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We present a density functional perturbation theory approach to estimate the transition temperature of the charge density wave transition of TiSe2. The softening of the phonon mode at the L-point where in TiSe2 a giant Kohn anomaly occurs,…

Materials Science · Physics 2015-12-02 Dinh Loc Duong , Marko Burghard , J. Christian Schoen

We employ an optical pump-probe technique to study coherent phonon oscillations in Ca$_2$RuO$_4$. We find that oscillation-amplitude of an $A_g$ symmetric phonon mode is strongly suppressed at 260 K, a putative transition point of orbital…

Strongly Correlated Electrons · Physics 2018-10-24 Min-Cheol Lee , Choong H. Kim , Inho Kwak , J. Kim , S. Yoon , Byung Cheol Park , Bumjoo Lee , F. Nakamura , C. Sow , Y. Maeno , T. W. Noh , K. W. Kim

We investigate with a microscopic model anharmonic K-cation oscillation observed by neutron experiments in beta-pyrochlore superconductor KOs2O6, which also shows a mysterious first-order structural transition at Tp=7.5 K. We have…

Superconductivity · Physics 2015-05-20 Kazumasa Hattori , Hirokazu Tsunetsugu

Zero-field muon-spin relaxation measurements of the frustrated triangular quantum magnet AgNiO2 are consistent with a model of charge disproportionation that has been advanced to explain the structural and magnetic properties of this…

Strongly Correlated Electrons · Physics 2009-11-13 T. Lancaster , S. J. Blundell , P. J. Baker , M. L. Brooks , W. Hayes , F. L. Pratt , R. Coldea , T. Soergel , M. Jansen

We performed a Raman scattering study of thin films of LiTi$_2$O$_4$ spinel oxide superconductor. We detected four out of five Raman active modes, with frequencies in good accordance with our first-principles calculations. Three T$_{2g}$…

Superconductivity · Physics 2017-09-13 D. Chen , Y. -L. Jia , T. -T. Zhang , Z. Fang , K. Jin , P. Richard , H. Ding

To understand emergent magnetic monopole dynamics in the spin ices Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$, it is necessary to investigate the mechanisms by which spins flip in these materials. Presently there are thought to be two…

Strongly Correlated Electrons · Physics 2017-04-05 M Ruminy , S Chi , S Calder , T Fennell

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

We have studied the influence of magnetic order on the optical phonons of the geometrically frustrated spinel ZnCr$_2$O$_4$ from first-principles. By mapping the first-principles phonon calculations onto a Heisenberg-like model, we…

Materials Science · Physics 2009-11-11 Craig J. Fennie , Karin M. Rabe

In metals in the vicinity of a polar transition, interactions between electrons and soft phonon modes remain to be determined. Here we explore the consequences of spin-orbit assisted electron-phonon coupling on the collective modes of such…

Strongly Correlated Electrons · Physics 2023-12-27 Abhishek Kumar , Premala Chandra , Pavel A. Volkov

In the orbitally ordered, quasi-one dimensional Heisenberg antiferromagnet KCuF3 the low-energy Eg and B1g phonon modes show an anomalous softening (25% and 13%) between room temperature and the characteristic temperature T_S = 50 K. In…

Strongly Correlated Electrons · Physics 2022-05-31 V. Gnezdilov , J. Deisenhofer , P. Lemmens , D. Wulferding , O. Afanasiev , P. Ghigna , A. Loidl , A. Yeremenko

The thermal conductivity of the antiferromagnet Nd$_2$CuO$_4$ was measured down to 50 mK. Using the spin-flop transition to switch on and off the acoustic Nd magnons, we can reliably separate the magnon and phonon contributions to heat…

Superconductivity · Physics 2009-11-11 S. Y. Li , Louis Taillefer , C. H. Wang , X. H. Chen

In order to explore the consequences of spin-orbit coupling on spin-phonon interactions in a set of chemically-similar mixed metal oxides, we measured the infrared vibrational properties of Co$_4B_2$O$_9$ ($B$ = Nb, Ta) as a function of…

Materials Science · Physics 2023-05-26 K. Park , J. Kim , S. Choi , S. Fan , C. Kim , D. G. Oh , N. Lee , S. -W. Cheong , V. Kiryukhin , Y. J. Choi , D. Vanderbilt , J. H. Lee , J. L. Musfeldt

Millimeter sized ThCr$_2$Si$_2$-type CeNi$_2$As$_2$ single crystal was synthesized by NaAs flux method and its physical properties were investigated by magnetization, transport and specific heat measurements. In contrast to the previously…

Strongly Correlated Electrons · Physics 2013-01-01 Yongkang Luo , Jinke Bao , Chenyi Shen , Jieke Han , Xiaojun Yang , Chen Lv , Yuke Li , Wenhe Jiao , Bingqi Si , Chunmu Feng , Jianhui Dai , Guanghan Cao , Zhu-an Xu

We investigated the infrared-active phonons in ferromagnetic Weyl semimetal Co3Sn3S3 using optical spectroscopy. Below the Curie temperature (T~175~K), we observed asymmetric Fano lineshapes of phonons peaks in the optical conductivities,…

Materials Science · Physics 2024-10-30 R. Yang , Y. -Y. Zhu , M. Steigleder , X. -G. Qiu , T. -T. Zhang , M. Dressel

The low field phase of the organic superconductor (TMTSF)2ClO4 is studied by muon spin rotation. The zero temperature limit of the magnetic penetration depth within the TMTSF layers is obtained to be lambda_{ab}(0) = 0.86(2) um. Temperature…

Superconductivity · Physics 2014-01-17 F. L. Pratt , T. Lancaster , S. J. Blundell , C. Baines

We report infrared and Raman spectroscopy results of the spin-1/2 quantum magnet TiOCl. Giant anomalies are found in the temperature dependence of the phonon spectrum, which hint to unusual coupling of the electronic degrees of freedom to…

Strongly Correlated Electrons · Physics 2022-06-08 P. Lemmens , K. Y. Choi , G. Caimi , L. Degiorgi , N. N. Kovaleva , A. Seidel , F. C. Chou

We report results on the electrodynamic response of $TiOCl$, a low-dimensional spin-1/2 quantum magnet that shows a spin gap formation for T$<T_{c1}$= 67 $K$. The Fano-like shape of a few selected infrared active phonons suggests an…

Strongly Correlated Electrons · Physics 2009-11-10 G. Caimi , L. Degiorgi , N. N. Kovaleva , P. Lemmens , F. C. Chou

Magneto-acoustic investigations of the frustrated triangular-lattice antiferromagnet Cs2CuCl4 were performed for the longitudinal modes c11 and c33 in magnetic fields along the a-axis. The temperature dependence of the sound velocity at…

Strongly Correlated Electrons · Physics 2016-09-21 P. T. Cong , L. Postulka , B. Wolf , N. van Well , F. Ritter , W. Assmus , C. Krellner , M. Lang

An antiferromagnetic transition is observed in single crystal EuRh2As2 at a high temperature T_N = 47 K compared to the ferromagnetic Weiss temperature theta = 12 K. We show that this is, surprisingly, consistent with mean field theory. A…

Strongly Correlated Electrons · Physics 2010-11-12 Yogesh Singh , Y. Lee , B. N. Harmon , D. C. Johnston

Spin-phonon interaction plays an important role in 2D magnetic materials and motivates the development of next-generation spin- and charge-dependent microelectronic devices. Understanding the spin-phonon interaction by tuning the growth…