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New Raman and incoherent neutron scattering data at various temperatures and molecular dynamic simulations in amorphous silica, are compared to obtain the Raman coupling coefficient $C(\omega)$ and, in particular, its low frequency limit.…

Disordered Systems and Neural Networks · Physics 2009-10-31 A. Fontana , R. Dell'Anna , M. Montagna , F. Rossi , G. Viliani , G. Ruocco , M. Sampoli , U. Buchenau , A. Wischnewski

Low-frequency Raman coupling coefficient of 11 different glasses is evaluated. It is found that the coupling coefficient demonstrates a universal linear frequency behavior near the boson peak maximum and a superlinear behavior at very low…

Materials Science · Physics 2009-11-07 N. V. Surovtsev , A. P. Sokolov

The effects of plasticization of poly(methyl methacrylate) glass on the boson peaks observed by Raman and neutron scattering are compared. In plasticized glass the cohesion heterogeneities are responsible for the neutron boson peak and…

Condensed Matter · Physics 2007-05-23 E. Duval , L. Saviot , A. Mermet , L. David , S. Etienne , V. Bershtein , A. J. Dianoux

We show that a {\em vibrational instability} of the spectrum of weakly interacting quasi-local harmonic modes creates the maximum in the inelastic scattering intensity in glasses, the Boson peak. The instability, limited by anharmonicity,…

Disordered Systems and Neural Networks · Physics 2009-11-07 V. L. Gurevich , D. A. Parshin , H. R. Schober

Inelastic light scattering is an intensively used tool in the study of electronic properties of solids. Triggered by the discovery of high temperature superconductivity in the cuprates and by new developments in instrumentation, light…

Strongly Correlated Electrons · Physics 2009-11-11 T. P. Devereaux , R. Hackl

Hyper-Raman scattering spectra of vitreous B$_2$O$_3$ are reported and compared to Raman scattering results. The main features are indexed in terms of vibrations of structural units. Particular attention is given to the low frequency boson…

Disordered Systems and Neural Networks · Physics 2009-11-11 G. Simon , B. Hehlen , E. Courtens , E. Longueteau , R. Vacher

We use the symmetry constrained low energy effective Hamiltonian of iron based superconductors to study the Raman scattering in the normal state of underdoped iron-based superconductors. The incoming and scattered Raman photons couple…

Strongly Correlated Electrons · Physics 2015-07-01 M. Khodas , A. Levchenko

In this Letter we analyze theoretically how the emergence of collective strong coupling between vibrational excitations and confined cavity modes affects Raman scattering processes. This work is motivated by recent experiments [Shalabney et…

Mesoscale and Nanoscale Physics · Physics 2016-11-10 Javier del Pino , Johannes Feist , F. J. García-Vidal

Strong coupling between cavity photons and molecular vibrations can lead to the formation of vibron-polaritons. In a recent experiment with PVAc molecules in a metal-metal microcavity [A.Shalabney et al., Ang.Chem.Int.Ed. 54 7971 (2015)],…

Optics · Physics 2016-08-31 Artem Strashko , Jonathan Keeling

Resonant inelastic (Raman) light scattering off neutral GaAs quantum dots which contain a mean number, N=42, of electron-hole pairs is computed. We find Raman amplitudes corresponding to strongly collective final states (charge-density…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Alain Delgado , Augusto Gonzalez , Eduardo Menendez-Proupin

Strong coupling of molecular vibrations with light creates polariton states, enabling control over many optical and chemical properties. However, the near-field signatures of strong coupling are difficult to map as most cavities are closed…

The Raman response of the metallic glass Ni$_{67}$Zr$_{33}$ is measured as a function of polarization and temperature and analyzed theoretically. Unexpectedly, the intensity in the range up to 300\wn increases upon cooling, which is…

Disordered Systems and Neural Networks · Physics 2015-05-20 B. Muschler , I. Tüttő , A. Zawadowski , J. Balogh , R. Hackl

We use dynamical mean field theory to find an exact solution for inelastic light scattering in strongly correlated materials such as those near a quantum-critical metal-insulator transition. We evaluate the results for $\textbf{q}=0$…

Strongly Correlated Electrons · Physics 2009-11-10 A. M. Shvaika , O. Vorobyov , J. K. Freericks , T. P. Devereaux

Anelastic light scattering is computed numerically for model disordered systems (linear chains and 2-dimensional site and bond percolators), with and without electrical disorder. A detailed analysis of the vibrational modes and of their…

Condensed Matter · Physics 2015-06-25 P. Benassi , W. Frizzera , M. Montagna , G. Viliani , V. Mazzacurati , G. Ruocco , G. Signorelli , .

Incoherent neutron scattering experiments are simulated for simple dynamic models: a glass (with a smooth distribution of harmonic vibrations) and a viscous liquid (described by schematic mode-coupling equations). In most situations…

Soft Condensed Matter · Physics 2009-10-31 Joachim Wuttke

A consistent calculation of resonant inelastic (Raman) scattering amplitudes for relatively large quantum dots, which takes account of valence-band mixing, discrete character of the spectrum in intermediate and final states, and…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Alain Delgado , Augusto Gonzalez

Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The…

Disordered Systems and Neural Networks · Physics 2009-10-31 L. Saviot , E. Duval , J. F. Jal , A. J. Dianoux

Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Maxime Dherbécourt , Joël Bellessa , Clémentine Symonds , Guillaume Weick , David Hagenmüller

The scaling behavior of the so-called boson peak in glass-formers and its relation to the elastic properties of the system remains a source of controversy. Here, the boson peak in a binary reactive mixture is measured by Raman scattering…

Soft Condensed Matter · Physics 2013-08-06 Silvia Corezzi , Silvia Caponi , Flavio Rossi , Daniele Fioretto

Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…

Optics · Physics 2021-08-10 Xiao Liu , Zelin Ma , Aku Antikainen , Siddharth Ramachandran
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