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We have studied the Tb$_2$Sn$_2$O$_7$ frustrated magnet by neutron diffraction under isotropic pressure of 4.6 GPa, combined with uniaxial pressure of 0.3 GPa, in the temperature range 0.06 K$<$T$<$100 K. Magnetic order persists under…

Strongly Correlated Electrons · Physics 2015-05-13 I. Mirebeau , I. Goncharenko , H. Cao , A. Forget

Pyrochlore magnets are candidates for spin-ice behavior. We present theoretical simulations of relevance for the pyrochlore family R2Ti2O7 (R= rare earth) supported by magnetothermal measurements on selected systems. By considering long…

Statistical Mechanics · Physics 2009-10-31 R. Siddharthan , B. S. Shastry , A. P. Ramirez , A. Hayashi , R. J. Cava , S. Rosenkranz

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Strongly Correlated Electrons · Physics 2010-02-25 B. G. Ueland , J. S. Gardner , A. J. Williams , M. L. Dahlberg , J. G. Kim , Y. Qiu , J. R. D. Copley , P. Schiffer , R. J. Cava

Highly frustrated antiferromagnets composed of magnetic rare-earth moments are currently attracting much experimental and theoretical interest. Rare-earth ions generally have small exchange interactions and large magnetic moments. This…

Statistical Mechanics · Physics 2009-11-10 Matthew Enjalran , Michel J. P. Gingras

The pyrochlore antiferromagnet Tb2Ti2O7 has proven to be an enigma to experimentalists and theorists working on frustrated magnetic systems. The experimentally determined energy level structure suggests a local <111> Ising antiferromagnet…

Statistical Mechanics · Physics 2009-11-10 M. Enjalran , M. J. P. Gingras , Y. -J. Kao , A. Del Maestro , H. R. Molavian

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

Strongly Correlated Electrons · Physics 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

Although materials that exhibit nearest-neighbor-only antiferromagnetic interactions and geometrical frustration theoretically should not magnetically order in the absence of disorder, few such systems have been observed experimentally. One…

Strongly Correlated Electrons · Physics 2016-08-31 S. -W. Han , J. S. Gardner , C. H. Booth

In a recent letter [Phys. Rev. Lett. {\bf 82}, 1012 (1999)] it was found that the Tb$^{3+}$ magnetic moments in the Tb$_2$Ti$_2$O$_7$ pyrochlore lattice of corner-sharing tetrahedra remain in a {\it collective paramagnetic} state down to…

Disordered Systems and Neural Networks · Physics 2009-10-31 M. J. P. Gingras , B. C. den Hertog , M. Faucher , J. S. Gardner , L. J. Chang , B. D. Gaulin , N. P. Raju , J. E. Greedan

Partially-ordered magnets are distinct from both spin liquids and conventional ordered magnets because order and disorder coexist in the same magnetic phase. Here, we determine the nature of partial order in the canonical frustrated…

We present here magnetization, specific heat and Raman studies on single-crystalline specimens of the first pyrochlore member $Sm_2Ti_2O_7$ of the rare-earth titanate series. Its analogous compound $Sm_2Zr_2O_7$ in the rare-earth zirconate…

Materials Science · Physics 2009-11-13 Surjeet Singh , Surajit Saha , S. K. Dhar , R. Suryanarayanan , A. K. Sood , A. Revcolevschi

High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

Geometrical frustration, as in pyrochlore lattices made of corner-sharing tetrahedra, precludes the onset of conventional magnetic ordering, enabling the stabilization of fluctuating spin states at low temperature. Disorder is a subtle…

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Using muon-spin-relaxation measurements we show that the pyrochlore compound Gd2Ti2O7, in its magnetically orderered phase below ~ 1 K, displays persistent spin dynamics down to temperatures as low as 20 mK. The characteristics of the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Yaouanc , P. Dalmas de Reotier , V. Glazkov , C. Marin , P. Bonville , J. A. Hodges , P. C. M. Gubbens , S. Sakarya , C. Baines

Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

Disordered Systems and Neural Networks · Physics 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras
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