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We report the specific heat and entropy of single crystals of the spin ice compound Dy2Ti2O7 at temperatures down to 0.35 K. We apply magnetic fields along the four characteristic directions: [100], [110], [111] and [112]. Because of Ising…

Strongly Correlated Electrons · Physics 2009-11-10 Ryuji Higashinaka , Hideto Fukazawa , Yoshiteru Maeno

We study the low-temperature behaviour of spin ice when uniaxial pressure induces a tetragonal distortion. There is a phase transition between a Coulomb liquid and a fully magnetised phase. Unusually, it combines features of discontinuous…

Statistical Mechanics · Physics 2010-09-07 Ludovic D. C. Jaubert , J. T. Chalker , Peter C. W. Holdsworth , R. Moessner

Muon spin relaxation measurements on some quantum spin ice candidate materials, the insulating pyrochlores Pr2B2O7 (B = Sn, Zr, Hf), have been performed for temperatures in the range 0.05-280 K. The results are indicative of a static…

Strongly Correlated Electrons · Physics 2015-06-22 F. R. Foronda , F. Lang , J. S. Möller , T. Lancaster , A. T. Boothroyd , F. L. Pratt , S. R. Giblin , D. Prabhakaran , S. J. Blundell

Around 0.5 K, the entropy of the spin-ice Dy$_2$Ti$_2$O$_7$ has a plateau-like feature close to Pauling's residual entropy derived originally for water ice, but an unambiguous quantification towards lower temperature is prevented by…

Strongly Correlated Electrons · Physics 2017-09-04 S. Scharffe , O. Breunig , V. Cho , P. Laschitzky , M. Valldor , J. F. Welter , T. Lorenz

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

Strongly Correlated Electrons · Physics 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

We investigated the possibility of temperature dependent lattice distortions in the pyrochlore compound Tb$_{2}$Ti$_{2}$O$_{7}$ by measuring the internal magnetic field distribution, using muon spin resonance, and comparing it to the…

Strongly Correlated Electrons · Physics 2015-06-25 Oren Ofer , Amit Keren , Chris Baines , Jason S. Gardner

We present here temperature-dependent Raman, x-ray diffraction and specific heat studies between room temperature and 12 K on single crystals of spin-ice pyrochlore compound $Dy_2Ti_2O_7$ and its non-magnetic analogue $Lu_2Ti_2O_7$. Raman…

Materials Science · Physics 2009-11-13 Surajit Saha , Surjeet Singh , B. Dkhil , S. Dhar , R. Suryanarayanan , G. Dhalenne , A. Revcolevschi , A. K. Sood

A "supercooled" liquid develops when a fluid does not crystallize upon cooling below its ordering temperature. Instead, the microscopic relaxation times diverge so rapidly that, upon further cooling, equilibration eventually becomes…

Rapidly developing science and technology demand new materials with versatile and promising properties for practical applications. In this context, pseudo-octahedral iron(II) spin crossover (SCO) complexes are particularly appealing - not…

Structural disorder in the magnetically frustrated pyrochlore system leads to intriguing magnetic states. We present the thermodynamic behavior and short range magnetic correlations in Tb$_{2}$Zr$_{2}$O$_{7}$ and…

Strongly Correlated Electrons · Physics 2026-04-16 Sujata Singh , Leon Carstens , M. Duc Le , R. Klingeler , C. S. Yadav

We have studied the influence of the magnetization on the superconducting transition temperature ($T_c$) in bi- and trilayers consisting of the half-metallic ferromagnet La$_{0.67}$Sr$_{0.33}$MnO$_3$ (LSMO) and the high-temperature…

Superconductivity · Physics 2009-04-15 M. van Zalk , M. Veldhorst , A. Brinkman , J. Aarts , H. Hilgenkamp

We examine the statistical mechanics of spin-ice materials with a [100] magnetic field. We show that the approach to saturated magnetisation is, in the low-temperature limit, an example of a 3D Kasteleyn transition, which is topological in…

Statistical Mechanics · Physics 2008-03-03 Ludovic D. C. Jaubert , J. T. Chalker , Peter C. W. Holdsworth , R. Moessner

We interpret recent measurements of the zero field muon relaxation rate in the frustrated magnetic pyrochlore Dy$_2$Ti$_2$O$_7$ as resulting from the quantum diffusion of muons in the substance. In this scenario, the plateau observed at low…

Strongly Correlated Electrons · Physics 2015-06-04 P. Quémerais , P. McClarty , R. Moessner

An analysis is presented of the behaviour of muons in the low-temperature state in spin ice. It is shown in detail how the behavior observed in some previous muon experiments on spin ice in a weak transverse field may result from the…

Strongly Correlated Electrons · Physics 2012-04-06 S. J. Blundell

Recent work has highlighted remarkable effects of classical thermal fluctuations in the dipolar spin ice compounds, such as "artificial magnetostatics", manifesting as Coulombic power-law spin correlations and particles behaving as…

Strongly Correlated Electrons · Physics 2011-10-11 Kate A. Ross , Lucile Savary , Bruce D. Gaulin , Leon Balents

The thermal equilibrium properties of the spin-ice material DTO, including specific heat, magnetization, and spin correlations, could be successfully reproduced by a model featuring magnetic interactions up to the third nearest neighbor and…

Strongly Correlated Electrons · Physics 2025-04-14 Mariano Marziali Bermudez , R. A. Borzi , D. A. Tennant , S. A. Grigera

Motivated by recent experiments on Ba$_3$Cr$_2$O$_8$, we propose a theory describing low-temperature properties in magnetic field $h$ of dimer spin-$\frac12$ systems on a stacked triangular lattice with spatially anisotropic exchange…

Strongly Correlated Electrons · Physics 2014-05-06 O. I. Utesov , A. V. Syromyatnikov

We investigate the spin-glass transition in the strongly frustrated well-known compound $Fe_2TiO_5$. A remarkable feature of this transition, widely discussed in the literature, is its anisotropic properties: the transition manifests itself…

Disordered Systems and Neural Networks · Physics 2021-06-16 P. G. LaBarre , D. Phelan , Y. Xin , F. Ye , T. Besara , T. Siegrist , S. V. Syzranov , S. Rosenkranz , A. P. Ramirez

The nature of the low temperature ground state of the pyrochlore compound Tb2Ti2O7 remains a puzzling issue. Dynamic fluctuations and short-range correlations persist down to 50 mK, as evidenced by microscopic probes. In parallel,…

Strongly Correlated Electrons · Physics 2012-08-02 E. Lhotel , C. Paulsen , P. Dalmas de Réotier , A. Yaouanc , C. Marin , S. Vanishri

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

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