properties. Faceting and solute segregation to minimize the GB energy is a commonly observed phenomenon. In this paper, a deposition…

Thin polymer films have attracted attention because of both their broad range of applications and of the fundamental questions they raise regarding the dynamic response of confined polymers. These films are unstable if the temperature is…

A phenomenological mean-field theory is used to investigate the properties of solvent-diluted di-block copolymers (BCP), in which the two BCP components (A and B) form a variety of phases that are diluted by a solvent (S). Using this…

Soft Condensed Matter · Physics 2014-04-22 Shai Cohen , David Andelman

The phase behavior of asymmetrically interacting ABC star triblock copolymer melts is investigated by the self-consistent field theory (SCFT). Motivated by the experimental systems, in this study, we focus on the systems in which the…

Soft Condensed Matter · Physics 2015-08-25 Kai Jiang , Juan Zhang , Qin Liang

The phase behavior of symmetric diblock copolymers under three-dimensional (3D) soft confinement is investigated using the self-consistent field theory. The soft confinement is realized in binary blends composed AB diblock copolymers and C…

Soft Condensed Matter · Physics 2024-08-28 Zhijuan He , Jin Huang , Kai Jiang , An-Chang Shi

Multilayer "ferromagnet-layered antiferromagnet" (Fe/Cr) structures frustrated due to the roughness of layer interfaces are studied by numerical modeling methods. The "thickness-roughness" phase diagrams for the case of thin ferromagnetic…

Materials Science · Physics 2016-08-31 V. D. Levchenko , A. I. Morosov , A. S. Sigov

The monograph summarizes the studies of the temperature limits for the existence of a supercooled liquid phase of the components of nanodisperse structures. Original in situ methods for studying supercooling during crystallization in…

Biological Physics · Physics 2024-09-24 S. V. Dukarov , S. I. Petrushenko , S. I. Bogatyrenko , V. M. Sukhov