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Related papers: High-order Dy multipole motifs observed in DyB2C2 …

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Resonant soft x-ray Bragg diffraction at the Dy M$_{4,5}$ edges has been used to study Dy multipoles in the combined magnetic and orbitally ordered phase of DyB$_2$C$_2$. The analysis incorporates both the intra-atomic magnetic and…

Strongly Correlated Electrons · Physics 2015-03-19 A. J. Princep , A. M. Mulders , U. Staub , V. Scagnoli , T. Nakamura , A. Kikkawa , S. W. Lovesey , E. Balcar

Soft resonant x-ray Bragg diffraction (SRXD) at the Ho M$_{4,5}$ edges has been used to study Ho $4f$ multipoles in the combined magnetic and orbitally ordered phase of HoB$_2$C$_2$. A full description of the energy dependence for both…

Strongly Correlated Electrons · Physics 2015-06-03 A. J. Princep , A. M. Mulders , E. Schierle , E. Weschke , J. Hester , W. D. Hutchison , Y. Tanaka , N. Terada , Y. Narumi , T. Nakamura

The dependence with energy of the resonant soft x-ray Bragg diffraction intensity in DyB$_2$C$_2$ for the $(00{1/2})$ reflection at the Dy M$_{4,5}$ edges have been calculated by using an atomic multiplet hamiltonian including the effect of…

Strongly Correlated Electrons · Physics 2014-05-22 Javier Fernandez-Rodriguez , Alessandro Mirone , Urs Staub

Soft x-ray resonant scattering has been used to examine the charge and magnetic interactions in the cycloidal antiferromagnetic compound \dyfeal. By tuning to the Dy $M_4$ and $M_5$ absorption edges and the Fe L(2) and L(3) absorption edges…

Strongly Correlated Electrons · Physics 2007-05-23 T. A. W. Beale , S. B. Wilkins , P. D. Hatton , P. Abbamonte , S. Stanescu , J. A. Paixao

Resonant soft x-ray Bragg diffraction at the Tb M4,5 edges and non resonant Bragg diffraction have been used to investigate orbitals in TbB2C2. The Tb 4f quadrupole moments are ordered in zero field below T_N and show a ferroquadrupolar…

Strongly Correlated Electrons · Physics 2009-11-11 A. M. Mulders , U. Staub , V. Scagnoli , Y. Tanaka , A. Kikkawa , K. Katsumata , J. M. Tonnerre

By means of circularly polarized x-ray beam at Dy L3 and Fe K absorption edges, the chiral structure of the electric quadrupole was investigated for a single crystal of DyFe3(BO3)4 in which both Dy and Fe ions are arranged in spiral…

A recent polarized neutron diffraction experiment on the 5d2 rhenium double perovskite Ba2YReO6 held at a low temperature uncovered weak magnetic diffraction peaks. Data analysis inferred a significantly reduced Re dipole moment, and…

Strongly Correlated Electrons · Physics 2021-03-24 S. W. Lovesey , D. D. Khalyavin , G. van der Laan , G. J. Nilsen

Possible ways of identification are discussed of an electronic order of higher multipoles such as octupoles and hexadecapoles. A particularly powerful method is resonant X-ray scattering (RXS) using quadrupolar resonance processes called…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Kuramoto , H. Kusunose , A. Kiss

A theory that fully describes previously observed neutron Bragg spots indicative of magnetic order in the pseudo-gap phase of YBa2Cu3O6 + x is presented. Magnetic diffraction intensities, unveiled by polarization analysis, are explained by…

Strongly Correlated Electrons · Physics 2015-05-01 S. W. Lovesey , D. D. Khalyavin , U. Staub

Experimental evidence of the d-f Coulomb interaction responsible for the resonant x-ray scattering (RXS) from antiferroquadrupolar order in DyB2C2 is presented. The energy dependences of the RXS intensity with polarization analysis are…

Strongly Correlated Electrons · Physics 2009-11-10 T. Matsumura , D. Okuyama , N. Oumi , K. Hirota , H. Nakao , Y. Murakami , Y. Wakabayashi

We have used element specific X-ray resonant scattering to investigate the M edge resonances in a single crystal of \unpo. Earlier neutron diffraction and M\"{o}ssbauer studies had shown the presence of long-range AF order below T$_{N}$ =…

Strongly Correlated Electrons · Physics 2009-11-10 S. B. Wilkins , J. A. Paxiao , R. Caciuffo , P. Javorsky , F. Wastin , J. Rebizant , C. Detlefs , N. Bernhoeft , P. Santini , G. H. Lander

We submit that the magnetic space-group Cac (#9.41) is consistent with the established magnetic structure of BaFe2Se3, with magnetic dipole moments in a motif that uses two ladders [Caron J M et al 2011 Phys. Rev. B 84 180409(R)]. The…

Strongly Correlated Electrons · Physics 2014-12-09 S W Lovesey , D D Khalyavin

Structural and magnetic transitions in a double perovskite hosting 5d1 Re ions are discussed on the basis of recently published high-resolution x-ray diffraction patterns [D. Hirai, et al., Phys. Rev. Res. 2, 022063(R) (2020)]. A reported…

Strongly Correlated Electrons · Physics 2021-06-30 S. W. Lovesey , D. D. Khalyavin

Successive phase transitions in a rare-earth monoaxial chiral magnet DyNi$_3$Ga$_{9}$ have been investigated by resonant x-ray diffraction. Magnetic dipole and electric quadrupole degrees of freedom arising from the large angular moment of…

Strongly Correlated Electrons · Physics 2022-02-11 Mitsuru Tsukagoshi , Takeshi Matsumura , Shinji Michimura , Toshiya Inami , Shigeo Ohara

Magnetic axial and polar (Dirac) nickel multipoles contribute to resonant x-ray Bragg amplitudes in a symmetry informed analysis of monoclinic Li2Ni3P4O14 presented for future diffraction experiments. Magnetic long-range order below a…

Strongly Correlated Electrons · Physics 2025-08-08 Stephen W. Lovesey

We study the resonant x-ray scattering (RXS) spectra at the Dy $L_{\rm III}$ absorption edge in the quadrupole ordering phase of DyB$_2$C$_2$. Analyzing the buckling of sheets of B and C atoms, we construct an effective model that the…

Strongly Correlated Electrons · Physics 2009-11-10 Jun-ichi Igarashi , Tatsuya Nagao

Recently, quadrupole helix chirality and its domain structure was observed in resonant x-ray diffraction experiments on DyFe$_3$(BO$_3$)$_4$ using circularly polarized x rays [T. Usui et al., Nature Materials 13, 611 (2014)]. We show that…

Materials Science · Physics 2017-04-05 M. N. Popova , E. P. Chukalina , K. N. Boldyrev , T. N. Stanislavchuk , B. Z. Malkin , I. A. Gudim

A systematic analysis of resonant x-ray Bragg diffraction data for UPd$_3$, with signal enhancement at the U M$_{IV}$ edge, including possible structural phase-transitions leads to a new determination of the space groups of the material in…

Strongly Correlated Electrons · Physics 2014-05-22 Javier Fernandez-Rodriguez , Stephen W. Lovesey , Jesus A. Blanco

Magnetite, Fe$_3$O$_4$, displays a highly complex low temperature crystal structure that may be charge and orbitally ordered. Many of the recent experimental claims of such ordering rely on resonant soft x-ray diffraction at the oxygen K…

Strongly Correlated Electrons · Physics 2015-05-13 S. B. Wilkins , S. Di Matteo , T. A. W. Beale , Y. Joly , C. Mazzoli , P. D. Hatton , P. Bencok , F. Yakhou , V. A. M. Brabers

A minimal model for multipole orders in CeB$_6$ shows that degeneracy of the quadrupole order parameters and strong spin-orbit coupling lead to peculiar temperature and magnetic-field dependences of the X-ray reflection intensity at…

Strongly Correlated Electrons · Physics 2016-08-31 Hiroshi N. Kono , Katsunori Kubo , Yoshio Kuramoto
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