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The electronic structures of Mn-doped zincblende GaAs and wurtzite GaN are calculated using both standard local-density functional theory (LSDA), and a novel pseudopotential self-interaction-corrected approach (pseudo-SIC), able to account…

Mesoscale and Nanoscale Physics · Physics 2025-06-10 Alessio Filippetti , Nicola A. Spaldin , Stefano Sanvito

The electronic structure of the conjugated polymer, polyaniline, has been studied by resonant and nonresonant X-ray emission spectroscopy using synchrotron radiation for the excitation. The measurements were made on polyaniline and a few…

Materials Science · Physics 2012-01-05 M. Magnuson , J. -H. Guo , S. M. Butorin , A. Agui , C. Såthe , J. Nordgren , A. P. Monkman

The full set of high-energy spectroscopy measurements including X-ray photoelectron valence band spectra and soft X-ray emission valence band spectra of both components of FeSi (Fe K_beta_5, Fe L_alpha, Si K_beta_1,3 and Si L_2,3) are…

Atom specific valence electronic structures at interface are elucidated successfully using soft x-ray absorption and emission spectroscopy. In order to demonstrate the versatility of this method, we investigated SiO2/Si interface as a…

We investigate the electronic structure of the metallic NiS$_{1-x}$Se$_x$ system using various electron spectroscopic techniques. The band structure results do not describe the details of the spectral features in the experimental spectrum,…

Strongly Correlated Electrons · Physics 2009-10-31 S. R. Krishnakumar , N. Shanthi , Priya Mahadevan , D. D. Sarma

Electronic structure calculations, using the charge and spin self-consistent Korringa- Kohn-Rostoker (KKR) method, have been performed for several $R$Mn$X$ compounds ($R$ = Mg, Ca, Sr, Ba, Y; $X$ = Si, Ge) of the CeFeSi-type structure. The…

Materials Science · Physics 2009-11-10 V. Klosek , J. Tobola , A. Verniere , S. Kaprzyk , B. Malaman

We have studied the effect of local Coulomb interactions on the electronic structure of the molecular magnet Mn12-acetate within the LDA+U approach. The account of the on-site repulsion results in a finite energy gap and an integer value of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 D. W. Boukhvalov , A. I. Lichtenstein , V. V. Dobrovitski , M. I. Katsnelson , B. N. Harmon , V. V. Mazurenko , V. I. Anisimov

We have carried out quantum Monte Carlo (QMC) calculations of silicon crystal focusing on the accuracy and systematic biases that affect the electronic structure characteristics. The results show that 64 and 216 atom supercells provide an…

Materials Science · Physics 2021-05-26 Abdulgani Annaberdiyev , Guangming Wang , Cody A. Melton , M. Chandler Bennett , Lubos Mitas

Using angle-resolved photoemission, we have investigated the development of the electronic structure and the Fermi level pinnning in Ga$_{1-x}$Mn$_{x}$As with Mn concentrations in the range 1--6%. We find that the Mn-induced changes in the…

Materials Science · Physics 2009-11-07 H. Asklund , L. Ilver , J. Kanski , J. Sadowski , R. Mathieu

We study the importance of inter-site coherences and quantum interference effects in the x-ray absorption spectroscopy (XAS) of mixed-valent systems. We demonstrate its importance, first for a simple diatomic mixed-valent molecule to…

Strongly Correlated Electrons · Physics 2015-05-20 Subhra Sen Gupta , Hiroki Wadati , G. A. Sawatzky

We investigate the effects of electronic correlations in the full-Heusler Co$_2$MnSi, by combining a theoretical analysis of the spin-resolved density of states with tunneling-conductance spectroscopy measurements using Co$_2$MnSi as…

Strongly Correlated Electrons · Physics 2009-11-13 L. Chioncel , Y. Sakuraba , E. Arrigoni , M. I. Katsnelson , M. Oogane , Y. Ando , T. Miyazaki , E. Burzo , A. I. Lichtenstein

We present first-principles electronic structure calculations of Mn doped III-V semiconductors based on the local spin-density approximation (LSDA) as well as the self-interaction corrected local spin density method (SIC-LSD). We find that…

Materials Science · Physics 2015-06-25 T. C. Schulthess , W. M. Temmerman , Z. Szotek , A. Svane , L. Petit

A full strength Coulomb interaction between trapped electrons can be felt only in absence of a neutralizing background. In order to study quantum degenerate electrons without such a background, an external trap is needed to compensate for…

Quantum Gases · Physics 2016-05-23 Ronen Kroeze , Jom Luiten , Servaas Kokkelmans

The electronic structure of an atomic-layer-deposited MoS2 monolayer on SiO2 was investigated using X-ray absorption spectroscopy (XAS) and synchrotron X-ray photoelectron spectroscopy (XPS). The angle-dependent evolution of the XAS spectra…

The Mg2X (X=Si, Ge, Sn) based alloy is an eco-friendly thermoelectric material for mid-temperature applications. The Mg2Si1-xSnx and Mg2Ge1-xSnx alloys can be phase-separated into Si(Ge)- and Sn-rich phases during material synthesis,…

Mn doped semiconductors are extremely interesting systems due to their novel magnetic properties suitable for the spintronics applications. It has been shown recently by both theory and experiment that Mn doped GaN systems have a very high…

Materials Science · Physics 2016-08-31 B. Sanyal , O. Bengone , S. Mirbt

We consider a quantum dot coupled to both superconducting and spin-polarized electrodes, and study the triad interplay of the Kondo effect, superconductivity, and ferromagnetism, any pair of which compete with and suppress each other. We…

Mesoscale and Nanoscale Physics · Physics 2019-03-06 Minchul Lee , Mahn-Soo Choi

The crystal structures and the physical (magnetic, electrical transport and thermodynamic) properties of the ternary compounds CeRhSi2 and Ce2Rh3Si5 (orthorhombic CeNiSi2- and U2Co3Si5-type structures, respectively) were studied in wide…

Strongly Correlated Electrons · Physics 2010-05-20 D. Kaczorowski , A. P. Pikul , U. Burkhardt , M. Schmidt , A. Slebarski , A. Szajek , M. Werwinski , Yu. Grin

We demonstrate that a theoretical framework fully incorporating intra-atomic correlations and multiplet structure of the localized 4f states is required in order to capture the essential physics of rare-earth semiconductors and semimetals.…

Strongly Correlated Electrons · Physics 2009-03-03 Leonid V. Pourovskii , Kris T. Delaney , Chris G. Van de Walle , Nicola A. Spaldin , Antoine Georges

We report first-principles calculations on the normal and superconducting state of CaBe(x)Si(2-x) (x=1), in the framework of density functional theory for superconductors (SCDFT). CaBeSi is isostructural and isoelectronic to MgB2 and this…

Superconductivity · Physics 2013-05-29 C. Bersier , A. Floris , A. Sanna , G. Profeta , A. Continenza , E. K. U. Gross , S. Massidda