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Rattling-induced superconductivity in the {\beta}-pyrochlore oxide KOs2O6 is investigated under high pressure up to 5 GPa. Resistivity measurements in a high-quality single crystal reveal a gradual decrease in the superconducting transition…

We report the discovery of a new pyrochlore oxide superconductor RbOs2O6. The compound crystallizes in the same beta-pyrochlore structure as the recently discovered superconductor KOs2O6, where Os atoms form a corner-sharing tetrahedral…

Superconductivity · Physics 2009-11-10 S. Yonezawa , Y. Muraoka , Y. Matsushita , Z. Hiroi

Electronic, magnetic, and dynamical properties of the new superconducting $\beta$-pyrochlore KOs$_2$O$_6$ and related RbOs$_2$O$_6$ and CsOs$_2$O$_6$ compounds are calculated and compared with experiment and contrasted with structurally…

Superconductivity · Physics 2009-11-10 J. Kunes , T. Jeong , W. E. Pickett

Single crystals of KOs2O6 have been grown in a sealed quartz ampoule. Detailed single crystal X-ray diffraction studies at room temperature show Bragg peaks that violate Fd-3m symmetry. With a comparative structure refinement the structure…

Superconductivity · Physics 2009-11-11 G. Schuck , S. M. Kazakov , K. Rogacki , N. D. Zhigadlo , J. Karpinski

Superconductivity in the potassium osmium oxide KOs2O6 crystallizing in the beta-pyrochlore structure is studied by means of electrical resistivity, magnetic susceptibility and specific heat. It is the second superconductor in the family of…

Superconductivity · Physics 2009-11-10 Z. Hiroi , S. Yonezawa , Y. Muraoka

A new modification of KOs2O6, the representative of a new structural type (Pearson symbol aP18, a=5.5668(1)A, b=6.4519(2)A, c=7.2356(2)A, space group P-1, no.2) was synthesized employing high pressure technique. Its structure was determined…

Superconductivity · Physics 2010-03-03 S. Katrych , Q. F. Gu , Z. Bukowski , N. D. Zhigadlo , G. Krauss , J. Karpinski

Chemical trends of fundamental superconducting parameters and normal-state properties are described for a family of pyrochlore oxide superconductors. Particularly, the change of Tc from 1.0 K for alpha-pyrochlore Cd2Re2O7 to 3.3 K (A = Cs),…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Jun-Ichi Yamaura , Shigeki Yonezawa , Hisatomo Harima

The superconducting properties of two beta-pyrochlore oxides, CsOs2O6 and RbOs2O6, are studied by thermodynamic and transport measurements using high-quality single crystals. It is shown that the character of superconductivity changes…

Superconductivity · Physics 2009-08-05 Yohei Nagao , Jun-ichi Yamaura , Hiroki Ogusu , Yoshihiko Okamoto , Zenji Hiroi

Rattling-induced superconductivity in the beta-pyrochlore oxide RbOs2O6 is investigated under high pressures up to 6 GPa. Resistivity measurements in a high-quality single crystal show that the superconducting transition temperature Tc…

Superconductivity · Physics 2011-10-04 Nao Takeshita , Hiroki Ogusu , Jun-ichi Yamaura , Yoshihiko Okamoto , Zenji Hiroi

Superconducting and normal-state properties of the beta-pyrochlore oxide KOs2O6 are studied by means of thermodynamic and transport measurements. It is shown that the superconductivity is of conventional s-wave type and lies in the…

Superconductivity · Physics 2009-11-13 Z. Hiroi , S. Yonezawa , Y. Nagao , J. Yamaura

{\ss}-pyrochore KOs2O6, which shows superconductivity below ~ 9.7K, has been converted into KxOs2O6 (x < 2/3 - 1/2) electrochemically to show spin glass-like behavior below ~ 6.1K. Room temperature sample surface potential versus charge…

Superconductivity · Physics 2015-05-27 C. C. Lee , W. L. Lee , J. -Y. Lin , C. C. Tsuei , J. G. Lin , F. C. Chou

Pressure dependence of superconducting transition temperature $T_{\rm c}$ has been determined through the DC magnetic measurements under pressure up to $P$=10 GPa for $\beta$-pyrochlore oxides AOs$_2$O$_6$ with A=Cs ($T_{\rm c}$=3.3 K), Rb…

Superconductivity · Physics 2009-11-13 K. Miyoshi , Y. Takaichi , Y. Takamatsu , M. Miura , J. Takeuchi

The crystal structure of Pb$_{10}$(PO$_4$)$_6$O, the proposed matrix for the potential room-temperature superconductor LK-99, Pb$_{10-x}$Cu$_x$(PO$_4$)$_6$O ($x = 0.9-1.0$), has been reinvestigated by single-crystal X-ray diffraction using…

Superconductivity · Physics 2023-08-10 Sergey V. Krivovichev

We report nuclear magnetic resonance studies on the beta-pyrochlore oxide superconductor KOs2O6. The nuclear relaxation at the K sites is entirely caused by fluctuations of electric field gradient, which we ascribe to highly anharmonic low…

Superconductivity · Physics 2009-11-11 M. Yoshida , K. Arai , R. Kaido , M. Takigawa , S. Yonezawa , Y. Muraoka , Z. Hiroi

Single crystals of RbOs2O6 have been grown from Rb2O and Os in sealed quartz ampoules. The crystal structure has been identified at room temperature as cubic with the lattice constant a = 10.1242(12) A. The anisotropy of the tetrahedral and…

Superconductivity · Physics 2009-11-13 K. Rogacki , G. Schuck , Z. Bukowski , N. D. Zhigadlo , J. Karpinski

Another phase transition that is probably of first order is found in the beta-pyrochlore oxide superconductor KOs2O6 with a superconducting transition temperature Tc of 9.6 K. It takes place at Tp=7.5 K in the superconducting state in a…

Superconductivity · Physics 2015-06-25 Z Hiroi , S Yonezawa , J Yamaura

We report a structural phase transition found at Ts = 200 K in a pyrochlore oxide Cd2Re2O7 which shows superconductivity at Tc = 1.0 K. X-ray diffractionexperiments indicate that the phase transition is of the second order, from a…

Superconductivity · Physics 2009-11-07 M. Hanawa , J. Yamaura , Y. Muraoka , F. Sakai , Z. Hiroi

Evidence for another phase transition at 120 K in the metallic pyrochlore oxide Cd2Re2O7, following the structural transition at 200 K and followed by the superconducting transition at 1.0 K, is given through resistivity, magnetoresistance,…

Strongly Correlated Electrons · Physics 2009-11-07 Zenji Hiroi , Jun-Ichi Yamaura , Yuji Muraoka , Masafumi Hanawa

The discovery of a new beta-pyrochlore oxide superconductor CsOs2O6 with Tc = 3.3 K is reported. It is the third superconductor in the family of beta-pyrochlore oxides, following KOs2O6 with Tc = 9.6 K and RbOs2O6 with Tc = 6.3 K. The Tc of…

Superconductivity · Physics 2009-11-10 Shigeki Yonezawa , Yuji Muraoka , Zenji Hiroi

We report a first-principles density-functional calculation of the electronic structure and properties of the recently discovered superconducting beta-pyrochlore oxide KOs_2O_6. We find that the electronic structure near the Fermi energy…

Superconductivity · Physics 2009-11-10 R. Saniz , J. E. Medvedeva , Lin-Hui Ye , T. Shishidou , A. J. Freeman
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