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KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

Strongly Correlated Electrons · Physics 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

Magnetization maesurements under hydrostatic pressure were performed on an S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic field H parallel to the [2,0,1] direction. With increasing applied pressure P, the gap…

Statistical Mechanics · Physics 2009-11-10 Kenji Goto , Masashi Fujisawa , Toshio Ono , Hidekazu Tanaka , Yoshiya Uwatoko

Magnetic phase transition under hydrostatic pressure in TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ was investigated by magnetization measurements. The parent compound TlCuCl$_3$ is a coupled spin dimer system, which undergoes a pressure-induced…

Strongly Correlated Electrons · Physics 2009-11-11 H. Imamura , T. Ono , K. Goto , H. Tanaka

We carried out zero-field muon-spin-rotation (ZF-$\mu$SR) measurements in hydrostatic pressures in impurity-doped quantum spin gap system Tl(Cu$_{0.985}$Mg$_{0.015}$)Cl$_3$ to investigate microscopic magnetic properties of the…

Strongly Correlated Electrons · Physics 2015-05-18 Takao Suzuki , Isao Watanabe , Fumiko Yamada , Motoki Yamada , Yasuyuki Ishii , Takayuki Kawamata , Takayuki Goto , Hidekazu Tanaka

Under the hydrostatic pressure $P=1.48$ GPa, polarized neutron elastic scattering experiments have been carried out on the coupled spin dimer system TlCuCl$_3$ with the gapped ground state at ambient pressure. Pressure-induced magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , K. Kakurai , T. Osakabe , M. Nakamura , M. Takeda , H. Tanaka

Magnetization measurements under a hydrostatic pressure of P = 1.4 GPa were performed on the coupled spin dimer system TlCuCl_3, which exhibits a pressure-induced quantum phase transition from a gapped singlet state to an antiferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-13 Fumiko Yamada , Yasuyuki Ishii , Takao Suzuki , Teiichiro Matsuzaki , Hidekazu Tanaka

Inelastic neutron scattering and bulk magnetic susceptibility studies of the quantum S=1/2 spin ladder system IPA-CuCl3 are performed under hydrostatic pressure. The pressure dependence of the spin gap $\Delta$ is determined. At $P=1.5$ GPa…

Strongly Correlated Electrons · Physics 2008-12-10 Tao Hong , V. O. Garlea , A. Zheludev , J. Fernandez-Baca , H. Manaka , S. Chang , J. B. Leao , S. J. Poulton

We have performed magnetization measurements of the gapped quantum magnet CsFeCl$_3$ at temperatures ($T$) down to 0.5\,K at ambient pressure and down to 1.8\,K at hydrostatic pressures ($P$) of up to 1.5\,GPa. The lower-field ($H$) phase…

Strongly Correlated Electrons · Physics 2016-09-28 Nobuyuki Kurita , Hidekazu Tanaka

Magnetic phase transitions under hydrostatic pressures in spin gap systems TlCu$_{0.988}$Mg$_{0.012}$Cl$_3$ and KCu$_{0.973}$Mg$_{0.027}$Cl$_3$ were investigated by magnetization measurements. The present doped systems exhibit…

Strongly Correlated Electrons · Physics 2015-06-25 T. Ono , H. Imamura , J. Kawakami , K. Goto , H. Tanaka

Magnetization measurements were performed on TlCuCl$_3$ with gapped ground state. The critical density and the magnetic phase diagram were obtained. The interacting constant was obtained as $U/k_{\rm B} = 313$ K. The experimental phase…

Strongly Correlated Electrons · Physics 2015-06-25 F. Yamada , T. Ono , M. Fujisawa , H. Tanaka , T. Sakakibara

Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…

Strongly Correlated Electrons · Physics 2017-12-18 Hyeong-Jin Kim , C. R. S. Haines , C. Liu , Sae Hwan Chun , Kee Hoon Kim , H. T. Yi , Sang-Wook Cheong , Siddharth S. Saxena

Neutron elastic scattering measurements have been performed under the hydrostatic pressure in order to investigate the spin structure of the pressure-induced magnetic ordering in the spin gap system TlCuCl$_3$. Below the ordering…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , M. Fujisawa , T. Osakabe , K. Kakurai , H. Tanaka

KCuCl$_3$ is a three-dimensional coupled spin-dimer system and has a singlet ground state with an excitation gap ${\Delta}/k_{\rm B}=31$ K. High-field magnetization measurements for KCuCl$_3$ have been performed in static magnetic fields of…

Strongly Correlated Electrons · Physics 2009-11-07 A. Oosawa , T. Takamasu , K. Tatani , H. Abe , N. Tsujii , O. Suzuki , H. Tanaka , G. Kido , K. Kindo

Single-crystal neutron inelastic scattering was performed in order to investigate the magnetic excitations in the spin gap system TlCuCl$_3$. The constant-${\bf Q}$ energy scan profiles were collected in the $a^*-c^*$ plane. Three…

Condensed Matter · Physics 2007-05-23 A. Oosawa , T. Kato , H. Tanaka , H. Uekusa , Y. Ohashi , K. Nakajima , M. Nishi , K. Kakurai

Thallium copper chloride is a quantum spin liquid of S = 1/2 Cu^2+ dimers. Interdimer superexchange interactions give a three-dimensional magnon dispersion and a spin gap significantly smaller than the dimer coupling. This gap is closed by…

Strongly Correlated Electrons · Physics 2009-11-10 M. Matsumoto , B. Normand , T. M. Rice , M. Sigrist

We report muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements on Cu(Cl,Br)La(Nb,Ta)$_{2}$O$_{7}$, which demonstrate: (a) the absence of static magnetism in (CuCl)LaNb$_{2}$O$_{7}$ down to 15 mK confirming a spin-gapped…

Quantum triangular-lattice antiferromagnets are important prototype systems to investigate phenomena of the geometrical frustration in condensed matter. Apart from highly unusual magnetic properties, they possess a rich phase diagram…

Strongly Correlated Electrons · Physics 2019-03-13 S. A. Zvyagin , D. Graf , T. Sakurai , S. Kimura , H. Nojiri , J. Wosnitza , H. Ohta , T. Ono , H. Tanaka

The insulating ferrimagnet Cu2OSeO3 shows a rich variety of phases such as skyrmion lattice and helical magnetism controlled by interplay of different exchange interactions which can be tuned by external pressure. In this work we have…

For magnets with a fully frustrated inter-layer interaction, we argue that the quantum phase transitions from a paramagnetic to an antiferromagnetic ground state, driven by pressure or magnetic field, are asymptotically three-dimensional,…

Strongly Correlated Electrons · Physics 2007-11-08 Oliver Rösch , Matthias Vojta

We present high-resolution measurements of the thermal expansion and the magnetostriction of TlCuCl$_{3}$ which shows field-induced antiferromagnetic order. We find pronounced anomalies in the field and temperature dependence of different…

Strongly Correlated Electrons · Physics 2009-11-10 N. Johannsen , A. Vasiliev , A. Oosawa , H. Tanaka , T. Lorenz
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