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The structure of dielectric perovskite BaZrO$_3$, long known to be cubic at room temperature without any structural phase transition with variation of temperature, has been recently disputed to have different ground state structures with…

Materials Science · Physics 2022-06-29 Dong-Hyeon Gim , Yeahan Sur , Yoon Han Lee , Jeong Hyuk Lee , Soonjae Moon , Yoon Seok Oh , Kee Hoon Kim

Fano resonance in molecular spectroscopy is reported with a dual-comb instrument. The effect is observed as asymmetric absorption lines of H12CN. Pulse chirping conditions in the gas cell are varied to show that Fano resonance is dependent…

Optics · Physics 2022-06-29 Philippe Guay , Mathieu Walsh , Jérôme Genest

Miniaturized spectrometry system is playing an essential role for materials analysis in the development of in-situ or portable sensing platforms across research and industry. However, there unavoidably exists trade-offs between the…

The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…

Optics · Physics 2024-03-07 Meng Qi , Wenrong Wang , Yuan-ji Li , Jin-xia Feng , Kuan-shou Zhang

The photoion spectrum of atomic potassium was measured over the 3s -> np excitation region with the photoion time-of-flight method and monochromatized synchrotron radiation. An unusual spectrum with paired windows structure was found…

We develop a simple thermodynamic model to describe the heat transfer mechanisms and generation of acoustic waves in photoacoustic Raman spectroscopy by small particulate suspensions in a gas. Using Langevin methods to describe the thermal…

Quantum Physics · Physics 2009-11-10 Kunal K. Das , Yuri V. Rostovtsev , Kevin Lehmann , Marlan O. Scully

The electronic structure of two V-based ladder compounds, the quarter-filled NaV$_2$O$_5$ in the symmetric phase and the iso-structural half-filled CaV$_2$O$_5$ is investigated by ab initio calculations. Based on the bandstructure we…

Other Condensed Matter · Physics 2009-11-10 J. Spitaler , E. Ya. Sherman , H. G. Evertz , C. Ambrosch-Draxl

We calculate the radio frequency (RF) spectrum of fermionic atoms near a narrow Feshbach resonance, explaining observations made in ultracold samples of $^6\rm{Li}$ [E. L. Hazlett {\it et al.}, Phys. Rev. Lett. {\bf 108}, 045304 (2012)]. We…

Quantum Gases · Physics 2014-01-31 Junjun Xu , Qiang Gu , Erich J. Mueller

For many materials, Raman spectra are intricately structured and provide valuable information about compositional stoichiometry and crystal quality. Here we use density-functional theory calculations, mass approximation, and the Raman…

Materials Science · Physics 2024-09-04 Nima Ghafari Cherati , I. Abdolhosseini Sarsari , Arsalan Hashemi , Tapio Ala-Nissila

We present a systematic first-principles study of the phonon spectrum of hexagonal YMnO3 in ferroelectric (multiferroic) phase. We investigated in detail the low-energy phonon modes, their dispersion, symmetry, as well as the infrared…

Materials Science · Physics 2012-07-30 Konstantin Z. Rushchanskii , Marjana Ležaić

Despite its simple crystal structure, layered boron nitride features a surprisingly complex variety of phonon-assisted luminescence peaks. We present a combined experimental and theoretical study on ultraviolet-light emission in hexagonal…

The polarized Raman scattering spectra of nonsuperconducting $\alpha$-FeTe and of the newly discovered, As-free superconductor Fe$_{1.03}$Se$_{0.3}$Te$_{0.7}$ are measured at room temperature on single crystals. The phonon modes are…

Superconductivity · Physics 2009-05-11 Tian-Long Xia , D. Hou , S. C. Zhao , A. M. Zhang , G. F. Chen , J. L. Luo , N. L. Wang , J. H. Wei , Z. -Y. Lu , Q. M. Zhang

The novel graphene allotropes $\alpha$-, $\beta$-, and $\gamma$-graphyne derive from graphene by insertion of acetylenic groups. The three graphynes are the only members of the graphyne family with the same hexagonal symmetry as graphene…

Mesoscale and Nanoscale Physics · Physics 2013-08-28 Valentin N. Popov , Philippe Lambin

We performed a polarized Raman scattering study of quasi-one-dimensional superconductor K$_2$Cr$_3$As$_3$. We detect two A$_1^\prime$ phonons and three E$^\prime$ phonons. One of the A$_1^\prime$ modes exhibits a nearly…

Superconductivity · Physics 2015-08-19 W. -L. Zhang , H. Li , Dai Xia , H. W. Liu , Y. -G. Shi , J. L. Luo , Jiangping Hu , P. Richard , H. Ding

High-harmonic spectroscopy is a promising candidate for imaging electronic structures and dynamics in condensed matter by all-optical means and with unprecedented temporal resolution. We investigate harmonic spectra from finite, hexagonal…

Mesoscale and Nanoscale Physics · Physics 2024-01-10 Helena Drüeke , Dieter Bauer

We use frequency entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive index sensing of a…

Quantum Physics · Physics 2014-03-27 Dmitry A. Kalashnikov , Zhenying Pan , Arseniy I. Kuznetsov , Leonid A. Krivitsky

Raman spectroscopy is used to study magnetic excitations in the quasi one dimensional $S=1/2$ quantum spin systems Cu(Qnx)(Cl$_{1-x}$Br$_x$)$_2$. The low energy spectrum is found to be dominated by a two-magnon continuum as expected from…

Strongly Correlated Electrons · Physics 2016-03-15 G. Simutis , S. Gvasaliya , F. Xiao , C. P. Landee , A. Zheludev

We investigated the effects of temperature and magnetic field on the electronic structure of hexagonal RMnO3 (R = Gd, Tb, Dy, and Ho) thin films using optical spectroscopy. As the magnetic ordering of the system was disturbed, a systematic…

Strongly Correlated Electrons · Physics 2010-05-17 Woo Seok Choi , Soon Jae Moon , Sung Seok A. Seo , Daesu Lee , Jung Hyuk Lee , Pattukkannu Murugavel , Tae Won Noh , Yun Sang Lee

Recent demonstrations of ultracoherent nanomechanical resonators introduce the prospect of new protocols for solid state sensing applications. Here, we propose to use two coupled ultracoherent resonator modes on a Si$_3$N$_4$ membrane for…

Applied Physics · Physics 2020-07-22 J. Košata , O. Zilberberg , Christian L. Degen , R. Chitra , A. Eichler

We present a practical method to compute the vibrational resonant Raman spectra in solids with delocalized excitations. We apply this approach to the study of tetrahedrous amorphous carbon. We determine the vibrational eigenmodes and…

Materials Science · Physics 2009-11-07 Mickael Profeta , Francesco Mauri