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The lithium manganese oxide spinel Li$_x$Mn$_2$O$_4$, with $0\leq x\leq 2$, is an important example for cathode materials in lithium ion batteries. However, an accurate description of Li$_x$Mn$_2$O$_4$ by first-principles methods like…

Materials Science · Physics 2020-05-20 Marco Eckhoff , Peter E. Blöchl , Jörg Behler

We report first principles LDA calculations of the electronic structure and thermoelectric properties of $\beta $-Zn$_{4}$Sb$_{3}$. The material is found to be a low carrier density metal with a complex Fermi surface topology and…

Materials Science · Physics 2009-10-30 Seong-Gon Kim , I. I. Mazin , D. J. Singh

In this work we investigate the electronic properties of mercaptocarboxylic acids with several carbon chain lengths adsorbed on ZnO-(10-10) surfaces via density functional theory calculations using semi-local and hybrid exchange-correlation…

Materials Science · Physics 2018-10-05 Dennis Franke , Michael Lorke , Thomas Frauenheim , Andrea L. daRosa

The rare physical property of negative thermal expansion (NTE) is intriguing because materials with large NTE over a wide temperature range can serve as high-performance thermal expansion compensators. However, applications of NTE are…

Divalent tin oxides have attracted considerable attention as novel p-type oxide semiconductors, which are essential for realizing future oxide electronic devices. Recently, p-type Sn2Nb2O7 and SnNb2O6 were developed; however, enhanced hole…

Materials Science · Physics 2020-12-25 Akane Samizo , Makoto Minohara , Naoto Kikuchi , Kyoko K. Bando , Yoshihiro Aiura , Ko Mibu , Keishi Nishio

The growing interest in tin-halide semiconductors for photovoltaic applications demands an in-depth knowledge of the fundamental properties of its constituents, starting from the smallest monomers entering the initial stages of formation.…

Materials Science · Physics 2024-02-21 Freerk Schütt , Ana M. Valencia , Caterina Cocchi

It has been demonstrated that InSb nanoinclusions, which are formed in situ, can simultaneously improve all three individual thermoelectric properties of the n-type half Heusler compound (Ti,Zr,Hf)(Co,Ni)Sb [Xie et al., Acta Mater. 58, 4795…

\ We combine density functional theory and molecular dynamics simulations to investigate the impact of Sr concentration and atomic ordering on the structural and ferroelectric properties of (Ba, Sr)TiO$_3$. On one hand, the macroscopic…

Materials Science · Physics 2023-08-28 Aris Dimou , Ankita Biswas , Anna Gruenebohm

Density functional theory based study of the pressure dependent physical properties of binary SnS compound has been carried out. The computed elastic constants reveal that SnS is mechanically stable and brittle under ambient conditions.…

Materials Science · Physics 2022-10-31 Ayesha Tasnim , Md. Mahamudujjaman , Md. Asif Afzal , R. S. Islam , S. H. Naqib

Two-dimensional (2D) perovskites show higher stability in comparison to their three-dimensional (3D) counterparts. Therefore, 2D perovskites have invoked remarkable attention in basic understanding of their physical properties and…

Materials Science · Physics 2025-07-01 Deepika Gill , Gunjana Yadav , Saswata Bhattacharya

In this work we use density functional theory (DFT) to investigate the influence of semi-local exchange and correlation effects on the electronic and optical properties of zinc oxide. We find that the inclusion of such effects using the…

Materials Science · Physics 2019-05-01 R. M. V. S. Almeida , A. L. da Rosa , J. S. de Almeida

In this work we have employed density-functional theory with hybrid functionals to investigate the atomic and electronic structure of bare and hydrogenated Mn doped ZnO nanowires with small diameter. We determine changes in magnetic and…

Materials Science · Physics 2018-10-23 A. L. Rosa , L. L. Tacca , E. N. Lima , Th. Frauenheim

We analyze the basic structural units of simple reconstructions of the (111) surface of SrTiO3 using density functional calculations. The prime focus is to answer three questions: what is the most appropriate functional to use; how accurate…

Materials Science · Physics 2025-09-22 Laurence D. Marks , Ann N. Chiaramonti , Fabien Tran , Peter Blaha

We report a series of calculations testing the predictions of the Tran-Blaha functional for the electronic structure and magnetic properties of condensed systems. We find a general improvement in the properties of semiconducting and…

Materials Science · Physics 2010-11-08 David J. Singh

Thermodynamic stability of N$_2$ clathrate hydrates in the sI and sII structures is investigated using density functional theory with several exchange-correlation functionals, explicitly accounting for composition (cage occupancies) and…

Materials Science · Physics 2025-12-19 L. Martin-Gondre , V. Meko Fotso , C. Métais , A. Patt , J. Ollivier , A. Desmedt

The solvation of hydrophobic solutes in water is special because liquid and gas are almost at coexistence. In the common hypernetted chain approximation to integral equations, or equivalently in the homogenous reference fluid of molecular…

Chemical Physics · Physics 2015-04-21 Guillaume Jeanmairet , Maximilien Levesque , Volodymyr Sergiievskyi , Daniel Borgis

We combine Z-contrast scanning transmission electron microscopy with density-functional-theory calculations to determine the atomic structure of the Fe/AlGaAs interface in spin-polarized light-emitting diodes. A 44% increase in…

Layered black arsenic (b-As) has recently emerged as a new anisotropic two-dimensional (2D) semiconducting material with applications in electronic devices. Understanding factors affecting the ambient stability of this material remains…

Materials Science · Physics 2022-07-07 Mayank Tanwar , Sagar Udyavara , Hwanhui Yun , Supriya Ghosh , K. Andre Mkhoyan , Matthew Neurock

We have investigated the effect of Sb-deficiency on the thermoelectric figure of merit (zT) of Zn4Sb3 prepared by solid state reaction route. At high temperatures, the Seebeck coefficient (S) and electrical conductivity ({\sigma}) increase…

Materials Science · Physics 2015-05-06 Anup V. Sanchela , Ajay D. Thakur , C. V. Tomy

Heusler compounds form a numerous class of intermetallics, which include two families of compositions ABC and AB2C, usually referred to as half- and full-Heusler compounds, respectively. Given their tunable electronic properties, made…

Materials Science · Physics 2018-07-17 M. Pani , I. Pallecchi , C. Bernini , N. Ardoino , D. Marré