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Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 Sahand Tabatabaei , Pritam Priyadarsi , Namanish Singh , Pardis Sahafi , Daniel Tay , Andrew Jordan , Raffi Budakian

The observed intermittent light emission from colloidal semiconductor nanocrystals has long been associated with Auger recombination assisted quenching. We test this view by observing transient emission dynamics of CdSe/CdS/ZnS…

Mesoscale and Nanoscale Physics · Physics 2010-02-23 Shamir Rosen , Osip Schwartz , Dan Oron

Three models of single colloidal quantum dot emission fluctuations (blinking) based on spectral diffusion were considered analytically and numerically. It was shown that the only one of them, namely the Frantsuzov and Marcus model…

Statistical Mechanics · Physics 2019-07-24 Vladislav K. Busov , Pavel A. Frantsuzov

We study the band-edge exciton fine structure and in particular its bright-dark splitting in colloidal semiconductor nanocrystals by four different optical methods based on fluorescence line narrowing and time-resolved measurements at…

Semiconductor nanocrystals are a promising class of materials for a variety of novel optoelectronic devices, since many of their properties, such as the electronic gap and conductivity, can be controlled. Much of this control is achieved…

Chemical Physics · Physics 2017-06-06 Nadav Geva , James J. Shepherd , Lea Nienhaus , Moungi G. Bawendi , Troy Van Voorhis

Intensity squeezing, i.e., photon number fluctuations below the shot noise limit, is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that the intensity squeezing could be…

We demonstrate a large light absorptance (80%) in a nanometric layer of quantum dots in rods (QRs) with a thickness of 23 nm. This behavior is explained in terms of the coherent absorption by interference of the light incident at a certain…

Inverted type-I heterostructure core/crown quantum rings (QRs) are quantum-efficient luminophores, whose spectral characteristics are highly tunable. Here, we study the optoelectronic properties of type-I core/crown CdS/CdSe QRs in the…

Mesoscale and Nanoscale Physics · Physics 2017-10-25 Sumanta Bose , Weijun Fan , Dao Hua Zhang

We present first-principles calculations on bulk CdSe and CdSe nanowires with diameters of up to 22 \AA. Density functional linear combination of atomic orbitals and plane wave calculations of the electronic and structural properties are…

Materials Science · Physics 2009-06-04 M. Mohr , C. Thomsen

Charge-current quasielastic (CCQE) (anti)neutrino scattering cross sections on a $^{12}$C target are analyzed using a spectral function $S(p,{\cal E})$ that gives a scaling function in accordance with the ($e,e'$) scattering data. The…

NV centers in diamond are generally recognized as highly promising as indefinitely stable highly efficient single-photon sources. We report an experimental quantification of the brightness, radiative decay rate, nonradiative decay rate and…

Optics · Physics 2015-06-12 Abbas Mohtashami , A. Femius Koenderink

Simulations and experiments of nanorods (NRs) show that co-assembly with block copolymer (BCP) melts leads to the formation of a superstructure of side-to-side NRs perpendicular to the lamellar axis. A mesoscopic model is validated against…

Soft Condensed Matter · Physics 2020-04-14 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga , Roy Shenhar

The ratios of inclusive electron scattering cross sections of $^4$He, $^{12}$C, and $^{56}$Fe to $^3$He have been measured for the first time. It is shown that these ratios are independent of $x_B$ at Q$^2>$1.4 (GeV/c)$^2$ for $x_B>$ 1.5…

Nuclear Experiment · Physics 2010-04-06 K. Sh Egiyan

A central question in the field of graphene-related research is how graphene behaves when it is patterned at the nanometer scale with different edge geometries. Perhaps the most fundamental shape relevant to this question is the graphene…

Energy transfer from photoexcited zero-dimensional systems to metallic systems plays a prominent role in modern day materials science. A situation of particular interest concerns the interaction between a photoexcited dipole and an…

Chemical Physics · Physics 2013-04-30 Zheyuan Chen , Stéphane Berciaud , Colin Nuckolls , Tony F. Heinz , Louis E. Brus

The utility of nanoscaled ferromagnetic particles requires both stabilized moments and maximized switching speeds. During reversal, the spatial modulation of the nanoparticle magnetization evolves in time, and the energy differences between…

We present a direct experimental evidence of photo-ionized CdTe quantum dot core having luminescence "off" state at band-edge photo-excitation. We use the autocorrelation of fluorescence fluctuations from dilute colloidal solution of CdTe…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 A. V. R. Murthy , Padmashri Patil , Shouvik Datta , Shivprasad Patil

In metallic nanoparticles, shifts in the ionization energy of surface atoms with respect to bulk atoms can lead to surface bands. Within a simple Tight Binding model we find that the projection of the electronic density of states on these…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. A. Gascon , H. M. Pastawski

Previous single-particle spectroscopic studies of colloidal quantum dots have indicated a significant spread in biexciton lifetimes across an ensemble of nominally identical nanocrystals. It has been speculated that in addition to…

Materials Science · Physics 2013-09-24 Young-Shin Park , Wan Ki Bae , Lazaro A. Padilha , Jeffrey M. Pietryga , Victor I. Klimov

Fluctuations affect nanoporous transport in complex and intricate ways, making optimization of signal-to-noise in artificial designs challenging. Here we focus on the simplest nanopore system, where non-interacting particles diffuse through…

Soft Condensed Matter · Physics 2021-05-19 Sophie Marbach