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Related papers: Resonant x-ray scattering study on multiferroic Bi…

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It is proposed that the observation of orbital ordering in manganite materials should be possible at the L_II and L_III edges of manganese using X-ray resonant scattering. If performed, dipole selection rules would make the measurements…

Condensed Matter · Physics 2009-10-31 C. W. M. Castleton , M. Altarelli

We provide a detailed study of the reflectivity of multiferroic TbMnO_3 for wave numbers from 40 cm^{-1} to 1000 cm^{-1} and temperatures 5 K < T < 300 K. Excitations are studied for polarization directions E || a, the polarization where…

Strongly Correlated Electrons · Physics 2010-01-22 M. Schmidt , Ch. Kant , T. Rudolf , F. Mayr , A. A. Mukhin , A. M. Balbashov , J. Deisenhofer , A. Loidl

Soft x-ray resonant scattering has been used to examine the charge and magnetic interactions in the cycloidal antiferromagnetic compound \dyfeal. By tuning to the Dy $M_4$ and $M_5$ absorption edges and the Fe L(2) and L(3) absorption edges…

Strongly Correlated Electrons · Physics 2007-05-23 T. A. W. Beale , S. B. Wilkins , P. D. Hatton , P. Abbamonte , S. Stanescu , J. A. Paixao

We report coherent x-ray scattering studies of charge and orbital domains in manganite systems. The experiments were carried out on LaMnO_3 and Pr_{0.6}Ca_{0.4}MnO_3, with the incident photon energy tuned near the Mn K edge. At room…

Strongly Correlated Electrons · Physics 2009-11-07 C. S. Nelson , J. P. Hill , Doon Gibbs , F. Yakhou , F. Livet , Y. Tomioka , T. Kimura , Y. Tokura

We have utilized the resonant x-ray diffraction technique at the Mn L-edge in order to directly compare magnetic and orbital correlations in the Mn sub-lattice of Pr0.6Ca0.4MnO3. The resonant line shape is measured below T_OO ~ 240 K at the…

Strongly Correlated Electrons · Physics 2009-11-10 K. J. Thomas , J. P. Hill , Y-J. Kim , S. Grenier , P. Abbamonte , L. Venema , A. Rusydi , Y. Tomioka , Y. Tokura , D. F. McMorrow , M. van Veenendaal

We investigate the mechanism of the resonant X-ray scattering on the Ti $K$ edge region of YTiO$_3$ using the band structure calculation combined with the local density approximation. A large intensity is obtained for the orbital…

Strongly Correlated Electrons · Physics 2007-05-23 Manabu Takahashi , Jun-ichi Igarashi

We report resonant inelastic x-ray scattering experiments of the orbital ordered manganite LaMnO3. When the incident photon energy is tuned near the Mn K absorption edge, the spectra reveal three features at 2.5 eV, 8 eV and 11 eV. The 8 eV…

Strongly Correlated Electrons · Physics 2007-05-23 T. Inami , S. Ishihara , H. Kondo , J. Mizuki , T. Fukuda , S. Maekawa , H. Nakao , T. Matsumura , K. Hirota , Y. Murakami , Y. Endoh

Ru M$_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of RuCl$_3$ with 27 meV resolution reveals a spin-orbit exciton without noticeable splitting. We extract values for the spin-orbit coupling constant ($\lambda=154\pm2$…

Strongly Correlated Electrons · Physics 2020-01-29 Blair W Lebert , Subin Kim , Valentina Bisogni , Ignace Jarrige , Andi M Barbour , Young-June Kim

The recent discovery that resonant inelastic x-ray scattering can probe single-magnon (SM) dispersions in transition metal (TM) oxides when the x-ray energy is tuned to the TM $L$-edge, has put this technique on a par with inelastic neutron…

Strongly Correlated Electrons · Physics 2015-08-19 Beom Hyun Kim , Jeroen van den Brink

Orbital degree of freedom of electrons and its interplay with spin, charge and lattice degrees of freedom are one of the central issues in colossal magnetoresistive manganites. The orbital degree of freedom has until recently remained…

Strongly Correlated Electrons · Physics 2009-11-07 Sumio Ishihara , Sadamichi Maekawa

We report measured dipolar asymmetry ratios at the LIII edges of the heavy rare earth metals. The results are compared with a first principles calculation and excellent agreement is found. A simple model of the scattering is developed,…

We calculated the polarization-dependent Raman scattering cross section spectra of LaMnO3 below the A-type magnetic ordering temperature. Two strong peaks appear around the MnO6 octahedra stretching phonon frequency. One mode shows Ag…

Strongly Correlated Electrons · Physics 2018-02-07 Purevdorj Munkhbaatar , Kim Myung-Whun

We have conducted a series of scattering experiments at the uranium M4 absorption edge on low-symmetry uranium compounds (U2N3 and U3O8) produced as epitaxial films. At weak and forbidden reflections, we find a resonant signal, independent…

Strongly Correlated Electrons · Physics 2024-10-02 E. Lawrence Bright , E. N. Ovchinnikova , L. M. Harding , D. G. Porter , R. Springell , V. E. Dmitrienko , R. Caciuffo , G. H. Lander

We have performed a resonant x-ray scattering (RXS) study near the Co K edge on a single crystal of Ca3Co2O6. In the magnetically ordered phase a new class of weak reflections appears at the magnetic propagation vector tau (1/3,1/3,1/3).…

Strongly Correlated Electrons · Physics 2009-11-13 A. Bombardi , C. Mazzoli , S. Agrestini , M. R. Lees

We investigated the effects of temperature and magnetic field on the electronic structure of hexagonal RMnO3 (R = Gd, Tb, Dy, and Ho) thin films using optical spectroscopy. As the magnetic ordering of the system was disturbed, a systematic…

Strongly Correlated Electrons · Physics 2010-05-17 Woo Seok Choi , Soon Jae Moon , Sung Seok A. Seo , Daesu Lee , Jung Hyuk Lee , Pattukkannu Murugavel , Tae Won Noh , Yun Sang Lee

We present a temperature and doping dependent resonant inelastic X-ray scattering experiment at the V L$_{2,3}$ and O K edges in La$_{1-x}$Sr$_x$VO$_3$ for $x=0$ and $x=0.1$. This material is a canonical example of a compound that exhibits…

We present results of our study of polarized Raman scattering and infrared reflectivity of rhombohedral ceramic La_1-ySr_yMn_1-xM_xO_3 manganites in the temperature range between 77 and 320K. In our samples, a part of the Mn atoms is…

Strongly Correlated Electrons · Physics 2009-11-11 A. Dubroka , J. Humlicek , M. V. Abrashev , Z. V. Popovic , F. Sapina , A. Cantarero

X-ray absorption and resonant inelastic x-ray scattering measurements are carried out on lithium nitrate LiNO$_3$. The $\sigma$ orbitals around the nitrogen atoms exhibit a large lifetime effect. Experimentally, this is manifest as an…

Materials Science · Physics 2019-09-04 John Vinson , Terrence Jach , Matthias Müller , Rainer Unterumsberger , Burkhard Beckhoff

Soft X-ray resonant powder diffraction has been performed at the Mn L2,3 edges of A-site ordered SmBaMn2O6. The energy and polarization dependence of the (1/2 1/2 0) reflection provide direct evidence for a (x2-z2)/(y2-z2) type orbital…

Strongly Correlated Electrons · Physics 2009-11-13 M. Garcia-Fernandez , U. Staub , Y. Bodenthin , S. M. Lawrence , A. M. Mulders , C. E. Buckley , S. Weyeneth , E. Pomjakushina , K. Conder

We report a Raman scattering investigation of KTa1-xNbxO3 (x = 0.35, 0.5) thin films deposited on MgO and LaAlO3 as a function of temperature. The observed phase sequence in the range from 90 K to 720 K is similar to the structural phase…

Materials Science · Physics 2010-07-16 A. Bartasyte , J. Kreisel , W. Peng , M. Guilloux-Viry