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We present a quaternion inspired formalism specifically developed to evaluate the intensity of the electrical current that traverses a single molecule connected to two semi-infinite electrodes as the applied external bias is varied. The…

Mesoscale and Nanoscale Physics · Physics 2012-01-18 Augusto C. L. Moreira , Celso P. de Melo

We present a general analytical formula and an ab initio study of quantum interference in multi-branch molecules. Ab initio calculations are used to investigate quantum interference in a benzene-1,2-dithiolate (BDT) molecule sandwiched…

Mesoscale and Nanoscale Physics · Physics 2016-08-14 R. E. Sparks , V. M. García-Suárez , D. Zs. Manrique , C. J. Lambert

We use the recently proposed scattering states numerical renormalization group (SNRG) approach to calculate $I(V)$ and the differential conductance through a single molecular level coupled to a local molecular phonon. We also discuss the…

Strongly Correlated Electrons · Physics 2015-06-12 Andre Jovchev , Frithjof Anders

The effects of a coupling between the quantized mechanical vibrations of a quantum dot and coherent tunneling of electrons through a single level in the dot are studied. The equation of motion for the reduced density operator describing the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 D. Fedorets , L. Y. Gorelik , R. I. Shekhter , M. Jonson

We report a systematic study of transport properties of nanosytems with charge density waves. We demonstrate, how the presence of density waves modifies the current-voltage characteristics. On the other hand hand, we show that the density…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Marcin Mierzejewski , Maciej M. Maska

The deviation of positions of atoms from their ideal lattice sites in crystalline solid state systems causes distortion and can lead to variation in structural [1] and functional properties [2]. Distortion in molecular systems has been…

Materials Science · Physics 2019-11-15 G. Anand , Markus Eisenbach , Russell Goodall , Colin L. Freeman

In a recent experiment, Hirjibehedin {\it et al.} [Science {\bf 317}, 1199 (2007)] performed inelastic tunneling spectroscopy of a single iron atom absorbed on a nonmagnetic substrate. The observed steps in the differential conductance…

Mesoscale and Nanoscale Physics · Physics 2010-08-16 Björn Sothmann , Jürgen König

Coherent electronic transport through individual molecules is crucially sensitive to quantum interference. Using exact diagonalization techniques, we investigate the zero-bias and zero-temperature conductance through $\pi$-conjugated…

Strongly Correlated Electrons · Physics 2015-05-14 Julian Rincon , K. Hallberg , S. Ramasesha

In this work, we have investigated conduction through an artificial molecule comprising two coupled quantum dots. The question addressed is the role of inter-dot coupling on electronic transport. We find that the current through the…

Mesoscale and Nanoscale Physics · Physics 2011-09-22 M. Imran , B. Tariq , M. Tahir , K. Sabeeh

Continuum states of the Dirac equation are calculated numerically for the electrostatic field generated by the charge distribution of an atomic nucleus. The behavior of the wave functions of an incoming electron with a given asymptotic…

Nuclear Theory · Physics 2007-05-23 Andreas Aste , Cyrill von Arx , Dirk Trautmann

We assess how quantum-mechanical effects associated with high-frequency chromophore vibrations influence excitation energy transfer in biological light-harvesting complexes. We begin with a mixed quantum-classical theory that combines a…

Chemical Physics · Physics 2025-01-07 Johan E. Runeson , David E. Manolopoulos

We have carried out calculations of electron transport through a metal-molecule-metal junction with metal nanoclusters taking the part of electrodes. We show that negative differential resistance peaks could appear in the current-voltage…

Materials Science · Physics 2008-10-22 Natalya A. Zimbovskaya , Mark R. Pederson

We investigate the electronic transport through a molecule in the Kondo regime. The tunneling between the electrode and the molecule is asymmetrically modulated by the oscillations of the molecule, i.e., if the molecule gets closer to one…

Mesoscale and Nanoscale Physics · Physics 2008-12-09 J. Mravlje , A. Ramsak

We present a microscopic model, describing current-driven switching in metallic atomic-size contacts. Applying a high current through an atomic-size contact, creates a strong electronic nonequilibrium that excites vibrational modes by…

Mesoscale and Nanoscale Physics · Physics 2024-05-03 Markus Ring , Fabian Pauly , Peter Nielaba , Elke Scheer

We look for manifestations of quantum interference effects in the Seebeck coefficient of a molecular junction, when the electronic conductance exhibits pronounced destructive interference features due to the presence of quasi-degenerate…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Lena Simine , Wei Jia Chen , Dvira Segal

It has been observed experimentally [H.R. Xia, C.Y. Ye, and S.Y. Zhu, Phys. Rev. Lett. {\bf 77}, 1032 (1996)] that quantum interference between two molecular transitions can lead to a suppression or enhancement of spontaneous emission. This…

Quantum Physics · Physics 2009-10-31 Jin Wang , H. M. Wiseman , Z. Ficek

The charge state stability of nitrogen-vacancy (NV) centers critically affects their application as quantum sensors and qubits. Understanding charge state conversion and equilibration is critical not only for NV centers in diamond but also…

Materials Science · Physics 2025-12-02 Audrius Alkauskas , Chris G. Van de Walle , Lukas Razinkovas , Ronald Ulbricht

We explore electron transport properties for the model of benzene-1, 4-dithiolate (BDT) molecule and for some other geometric models of benzene molecule attached to two semi-infinite one-dimensional metallic electrodes using the Green's…

Mesoscale and Nanoscale Physics · Physics 2010-04-13 Santanu K. Maiti

We measure the low bias conductance of a series of substituted benzene diamine molecules while breaking a gold point contact in a solution of the molecules. Transport through these substituted benzenes is by means of nonresonant tunneling…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Latha Venkataraman , Young S. Park , Adam C. Whalley Colin Nuckolls , Mark S. Hybertsen , Michael L. Steigerwald

Nuclear-spin-dependent (NSD) parity violating (PV) effects can be strongly enhanced in diatomic molecules containing heavy atoms. Future measurements are anticipated to provide nuclear anapole moments and strength constants for PV nuclear…

Atomic Physics · Physics 2012-11-20 A. Borschevsky , M. Iliaš , V. A. Dzuba , K. Beloy , V. V. Flambaum , P. A. Schwerdtfeger