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Designing and understanding functional electronic and magnetic properties in perovskite oxides requires controlling and tuning the underlying crystal lattice. Here we report the structure, including oxygen and cation positions, of a…

In this work the charge transport properties of charge ordered (CO) La1-xCaxMnO3 (LCMO) (x= 0.55, 0.67) epitaxial thin films and polycrystals are discussed following the recent controversy of localised electron states vs. weakly or de-…

Strongly Correlated Electrons · Physics 2009-11-13 Rainer Schmidt

We present angle-resolved photoemission spectroscopy results for thin films of the three-dimensional manganese perovskite La$_{1-x}$Sr$_{x}$MnO$_{3}$. We show that the transition temperature ($T_c$) from the paramagnetic insulating to…

Strongly Correlated Electrons · Physics 2008-04-23 M. Shi , M. C. Falub , P. R. Willmott , J. Krempasky , R. Herger , L. Patthey , K. Hricovini , C. Falub , M. Schneider

Low as well as high-temperature electron and x-ray diffraction studies have been carried out on a rare-earth free B-site disordered electron-doped manganite SrMn0.875.Mo0.125O3-{\delta} in the temperature range of 83K to 637K. These studies…

Strongly Correlated Electrons · Physics 2015-03-23 Aga Shahee , N. P. Lalla

We report and compare the structural, magnetic, and optical properties of ordered La2NiMnO6 thin films and its disordered LaNi0.5Mn0.5O3 counterpart. An x-ray diffraction study reveals that the B-site Ni/Mn ordering induces additional XRD…

Materials Science · Physics 2015-05-13 M. P. Singh , K. D. Truong , S. Jandl , P. Fournier

Structural study of orbital-ordered manganite thin films has been conducted using synchrotron radiation, and a ground state electronic phase diagram is made. The lattice parameters of four manganite thin films, Nd0.5Sr0.5MnO3 (NSMO) or…

Strongly Correlated Electrons · Physics 2011-03-08 Y. Wakabayashi , D. Bizen , Y. Kubo , H. Nakao , Y. Murakami , M. Nakamura , Y. Ogimoto , K. Miyano , H. Sawa

We performed resonant and nonresonant x-ray diffraction studies of a Nd0.5Sr0.5MnO3 thin film that exhibits a clear first-order transition. Lattice parameters vary drastically at the metal-insulator transition at 170K (=T_MI), and…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Wakabayashi , D. Bizen , H. Nakao , Y. Murakami , M. Nakamura , Y. Ogimoto , M. Izumi , K. Miyano , H. Sawa

A variety of emergent phenomena has been enabled by interface engineering in the complex oxides heterostructures. While extensive attention has been attracted to LaMnO3 (LMO) thin films for observing the control of functionalities at its…

We demonstrate the stability of ferromagnetic order of one unit cell thick optimally doped manganite (La0.7Ba0.3MnO3, LBMO) epitaxially grown between two layers of SrRuO3 (SRO) by using x-ray magnetic circular dichroism. At low temperature…

A microscopic characterisation of the phase transitions associated with colossal magnetoresistance (CMR) in manganese perovskite oxides is a very important ingredient in the quest of understanding its underlying mechanism. Scanning…

Strongly Correlated Electrons · Physics 2007-05-23 Ch. Renner , G. Aeppli , H. M. Ronnow

We have studied the atomic ordering of B-site transition metals and magnetic properties in the pulsed-laser deposited films of La2CrFeO6 (LCFO) and La2VMnO6 (LVMO), whose bulk materials are known to be single perovskites with random…

Materials Science · Physics 2015-06-12 Akira Ohtomo , Suvankar Chakraverty , Hisanori Mashiko , Takayoshi Oshima , Masashi Kawasaki

Thin-film colossal magnetoresistance manganites such as La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ (LCMO) have now been intensely studied for more than a decade, but the issue of possible nanoscale electronic phase separation is not fully solved.…

Strongly Correlated Electrons · Physics 2009-02-05 S. Kelly , F. Galli , I. Komissarov , J. Aarts

$^{139}$La- and $^{55}$Mn-NMR spectra demonstrate that the ground state of the A-site ordered perovskite manganite LaBaMn$_2$O$_6$ is a spatial mixture of the ferromagnetic (FM) and antiferromagnetic (AFI(CE)) regions, which are assigned to…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Kawasaki , T. Minami , Y. Kishimoto , T. Ohno , K. Zenmyo , H. Kubo , T. Nakajima , Y. Ueda

Phase-separated manganites provide a unique platform to study the dynamics of competing electronic and structural orders in correlated systems. In La0.275Pr0.35Ca0.375MnO3 (LPCMO), we use temperature-cycling Raman spectroscopy to uncover a…

We have succeeded in preparing A-site ordered- and disordered-Y1/4Sr3/4CoO3-d with various oxygen deficiencies delta, and have made comparative study of their structural and physical properties. In the A-site ordered structure, oxygen…

Strongly Correlated Electrons · Physics 2008-01-30 S. Fukushima , T. Sato , D. Akahoshi , H. Kuwahara

The crystal and magnetic structure of polycrystalline $La{}_{0.5-x}Nd{}_{x}Ca_{0.5}MnO{}_{3}$ (0.0 \ensuremath{\le} x \ensuremath{\le} 0.5) samples have been investigated using magnetization, resistivity, transmission electron microscope,…

Materials Science · Physics 2010-11-01 Indu Dhiman , A. Das , P. K. Mishra , N. P. Lalla , A. Kumar

We have synthesized epitaxial La(1-x)Sr(1+x)MnO4 (x=1/3) films as random alloys and cation-ordered analogues to probe how cation order affects the properties of a 2D manganite. The films show weak ferromagnetic ordering up to 130 K,…

Strongly Correlated Electrons · Physics 2015-05-20 B. B. Nelson-Cheeseman , A. B. Shah , T. S. Santos , S. D. Bader , J. -M. Zuo , A. Bhattacharya

We present resonant soft X-ray scattering (RSXS) results from small band width manganites (Pr,Ca)MnO$_3$, which show that the CE-type spin ordering (SO) at the phase boundary is stabilized only below the canted antiferromagnetic transition…

Atomically sharp oxide heterostructures often exhibit unusual physical properties that are absent in the constituent bulk materials. The interplay between electrostatic boundary conditions, strain and dimensionality in ultrathin epitaxial…

Charge-lattice fluctuations are observed in the layered perovskite manganite LaSr2Mn2O7 by Raman spectroscopy as high as 340 K and with decreasing temperature they become static and form a charge ordered (CO) phase below TCO=210 K. In the…

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