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Related papers: Spin dynamics in the low-dimensional magnet TiOCl

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We present electron spin resonance data of Ti$^{3+}$ (3$d^1$) ions in single crystals of the novel layered quantum spin magnet TiOCl. The analysis of the g tensor yields direct evidence that the d_{xy} orbital from the t_{2g} set is…

Strongly Correlated Electrons · Physics 2009-11-10 V. Kataev , J. Baier , A. Moeller , L. Jongen , G. Meyer , A. Freimuth

Measurements of the heat capacity C(T,H) of the one-dimensional quantum magnet TiOCl are presented for temperatures 2K < T < 300K and magnetic fields up to 5T. Distinct anomalies at 91K and 67K signal two subsequent phase transitions. The…

Strongly Correlated Electrons · Physics 2007-05-23 J. Hemberger , M. Hoinkis , M. Klemm , M. Sing , R. Claessen , S. Horn , A. Loidl

We explore spin dynamics in Cu(1,3-bdc), a quasi-2D topological magnon insulator. The results show that the thermal evolution of Land\'e $g$-factor ($g$) is anisotropic: $g_\textrm{in-plane}$ reduces while $g_\textrm{out-plane}$ increases…

The local magnetic properties of Yb$^{3+}$ in the layered honeycomb material YbCl$_{3}$ were investigated by electron spin resonance on single crystals. For in-plane and out-of-plane field orientations the $g$-factor shows a clear…

Strongly Correlated Electrons · Physics 2023-08-15 Jörg Sichelschmidt , Ellen Häußler , Ekaterina Vinokurova , M. Baenitz , Thomas Doert

We present an experimental study of macroscopic and microscopic magnetic anisotropy of a spin tetramer system \cso using torque magnetometry and ESR spectroscopy. Large rotation of macroscopic magnetic axes with temperature observed from…

Strongly Correlated Electrons · Physics 2016-08-08 Mirta Herak , Dijana Žilić , Dubravka Matković Čalogović , Helmuth Berger

In this work we present a study of the low temperature magnetic phases of polycrystalline MnCr$_2$O$_4$ spinel through dc magnetization and ferromagnetic resonance spectroscopy (FMR). Through these experiments we determined the main…

Materials Science · Physics 2014-12-03 Dina Tobia , Julián Milano , María Teresa Causa , Elin L. Winkler

In the layered quantum spin systems TiOCl and TiOBr the magnetic susceptibility shows a very weak temperature dependence at high temperatures and transition-induced phenomena at low temperatures. There is a clear connection of the observed…

Strongly Correlated Electrons · Physics 2010-03-09 P. Lemmens , K. Y. Choi , R. Valenti , T. Saha-Dasgupta , E. Abel , Y. S. Lee , F. C. Chou

We investigate the magnetic properties of the multiferroic quantum-spin system LiCu$_2$O$_2$ by electron spin resonance (ESR) measurements at $X$- and $Q$-band frequencies in a wide temperature range $(T_{\rm N1} \leq T \leq 300$\,K). The…

We combine high-resolution resonant inelastic x-ray scattering with cluster calculations utilizing a recently derived effective magnetic scattering operator to analyze the polarization, excitation energy, and momentum dependent excitation…

We present an experimental study of macroscopic and microscopic magnetic anisotropy of a spin tetramer system SeCuO$_3$ using torque magnetometry and ESR spectroscopy. Large rotation of macroscopic magnetic axes with temperature observed…

Strongly Correlated Electrons · Physics 2014-05-20 Mirta Herak , Antonija Grubišić Čabo , Dijana Žilić , Boris Rakvin , Krešimir Salamon , Ognjen Milat , Helmuth Berger

Multi-frequency electron spin resonance (ESR) transmission spectra have been measured as function of temperature and magnetic field on single crystals of the quasi-one-dimensional spin-1 chain compound SrNi2V2O8 in the GHz frequency range.…

Strongly Correlated Electrons · Physics 2013-03-18 Zhe Wang , M. Schmidt , A. K. Bera , A. T. M. N. Islam , B. Lake , A. Loidl , J. Deisenhofer

Temperature-dependent x-ray diffraction of the low-dimensional spin 1/2 quantum magnet TiOCl shows that the phase transition at T_{c2} = 90 K corresponds to a lowering of the lattice symmetry. Below T_{c1} = 66 K a twofold superstructure…

Materials Science · Physics 2009-11-11 M. Shaz , S. van Smaalen , L. Palatinus , M. Hoinkis , M. Klemm , S. Horn , R. Claessen

The low energy excitation spectrum of a two-dimensional ferromagnetic material is dominated by single-magnon excitations that show a gapless parabolic dispersion relation with the spin wave vector. This occurs as long as magnetic anisotropy…

Mesoscale and Nanoscale Physics · Physics 2023-10-25 F. Delgado , M. M. Otrokov , A. Arnau

The magnetic nature of low dimensional compound, CrCl$_3$, was investigated by muon spin rotation, relaxation and resonance ($\mu^+$SR). The $\mu^+$SR measurements revealed three distinct phases as a function of temperature: an…

Electronic structure calculations on the low dimensional spin-1/2 compound TiOCl were performed at several pressures in the orthorhombic phase, finding that the structure is quasi-one-dimensional. The Ti3+ (d1) ions have one t2g orbital…

Strongly Correlated Electrons · Physics 2010-12-15 A. Piñeiro , V. Pardo , D. Baldomir , S. Blanco-Canosa , F. Rivadulla , J. E. Arias , J. Rivas

We report a comprehensive high-field/high-frequency electron spin resonance (ESR) study on single crystals of the van der Waals magnet CrCl$_3$. This material, although being known for quite a while, has received recent significant…

Materials Science · Physics 2020-06-09 J. Zeisner , K. Mehlawat , A. Alfonsov , M. Roslova , T. Doert , A. Isaeva , B. Büchner , V. Kataev

We report results on the electrodynamic response of $TiOCl$, a low-dimensional spin-1/2 quantum magnet that shows a spin gap formation for T$<T_{c1}$= 67 $K$. The Fano-like shape of a few selected infrared active phonons suggests an…

Strongly Correlated Electrons · Physics 2009-11-10 G. Caimi , L. Degiorgi , N. N. Kovaleva , P. Lemmens , F. C. Chou

We present comprehensive electron spin resonance (ESR) studies of in-plane oriented single crystals of $\alpha$-RuCl$_3$, a quasi-two-dimensional material with honeycomb structure, focusing on its high-field spin dynamics. The measurements…

We study the magnetisation dynamics of a bulk single crystal Cr$_2$Ge$_2$Te$_6$ (CGT), by means of broadband ferromagnetic resonance (FMR), for temperatures from 60 K down to 2 K. We determine the Kittel relations of the fundamental FMR…

Materials Science · Physics 2019-11-05 S. Khan , C. W. Zollitsch , D. M. Arroo , H. Cheng , I. Verzhbitskiy , A. Sud , Y. P. Feng , G. Eda , H. Kurebayashi

Magnetic properties of high-quality Al-free nonsuperconducting GdBa_2Cu_3O_{6+y} single crystals grown by flux method have been studied. The magnetic anisotropy below the N\'eel temperature T_N~2.3K corresponds to the direction of Gd^{3+}…

Materials Science · Physics 2016-08-31 V. N. Narozhnyi , D. Eckert , G. Fuchs , V. Nekvasil , K. -H. Müller
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